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BEC-BCS crossover, phase transitions and phase separation in polarized resonantly-paired superfluids

Daniel E. Sheehy, Leo Radzihovsky

Published Aug 1, 2007• 100 citations
OpenAlex

Abstract

We study resonantly-paired s-wave superfluidity in a degenerate gas of two species (hyperfine states labeled by ↑, ↓) of fermionic atoms when the numbers N↑ and N↓ of the two species are unequal, i.e., the system is "polarized." We find that the continuous crossover from the Bose-Einstein condensate (BEC) limit of tightly-bound diatomic molecules to the Bardeen-Cooper-Schrieffer (BCS) limit of weakly correlated Cooper pairs, studied extensively at equal populations, is interrupted by a variety of distinct phenomena under an imposed population difference ΔN ≡ N↑ - N↓. Our findings are summarized by a "polarization" (ΔN) versus Feshbach-resonance detuning (δ) zero-temperature phase diagram, which exhibits regions of phase separation, a periodic FFLO superfluid, a polarized normal Fermi gas and a polarized molecular superfluid consisting of a molecular condensate and a fully polarized Fermi gas. We describe numerous experimental signatures of such phases and the transitions between them, in particular focusing on their spatial structure in the inhomogeneous environment of an atomic trap. © 2006 Elsevier Inc. All rights reserved.

Related papers

BEC-BCS Crossover in “Magnetized” Feshbach-Resonantly Paired Superfluids

Daniel E. Sheehy, Leo Radzihovsky

We map out the detuning-magnetization phase diagram for a magnetized (unequal number of atoms in two pairing hyperfine states) gas of fermionic atoms interacting via an s-wave Feshbach resonance (FR). The phase diagram is dominated by the coexistence of a magnetized normal gas and a singlet-paired superfluid with the latter exhibiting a BCS-Bose Einstein condensate crossover with reduced FR detuning. On the BCS side of strongly overlapping Cooper pairs, a sliver of finite-momentum paired Fulde-Ferrell-Larkin-Ovchinnikov magnetized phase intervenes between the phase-separated and normal states. In contrast, for large negative detuning a uniform, polarized superfluid, that is, a coherent mixture of singlet Bose-Einstein-condensed molecules and fully magnetized single-species Fermi sea, is a stable ground state.

arXiv:cond-mat/0508430•Physical Review Letters•Feb 13, 2006•330 citations

BCS-BEC CROSSOVER IN A SUPERFLUID FERMI GAS

Yoji Ohashi

We discuss the superfluid phase transition in a gas of Fermi atoms with a Feshbach resonance. A tunable pairing interaction associated with the Feshbach resonance is shown to naturally lead to the BCS-BEC crossover, where the character of superfluidity continuously changes from the weak-coupling Bardeen-Cooper-Schrieffer (BCS) type to the Bose-Einstein condensation (BEC) of tightly bound molecules, as one decreases the threshold energy 2ν of the Feshbach resonance. We also discuss effects of a trap, as well as the p-wave BCS-BEC crossover adjusted by a p-wave Feshbach resonance.

International Journal of Modern Physics B•Dec 15, 2006•1 citation

BCS to BEC evolution and quantum phase transitions in superfluid Fermi gases

M. Iskin

This thesis focuses on the analysis of Bardeen-Cooper-Schrieffer (BCS) \nto Bose-Einstein condensation (BEC) evolution in ultracold superfluid \nFermi gases when the interaction between atoms is varied. The tuning of \nattractive interactions permits the ground state of the system to evolve from a weak \nfermion attraction BCS limit of loosely bound and largely overlapping Cooper pairs \nto a strong fermion attraction limit of tightly bound small bosonic molecules \nwhich undergo BEC. \nThis evolution is accompanied by anomalous behavior of many superfluid \nproperties, and reveals several quantum phase transitions. \nThis thesis has two parts: \nIn the first part, I analyze zero and nonzero orbital angular momentum \npairing effects, and show that a quantum phase transition occurs for \nnonzero angular momentum pairing, unlike the $s$-wave case where the BCS \nto BEC evolution is just a crossover. \nIn the second part, I analyze two-species fermion mixtures with mass and \npopulation imbalance in continuum, trap and lattice models. In contrast with \nthe crossover physics found in the mass and population balanced mixtures, \nI demonstrate the existence of phase transitions between normal and \nsuperfluid phases, as well as phase separation between superfluid (paired) \nand normal (excess) fermions in imbalanced mixtures as a function of scattering \nparameter and mass and population imbalance.

