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arXiv:cond-mat/0609140 · Physical Review B

Spin-nematic phases in models of correlated electron systems: A numerical study

Sylvain Capponi, Fakher F. Assaad

Published Jan 16, 2007• 5 citations
arXivHTMLPDF

Abstract

Strongly interacting systems are known to often spontaneously develop exotic ground states under certain conditions. For instance, spin nematic phases have been discovered in various magnetic models. Such phases, which break spin symmetry but have no net local magnetization, have also been proposed by Nersesyan et al. [J. Phys.: Condens. Matter 3, 3353 (1991)] in the context of electronic models. We introduce a $N$-flavor microscopic model that interpolates from the large-$N$ limit, where mean field is valid and such a nematic phase occurs, to the more realistic $N=1$ case. By using a sign-free quantum Monte Carlo, we show the existence of a spin nematic phase (analogous to a spin flux phase) for finite $N$; when $N$ decreases, quantum fluctuations increase and this phase ultimately disappears in favor of an $s$-wave superconducting state. We also show that this nematic phase extends up to a finite critical charge doping. Dynamical studies allow us to clarify the Fermi surface property: in the nematic phase at half-filling, it consists of four points and the low-energy structure has a Dirac conelike shape. Under doping, we observe clear signatures of Fermi pockets around these points. This is one of the few examples where numerical simulations show how quantum fluctuations can destroy a large-$N$ phase.

