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arXiv:cond-mat/0607257 · Physical Review E

Density of Yang-Lee zeros for the Ising ferromagnet

Seung‐Yeon Kim

Published Jul 26, 2006• 26 citations
arXivHTMLPDF

Abstract

The densities of Yang-Lee zeros for the Ising ferromagnet on the L x L square lattice are evaluated from the exact grand partition functions (L=3 approximately 16). The properties of the density of Yang-Lee zeros are discussed as a function of temperature T and system size L. The three different classes of phase transitions for the Ising ferromagnet--first-order phase transition, second-order phase transition, and Yang-Lee edge singularity--are clearly distinguished by estimating the magnetic scaling exponent yh from the densities of zeros for finite-size systems. The divergence of the density of zeros at Yang-Lee edge in high temperatures (Yang-Lee edge singularity), which has been detected only by the series expansion until now for the square-lattice Ising ferromagnet, is obtained from the finite-size data. The identification of the orders of phase transitions in small systems is also discussed using the density of Yang-Lee zeros.

DOI
10.1103/physreve.74.011119

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The densities of Yang-Lee zeros for the Ising ferromagnet on the L x L square lattice are evaluated from the exact grand partition functions (L=3 approximately 16). The properties of the density of Yang-Lee zeros are discussed as a function of temperature T and system size L. The three different classes of phase transitions for the Ising ferromagnet--first-order phase transition, second-order phase transition, and Yang-Lee edge singularity--are clearly distinguished by estimating the magnetic scaling exponent yh from the densities of zeros for finite-size systems. The divergence of the density of zeros at Yang-Lee edge in high temperatures (Yang-Lee edge singularity), which has been detected only by the series expansion until now for the square-lattice Ising ferromagnet, is obtained from the finite-size data. The identification of the orders of phase transitions in small systems is also discussed using the density of Yang-Lee zeros.
The Ising ferromagnet, consisting of magnetic spins, is the simplest system showing phase transitions and critical phenomena at finite temperatures. The Ising ferromagnet has played a central role in our understanding of phase transitions and critical phenomena. Also, the Ising ferromagnet explains the gas-liquid phase transitions accurately. In particular, the Ising ferromagnet in a nonzero magnetic field has been one of the most intriguing and outstanding unsolved problems. We study analytically the partition function zeros in the complex magnetic-field plane and the Yang-Lee edge singularity of the infinite-range Ising ferromagnet in an external magnetic field. In addition, we compare the Yang-Lee edge singularity of the infinite-range Ising ferromagnet with that of the square-lattice Ising ferromagnet in an external magnetic field.
We revisit the somewhat less studied problem of Yang-Lee zeros of the Ising antiferromagnet. For this purpose, we study two models, the nearest-neighbor model on a square lattice and the more tractable mean-field model corresponding to infinite-ranged coupling between all sites. In the high-temperature limit, we show that the logarithm of the Yang-Lee zeros can be written as a series in half odd integer powers of the inverse temperature, k, with the leading term ∼k^{1/2}. This result is true in any dimension and for arbitrary lattices. We also show that the coefficients of the expansion satisfy simple identities (akin to sum rules) for the nearest-neighbor case. These identities are verified numerically by computing the exact partition function for a two-dimensional square lattice of size 16×16. For the mean-field model, we write down the partition function (termed the mean-field polynomials) for the ferromagnetic (FM) and antiferromagnetic (AFM) cases and derive from them the mean-field equations. We analytically show that at high temperatures the zeros of the AFM mean-field polynomial scale as ∼k^{1/2} as well. Using a simple numerical method, we find the roots lie on certain curves (the root curves), in the thermodynamic limit for the mean-field polynomials for the AFM case as well as for the FM one. Our results show a new root curve that was not found earlier. Our results also clearly illustrate the phase transition expected for the FM and AFM cases, in the language of Yang-Lee zeros. Moreover, for the AFM case, we observe that the root curves separate two distinct phases of zero and nonzero complex staggered magnetization, and thus depict a complex phase boundary.
The isothermal magnetization m(H) of the metamagnet FeCl2 is measured in axial magnetic fields 0≤µ0Ha≤12 T at temperatures 34≤T≤53 K above the Néel temperature, where the system is essentially a two-dimensional Ising ferromagnet. The analysis of the data indicates experimental accessibility of the critical exponent µ of the Yang-Lee edge singularities. They manifest themselves in divergences of the density functions g(θ), which quantify the distribution of the zeros of the partition function on the Lee-Yang unit circle in the complex plane. In accordance with the hypothesis of universality, a critical exponent close to the theoretical prediction for the two-dimensional Ising ferromagnet, µ = -1/6, is found.
We study Yang-Lee zeros as they approach the thermodynamic limit of the two-dimensional (2D) nearest-neighbor antiferromagnetic Ising model on square and triangular lattices. We employ the numerical linked cluster expansion (NLCE) equipped with exact enumeration (EE) of the partition function to estimate the Laplacian of the free energy, which is proportional to the zeros density. Using a modified NLCE, where the expansion can be carried directly on the Yang-Lee zeros of the involved clusters, we estimate the density of Yang-Lee zeros in the thermodynamic limit. NLCE gives significantly more zeros than EE in the complex field plane providing more insights on how the root curves look in the thermodynamic limit. For the square lattice at $T\ensuremath{\ll}{T}_{c}$, the results suggest that two vertical lines at $\ifmmode\pm\else\textpm\fi{}{h}_{c}(T)$ in the complex field plane (i.e., two concentric circles in the complex fugacity plane) are the thermodynamic root curves. A similar picture is found for the triangular lattice for phase transitions at large values of magnetic field while further study is needed for phase transitions at smaller values of magnetic field. The convergence of the NLCE and (EE) calculations of the partition function to the thermodynamic limit is studied in both lattices and the temperature-field phase diagram is obtained from Yang-Lee zeros using both methods. This NLCE-based approach will facilitate the study of different types of phase transitions using Yang-Lee zeros in future research.
There exists the famous circle theorem on the Yang-Lee zeros of the ferromagnetic Ising model. However, the Yang-Lee zeros of the antiferromagnetic Ising model are much less well understood than those of the ferromagnetic model. The precise distribution of the Yang-Lee zeros of the antiferromagnetic Ising model only with nearest-neighbor interaction J on LxL square lattices is determined as a function of temperature a=e(2betaJ) (J<0), and its relation to the phase transitions is investigated. In the thermodynamic limit (L-->infinity), the distribution of the Yang-Lee zeros of the antiferromagnetic Ising model cuts the positive real axis in the complex x=e(-2betaH) plane, resulting in the critical magnetic field +/-H(c)(a), where H(c)>0 below the critical temperature a(c)=square root of 2-1. The results suggest that the value of the scaling exponent y(h) is 1 along the critical line for a<a(c).
The Ising model in an external magnetic field is one of the most outstanding and intriguing unsolved problems. One of the important properties of the Ising model in an external magnetic field is the Yang-Lee edge singularity. The zeros in the complex magnetic-field plane of the grand partition function of the Ising model on a honeycomb lattice in an external magnetic field are exactly calculated by using the exact integer values for the density of states on L × 2L honeycomb lattices (up to L = 14). The critical line of the Yang-Lee edge singularity of the Ising model on a honeycomb lattice in an external magnetic field is accurately investigated from its Yang-Lee zeros.