•Jun 29, 2007•0 citations

Imbalanced Feshbach-resonant Fermi gases

Leo Radzihovsky, Daniel E. Sheehy

We present an overview of recent developments in species-imbalanced (‘polarized’) Feshbach-resonant Fermi gases. We summarize the current status of thermodynamics of these systems in terms of a phase diagram as a function of the Feshbach resonance detuning, polarization and temperature. We review instabilities of the s -wave superfluidity across the Bose–Einstein condensation-to-Bardeen–Cooper–Schrieffer crossover to phase separation, Fulde–Ferrell–Larkin–Ovchinnikov states, polarized molecular superfluidity and the normal state, driven by the species imbalance. We discuss different models and approximations of this system and compare their predictions with current experiments.

arXiv:0911.1740•Reports on Progress in Physics•Jun 18, 2010•219 citations

Pairing of fermionic lithium-6 throughout the BEC-BCS crossover

Guthrie B. Partridge

The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.

•Jan 1, 2007•0 citations

Pair condensation of polarized fermions in the BCS–BEC crossover

G Bighin, G Mazzarella, L DellʼAnna +1 more

We investigate a two-component Fermi gas with unequal spin populations along the BCS-BEC crossover. By using the extended BCS equations and the concept of off-diagonal-long-range-order we derive a formula for the condensate number of Cooper pairs as a function of energy gap, average chemical potential, imbalance chemical potential and temperature. Then we study the zero-temperature condensate fraction of Cooper pairs by varying interaction strength and polarization, finding a depletion of the condensate fraction by increasing the population imbalance. We also consider explicitly the presence of an external harmonic confinement and we study, within the local-density approximation, the phase separation between superfluid and normal phase regions of the polarized fermionic cloud. In particular, we calculate both condensate density profiles and total density profiles from the inner superfluid core to the normal region passing for the interface, where a finite jump in the density is a clear manifestation of this phase-separated regime. Finally, we compare our theoretical results with the available experimental data on the condensate fraction of polarized 6Li atoms [Science 311, 492 (2006)]. These experimental data are in reasonable agreement with our predictions in a suitable range of polarizations, but only in the BCS side of the crossover up to unitarity.

