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arXiv:cond-mat/0606656

From Cooper-pairs to resonating bipolarons

J. Ranninger

Published Jun 26, 2006• 0 citations
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Abstract

After a short review of the different physics in the weak and strong coupling regime, resulting in amplitude fluctuation controlled Cooper pair superconductivity and phase fluctuation controlled superfluidity of tightly bound local polaron pairs, we suggest a scenario for the cross-over regime between those two. It is based on the idea of resonating Bipolarons inside a Fermi sea of uncorrelated electrons, similar to the Feshbach resonance in Fermionic gases in optical traps. Due to the competition between amplitude and phase correlations such systems in the cross-over regime can exhibit a superconductor to insulator transition upon varying the strength of that resonance.

DOI
10.48550/arxiv.cond-mat/0606656

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After a short review of the different physics in the weak and strong coupling regime, resulting in amplitude fluctuation controlled Cooper pair superconductivity and phase fluctuation controlled superfluidity of tightly bound local polaron pairs, we suggest a scenario for the cross-over regime between those two. It is based on the idea of resonating Bipolarons inside a Fermi sea of uncorrelated electrons, similar to the Feshbach resonance in Fermionic gases in optical traps. Due to the competition between amplitude and phase correlations such systems in the cross-over regime can exhibit a superconductor to insulator transition upon varying the strength of that resonance.
We address the phase of a highly polarized Fermi gases across a narrow Feshbach resonance starting from the problem of a single down-spin fermion immersed in a Fermi sea of up spins. Both polaron and pairing states are considered using the variational wave function approach, and we find that the polaron-to-pairing transition will take place on the BCS side of the resonance, strongly in contrast to a wide resonance where the transition is located at the BEC side. For the pairing phase, we find the critical strength of the repulsive interaction between pairs above which the mixture of pairs and fermions will not phase separate. Therefore, nearby a narrow resonance, it is quite likely that magnetism can coexist with sss-wave BCS superfluidity at large Zeeman fields, which is a remarkable property absent in conventional BCS superconductors (or fermion-pair superfluids).
We review a series of exact, analytical and numerical results obtained on the adiabatic Holstein–Hubbard model, many of which are new and non-trivial. We study next the role of the quantum lattice fluctuations that were initially neglected. The possibility of having high- T c bipolaronic superconductors is analysed on the basis of these results. We suggest that models that involve only electron–phonon coupling are very unlikely to produce bipolaronic superconductivity, which is prevented by the spatial ordering of the bipolarons associated with a lattice instability. This is due to a very large effective mass of the bipolarons that can be related to the large Peierls–Nabarro energy barrier required to move these bipolarons through the lattice in the adiabatic limit. We conjecture that high- T c superconductivity originates specifically from the exceptionally well-balanced competition between electron–phonon coupling and electron–electron repulsion. In the restricted region in which, within the mean field approach, the energy of a bipolaron is close to those of two polarons, a new type of electron pairing occurs by formation of pairs of polarons in the spin singlet state. Such a polaron pair, called a spin resonant bipolaron (SRB), is not the standard bipolaron (both could exist in the adiabatic case). Its Peierls–Nabarro energy barrier can be sharply depressed, almost to zero. As a result of quantum lattice fluctuations, its tunnelling energy is sharply enhanced. Then, superconductivity could persist for a relatively large electron–phonon coupling, with an unusually large critical temperature as a Bose condensate of SRBs before becoming, at larger coupling and in any case, an insulating spin–Peierls polaronic phase.
We consider systems where the amplitude and the phase of a superfluid order parameter are controlled independently by local, respectively non-local phase correlations of the internal degrees of freedom of quasi-particles which characterize the different phases of such fermionic systems. A possible realization of such a situation is when pairing into the bosonic entities occurs via resonant scattering of itinerant fermionic particles. Examples for that are the ultracold fermionic gases in optical traps and lattices, the correlated electronic systems and strongly coupled electron-phonon systems, such as seen in the high Tc cuprates. We demonstrate the occurrence of a quantum phase transition from a superfluid to a phase uncorrelated boson liquid state in such systems, which is controlled by the competing effects of long and short range phase correlations of the constituents of composite quasi-particles.
The ability to control the interaction strength between atoms within strongly interacting Fermi gases by sweeping a magnetic field across a Feshbach resonance provides a powerful experimental system in which to study many-body physics. One example is the crossover from a Bose-Einstein condensate (BEC) regime, in which the atoms are strongly coupled into pairs, to the weak-coupling regime that mimics Bardeen-Cooper-Schrieffer (BCS) coupling of electrons in superconducting metals. Although behavior on either side of the resonance is fairly well understood, of immediate interest is to find out what happens in the BEC-BCS crossover regime. However, determining the relative contributions of atom pairing mechanisms is an experimental and theoretical challenge.
We study resonantly-paired s-wave superfluidity in a degenerate gas of two species (hyperfine states labeled by ↑, ↓) of fermionic atoms when the numbers N↑ and N↓ of the two species are unequal, i.e., the system is "polarized." We find that the continuous crossover from the Bose-Einstein condensate (BEC) limit of tightly-bound diatomic molecules to the Bardeen-Cooper-Schrieffer (BCS) limit of weakly correlated Cooper pairs, studied extensively at equal populations, is interrupted by a variety of distinct phenomena under an imposed population difference ΔN ≡ N↑ - N↓. Our findings are summarized by a "polarization" (ΔN) versus Feshbach-resonance detuning (δ) zero-temperature phase diagram, which exhibits regions of phase separation, a periodic FFLO superfluid, a polarized normal Fermi gas and a polarized molecular superfluid consisting of a molecular condensate and a fully polarized Fermi gas. We describe numerous experimental signatures of such phases and the transitions between them, in particular focusing on their spatial structure in the inhomogeneous environment of an atomic trap. © 2006 Elsevier Inc. All rights reserved.
Electrons coupled to local lattice deformations end up in self-trapped localized molecular states involving their binding into bipolarons when the coupling is stronger than a certain critical value. Below that value they exist as essentially itinerant electrons. We propose that the abrupt crossover between the two regimes can be described by resonant pairing similar to the Feshbach resonance in binary atomic collision processes. Given the intrinsically local nature of the exchange of pairs of itinerant electrons and localized bipolarons, we demonstrate the occurrence of such a resonance on a finite-size cluster made out of metallic atoms surrounding a polaronic ligand center.