DOI
10.1103/physrevb.75.045115

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Strongly interacting systems are known to often spontaneously develop exotic ground states under certain conditions. For instance, spin nematic phases have been discovered in various magnetic models. Such phases, which break spin symmetry but have no net local magnetization, have also been proposed by Nersesyan et al. [J. Phys.: Condens. Matter 3, 3353 (1991)] in the context of electronic models. We introduce a NNN-flavor microscopic model that interpolates from the large-NNN limit, where mean field is valid and such a nematic phase occurs, to the more realistic N=1N=1N=1 case. By using a sign-free quantum Monte Carlo, we show the existence of a spin nematic phase (analogous to a spin flux phase) for finite NNN; when NNN decreases, quantum fluctuations increase and this phase ultimately disappears in favor of an sss-wave superconducting state. We also show that this nematic phase extends up to a finite critical charge doping. Dynamical studies allow us to clarify the Fermi surface property: in the nematic phase at half-filling, it consists of four points and the low-energy structure has a Dirac conelike shape. Under doping, we observe clear signatures of Fermi pockets around these points. This is one of the few examples where numerical simulations show how quantum fluctuations can destroy a large-NNN phase.
"This thesis is devoted to the investigation of the quantum liquid crystal phases in strongly correlated electronic systems. Such phases are characterized by their partially broken spatial symmetries and are observed in various strongly correlated systems as being summarized in Chapter 1. In quantum liquid crystal phases formed by fermions, behaviors beyond Landau's theory of the Fermi liquids appear naturally, signed by the absence of well-defined quasiparticle excitations. Although quantum liquid crystal phases often involve strong-coupling physics, the associated symmetry analysis can often be carried out also in a relatively weak coupling regime and this is the main approach taken in this thesis. Two different quantum liquid crystal phases, the nematic state and the smectic state, are studied in Chapters 2 and 3 respectively, by investigating various instabilities of a Landau Fermi liquid. A nematic phase is a state that breaks the rotational symmetry spontaneously but preserves the translational symmetries. It can be reached by the Pomeranchuk instability of a Landau Fermi liquid. The Pomeranchuk instability in the charge (spin-singlet) sector of a Fermi liquid was studied previously within a random phase approximation and by a high-dimensional bosonization method. In Chapter 2, we concentrate on the Pomeranchuk instability in the spin-triplet sector, and two different classes of ordered phases are discovered, dubbed the a and ,8-phases by analogy to the superfluid 3He-A and B-phases. The Fermi surfaces in the a-phases exhibit spontaneous anisotropic distortions, while in the ,8-phases the Fermi surfaces remain circular or spherical with topologically non-trivial spin configurations in momentum space. The behaviors of the low energy bosonic excitations are studied both in the order phases (a and .B) and at the quantum critical point separating the ordered phases from the Fermi liquid phase. In Chapter 3, the smectic phase and the quantum phase transition between a metallic nematic state and a metallic smectic phase are investigated using the random phase approximation, by considering the formation of a unidirectional charge density wave in an electronic nematic state. The associated quantum critical point is investigated within the Hertz-Millis approach. Non-Fermi liquid behaviors are discovered both at the quantum phase transition and in the smectic ordered phase. The theory we studied here provides a simple description for the so-called ""fluctuating stripe"" phase in cuprates. Similar to its classical counterpart, the phase transition between the nematic and smectic phases are described by a ""gauge-like"" theory as required by the rotational invariance in close analogy with the McMillan-deGennes theory of the smectic-nematic phase transition in classical liquid crystals. However, unlike the classical McMillandeGennes theory, in which the coupling between the ""gauge-like"" nematic fluctuations and the ""matter-like"" smectic fields is relevant, in the sense of renormalization group, this coupling is irrelevant at the quantum phase transition. This property enables the study of low energy fluctuations and the fate of fermions near this quantum critical point. In Chapter 4, quantum liquid crystal phases with a broken time-reversal symmetry are investigated. We start by studying the general scenario of timereversal symmetry breaking phases in the absence of magnetic ordering in systems with long-lived low-energy fermionic quasiparticle excitations in two dimensions. Using a Berry phase approach, we classified possible time-reversal symmetry breaking phases by the accompanying spatial symmetry breaking patterns. Two of the simplest situations are referred to as the type I state, which breaks simultaneously the space-inversion symmetry and the time-reversal symmetry, and the type I I state, in which the chiral symmetry is broken in addition to the breaking of the time-reversal symmetry. Although the starting point is general and has little relation with the quantum liquid crystal phases, both type I and type II states defined above are realized by (generalized) Pomeranchuk instabilities. In fact , a type I I state is usually a nematic state which also breaks the time-reversal symmetry. Interestingly, the type II states also shows spontaneously generated Hall effect even in the absence of a magnetic field, which is known as the spontaneous anomalous Hall effect. In Chapter 5, we investigate the stability of a quadratic band-crossing point in two-dimensional fermionic systems that provide an explicit example, within well controlled approximations, for the nematic ordering discussed in Chapter 2 and spontaneous anomalous Hall effect discussed in Chapter 4. At the non-interacting level, we show that a quadratic band-crossing point exists and is topologically stable when the Berry flux of this crossing point is ±27r and the point symmetry group at this point has either fourfold or sixfold rotational symmetries. Strikingly, we find that this would-be topologically stable quadratic band-crossing is marginally unstable against short-range interactions: a quadratic band-crossing point in two dimensions is unstable against shortrange repulsion, no matter how weak! Four ordered phases are found in this system, the quantum anomalous Hall state, the quantum spin Hall phase, the nematic phase, and the nematic-spin-nematic phase."
Nematicity is a well-known property of liquid crystals and has been recently discussed in the context of strongly interacting electrons. An electronic nematic phase has been seen in many experiments in certain strongly correlated materials, in particular, in the pseudogap phase generic to many hole-doped cuprate superconductors. Recent measurements in high Tc superconductors have shown that even if the lattice is perfectly rotationally symmetric, the ground state can still have strongly nematic local properties. Our study of the two-dimensional one-band Hubbard model provides strong support for the recent experimental results on local rotational C4 symmetry breaking. The variational cluster approach is used here to show the possibility of an electronic nematic state and the proximity of the underlying symmetry-breaking ground state within the Hubbard model. We identify this nematic phase in the overdoped region and show that the local nematicity decreases with increasing electron filling. Our results also indicate that strong Coulomb interaction may drive the nematic phase into a phase similar to the stripe structure. The calculated spin (magnetic) correlation function in momentum space shows the effects resulting from real-space nematicity.