arXiv:1404.3178•Journal of Physics B Atomic Molecular and Optical Physics•Sep 24, 2014•2 citations
We study resonantly-paired s-wave superfluidity in a degenerate gas of two species (hyperfine states labeled by ↑, ↓) of fermionic atoms when the numbers N↑ and N↓ of the two species are unequal, i.e., the system is "polarized." We find that the continuous crossover from the Bose-Einstein condensate (BEC) limit of tightly-bound diatomic molecules to the Bardeen-Cooper-Schrieffer (BCS) limit of weakly correlated Cooper pairs, studied extensively at equal populations, is interrupted by a variety of distinct phenomena under an imposed population difference ΔN ≡ N↑ - N↓. Our findings are summarized by a "polarization" (ΔN) versus Feshbach-resonance detuning (δ) zero-temperature phase diagram, which exhibits regions of phase separation, a periodic FFLO superfluid, a polarized normal Fermi gas and a polarized molecular superfluid consisting of a molecular condensate and a fully polarized Fermi gas. We describe numerous experimental signatures of such phases and the transitions between them, in particular focusing on their spatial structure in the inhomogeneous environment of an atomic trap. © 2006 Elsevier Inc. All rights reserved.
We map out the detuning-magnetization phase diagram for a magnetized (unequal number of atoms in two pairing hyperfine states) gas of fermionic atoms interacting via an s-wave Feshbach resonance (FR). The phase diagram is dominated by the coexistence of a magnetized normal gas and a singlet-paired superfluid with the latter exhibiting a BCS-Bose Einstein condensate crossover with reduced FR detuning. On the BCS side of strongly overlapping Cooper pairs, a sliver of finite-momentum paired Fulde-Ferrell-Larkin-Ovchinnikov magnetized phase intervenes between the phase-separated and normal states. In contrast, for large negative detuning a uniform, polarized superfluid, that is, a coherent mixture of singlet Bose-Einstein-condensed molecules and fully magnetized single-species Fermi sea, is a stable ground state.
We discuss the superfluid phase transition in a gas of Fermi atoms with a Feshbach resonance. A tunable pairing interaction associated with the Feshbach resonance is shown to naturally lead to the BCS-BEC crossover, where the character of superfluidity continuously changes from the weak-coupling Bardeen-Cooper-Schrieffer (BCS) type to the Bose-Einstein condensation (BEC) of tightly bound molecules, as one decreases the threshold energy 2ν of the Feshbach resonance. We also discuss effects of a trap, as well as the p-wave BCS-BEC crossover adjusted by a p-wave Feshbach resonance.
This thesis focuses on the analysis of Bardeen-Cooper-Schrieffer (BCS) \nto Bose-Einstein condensation (BEC) evolution in ultracold superfluid \nFermi gases when the interaction between atoms is varied. The tuning of \nattractive interactions permits the ground state of the system to evolve from a weak \nfermion attraction BCS limit of loosely bound and largely overlapping Cooper pairs \nto a strong fermion attraction limit of tightly bound small bosonic molecules \nwhich undergo BEC. \nThis evolution is accompanied by anomalous behavior of many superfluid \nproperties, and reveals several quantum phase transitions. \nThis thesis has two parts: \nIn the first part, I analyze zero and nonzero orbital angular momentum \npairing effects, and show that a quantum phase transition occurs for \nnonzero angular momentum pairing, unlike the sss-wave case where the BCS \nto BEC evolution is just a crossover. \nIn the second part, I analyze two-species fermion mixtures with mass and \npopulation imbalance in continuum, trap and lattice models. In contrast with \nthe crossover physics found in the mass and population balanced mixtures, \nI demonstrate the existence of phase transitions between normal and \nsuperfluid phases, as well as phase separation between superfluid (paired) \nand normal (excess) fermions in imbalanced mixtures as a function of scattering \nparameter and mass and population imbalance.
We present an overview of recent developments in species-imbalanced (‘polarized’) Feshbach-resonant Fermi gases. We summarize the current status of thermodynamics of these systems in terms of a phase diagram as a function of the Feshbach resonance detuning, polarization and temperature. We review instabilities of the s -wave superfluidity across the Bose–Einstein condensation-to-Bardeen–Cooper–Schrieffer crossover to phase separation, Fulde–Ferrell–Larkin–Ovchinnikov states, polarized molecular superfluidity and the normal state, driven by the species imbalance. We discuss different models and approximations of this system and compare their predictions with current experiments.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.
We investigate a two-component Fermi gas with unequal spin populations along the BCS-BEC crossover. By using the extended BCS equations and the concept of off-diagonal-long-range-order we derive a formula for the condensate number of Cooper pairs as a function of energy gap, average chemical potential, imbalance chemical potential and temperature. Then we study the zero-temperature condensate fraction of Cooper pairs by varying interaction strength and polarization, finding a depletion of the condensate fraction by increasing the population imbalance. We also consider explicitly the presence of an external harmonic confinement and we study, within the local-density approximation, the phase separation between superfluid and normal phase regions of the polarized fermionic cloud. In particular, we calculate both condensate density profiles and total density profiles from the inner superfluid core to the normal region passing for the interface, where a finite jump in the density is a clear manifestation of this phase-separated regime. Finally, we compare our theoretical results with the available experimental data on the condensate fraction of polarized 6Li atoms [Science 311, 492 (2006)]. These experimental data are in reasonable agreement with our predictions in a suitable range of polarizations, but only in the BCS side of the crossover up to unitarity.