The understanding of matter does not only require a precise analysis of individual characteristics of the fundamental constituents, but also the study of their collective behavior.Solid state physics, and in particular research in strongly correlated electron systems, deals with such collective phenomena.The properties of the electrons, charge and spin quantum numbers, do not on their own explain the rich world of states of matter, however mutual interactions lead to various states or phases of matter.This work focuses on phases in quantum spin systems.On the basis of the Heisenberg model one (1D) and two dimensional (2D) spin lattices are investigated.In a first part the bilayer Heisenberg Model and the 2D Kondo necklace model are studied.Both models exhibit a quantum phase transition between an ordered and disordered phase.For small interlayer couplings the models have antiferromagnetic long-range order, which is destroyed by increasing the coupling.However, even in the disordered phase the models show global features in terms of collective excitations called magnons.Coming from the disordered phase the gapped magnons condense at a critical coupling and form the order of the ordered phase.Here, another interesting question arises, namely that of the coupling of a single doped hole to such critical fluctuations.A self-consistent Born approximation predicts that the doped hole couples to the magnons such that the quasiparticle residue vanishes at the quantum critical point.In this work the delicate question about the fate of the quasiparticle residue across the quantum phase transition is also tackled by means of large scale quantum Monte Carlo simulations.Furthermore the dynamics of a single hole doped in the magnetic background is investigated.
This thesis considers various strongly correlated quantum phases in solid state and cold atom spin systems. In the first part we focus on phases emerging in multi-orbital materials. We study even-parity spin-triplet superconductivity originating from Hund's coupling between t2g orbitals and investigate the effect of spin-orbit interaction on spin-triplet and spin-singlet pairing. Various aspects of the pairing state are discussed against the backdrop of the spin-triplet superconductor Sr2RuO4. Motivated by the remarkable phenomena observed in the bilayer compound Sr3Ru2O7, which point to the formation of an electronic nematic phase in the presence of critical fluctuations, we investigate how such a broken symmetry state emerges from electronic interactions. Since the broken x-y symmetry is revealed experimentally by applying a small in-plane magnetic field component, we examine nematic phases in a bilayer system and the role of the in-plane magnetic field using a phenomenological approach. In addition, we propose a microscopic mechanism for nematic phase formation specific to Sr3Ru2O7. The model is based on a realistic multi-orbital band structure and local and nearest neighbour interactions. Considering all t2g-orbital derived bands on an equal footing, we find a nematic quantum critical point and a nearby meta-nematic transition in the phase diagram. This finding harbours important implications for the phenomena observed in Sr3Ru2O7. The second part is devoted to the study of the anisotropic bilinear biquadratic spin-1 Heisenberg model, where the existence of an unusual direct phase transition between a spin-nematic phase and a dimerized valence bond solid phase in the quasi-1D limit was conjectured based on Quantum Monte Carlo simulations. We establish the quasi-1D phase diagram using a large-N Schwinger boson approach and show that the phase transition is largely conventional except possibly at two particular points. We further discuss how to realize and to detect such phases in an optical lattice.
In this thesis, we investigate several topics pertaining to emergent collective quantum phenomena in the domain of correlated fermions, using the quantum Monte Carlo method. They display exotic low temperature phases as well as phase transitions which are beyond the Landau–Ginzburg theory. The interplay between three key points is crucial for us: fermion statistics, many body effects and topology. We highlight the following several achievements: 1. Successful modeling of continuum field theories with lattice Hamiltonians, 2. their sign-problem-free Monte Carlo simulations of these models, 3. and numerical results beyond mean field descriptions. First, we consider a model of Dirac fermions with a spin rotational invariant inter- action term that dynamically generates a quantum spin Hall insulator. Surprisingly, an s-wave superconducting phase emerges due to the condensation of topological de- fects of the spin Hall order parameter. When particle-hole symmetry is present, the phase transition between the topological insulator and the superconducting phase is an example of a deconfined quantum critical point(DQCP). Although its low energy effec- tive field theory is purely bosonic, the exact conservation law of the skyrmion number operator rules out the possibility of realizing this critical point in lattice boson models. This work is published in Ref. [1]. Second, we dope the dynamically generated quantum spin Hall insulator mentioned above. Hence it is described by a field theory without Lorentz invariance due to the lack of particle-hole symmetry. This sheds light on the extremely hot topic of twisted bilayergraphene: Why is superconductivity generated when the repulsive Coulomb interaction is much stronger than the electron-phonon coupling energy scale? In our case, Cooper pairs come from the topological skyrmion defects of the spin current order parameter, which are charged. Remarkably, the nature of the phase transition is highly non-mean-field-like: one is not allowed to simply view pairs of electrons as single bosons in a superfluid-Mott insulator transition, since the spin-current order parameter can not be ignored. Again, due to the aforementioned skyrmions, the two order parameters are intertwined: One phase transition occurs between the two symmetry breaking states. This work is summarized in Ref. [2]. Third, we investigate the 2 + 1 dimensional O(5) nonlinear sigma model with a topological Wess-Zumino-Witten term. Remarkably, we are able to perform Monte Carlo calculations with a UV cutoff given by the Dirac Landau level quantization. It is a successful example of simulating a continuous field theory without lattice regularization which leads to an additional symmetry breaking. The Dirac background and the five anti-commuting Dirac mass terms naturally introduce the picture of a non-trivial Berry phase contribution in the parameter space of the five component order parameter. Using the finite size scaling method given by the flux quantization, we find a stable critical phase in the low stiffness region of the sigma model. This is a candidate ground state of DQCP when the O(5) symmetry breaking terms are irrelevant at the critical point. Again, it has a bosonic low energy field theory which is seemingly unable to be realized in pure boson Hamiltonians. This work is summarized in Ref. [3].
Frustration in quantum spin systems promote a variety of novel quantum phases. An important example is the frustrated spin-1 model on the square lattice with the nearest-neighbor bilinear (J1{J}_{1}J1​) and biquadratic (K1{K}_{1}K1​) interactions. We provide strong evidence for a nematic spin liquid phase in a range of K1/J1{K}_{1}/{J}_{1}K1​/J1​ near the SU(3)-symmetric point (J1=K1{J}_{1}={K}_{1}J1​=K1​), based on the linear flavor-wave theory and extensive density matrix renormalization group calculation. This phase displays no spin dipolar or quadrupolar order, preserves translational symmetry but spontaneously breaks C4{C}_{4}C4​ lattice rotational symmetry, and possesses fluctuations peaked at the wave vector $(\ensuremath{\pi},2\ensuremath{\pi}/3)$. The spin excitation gap drops rapidly with system size and appears to be gapless, and the nematic order is attributed to the dominant $(\ensuremath{\pi},2\ensuremath{\pi}/3)$ fluctuations. Our results provide a novel mechanism for electronic nematic order and, more generally, open up a new avenue to explore frustration-induced exotic ground states.