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arXiv:cond-mat/0508430 · Physical Review Letters

BEC-BCS Crossover in “Magnetized” Feshbach-Resonantly Paired Superfluids

Daniel E. Sheehy, Leo Radzihovsky

Published Feb 13, 2006• 330 citations
arXivHTMLPDF

Abstract

We map out the detuning-magnetization phase diagram for a magnetized (unequal number of atoms in two pairing hyperfine states) gas of fermionic atoms interacting via an s-wave Feshbach resonance (FR). The phase diagram is dominated by the coexistence of a magnetized normal gas and a singlet-paired superfluid with the latter exhibiting a BCS-Bose Einstein condensate crossover with reduced FR detuning. On the BCS side of strongly overlapping Cooper pairs, a sliver of finite-momentum paired Fulde-Ferrell-Larkin-Ovchinnikov magnetized phase intervenes between the phase-separated and normal states. In contrast, for large negative detuning a uniform, polarized superfluid, that is, a coherent mixture of singlet Bose-Einstein-condensed molecules and fully magnetized single-species Fermi sea, is a stable ground state.

DOI
10.1103/physrevlett.96.060401

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We map out the detuning-magnetization phase diagram for a magnetized (unequal number of atoms in two pairing hyperfine states) gas of fermionic atoms interacting via an s-wave Feshbach resonance (FR). The phase diagram is dominated by the coexistence of a magnetized normal gas and a singlet-paired superfluid with the latter exhibiting a BCS-Bose Einstein condensate crossover with reduced FR detuning. On the BCS side of strongly overlapping Cooper pairs, a sliver of finite-momentum paired Fulde-Ferrell-Larkin-Ovchinnikov magnetized phase intervenes between the phase-separated and normal states. In contrast, for large negative detuning a uniform, polarized superfluid, that is, a coherent mixture of singlet Bose-Einstein-condensed molecules and fully magnetized single-species Fermi sea, is a stable ground state.
We study resonantly-paired s-wave superfluidity in a degenerate gas of two species (hyperfine states labeled by ↑, ↓) of fermionic atoms when the numbers N↑ and N↓ of the two species are unequal, i.e., the system is "polarized." We find that the continuous crossover from the Bose-Einstein condensate (BEC) limit of tightly-bound diatomic molecules to the Bardeen-Cooper-Schrieffer (BCS) limit of weakly correlated Cooper pairs, studied extensively at equal populations, is interrupted by a variety of distinct phenomena under an imposed population difference ΔN ≡ N↑ - N↓. Our findings are summarized by a "polarization" (ΔN) versus Feshbach-resonance detuning (δ) zero-temperature phase diagram, which exhibits regions of phase separation, a periodic FFLO superfluid, a polarized normal Fermi gas and a polarized molecular superfluid consisting of a molecular condensate and a fully polarized Fermi gas. We describe numerous experimental signatures of such phases and the transitions between them, in particular focusing on their spatial structure in the inhomogeneous environment of an atomic trap. © 2006 Elsevier Inc. All rights reserved.
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We discuss the superfluid phase transition of a strongly interacting Fermi gas with unequal (asymmetric) chemical potentials in two pairing hyperfine states, and map out its phase diagram near the BCS-BEC crossover. Our approach includes the fluctuation contributions of "preformed Cooper pairs" to the thermodynamic potential at finite temperature. We show that, below a critical difference in chemical potentials between species, a normal gas is unstable towards the formation of either a finite-momentum paired Fulde-Ferrell-Larkin-Ovchinnikov superconducting phase or a uniform superfluid, depending on the asymmetry and interaction strengths. We determine the value of critical chemical potential mismatch, and find that it is consistent with a recent measurement by Zwierlein et al. ( Science , 311 (2006) 492).
We study the phase diagram of the dilute two-component Fermi gas at zero temperature as a function of the polarization and coupling strength. We map out the detailed phase separations between superfluid and normal states near the Feshbach resonance. We show that there are three different coexistence of superfluid and normal phases corresponding to phase separated states between: (I) the partially polarized superfluid and the fully polarized normal phases, (II) the unpolarized superfluid and the fully polarized normal phases and (III) the unpolarized superfluid and the partially polarized normal phases from strong-coupling BEC side to weak-coupling BCS side. For pairing between two species, we found this phase separation regime gets wider and moves toward the BEC side for the majority species are heavier but shifts to BCS side and becomes narrow if they are lighter.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.
We address the phase of a highly polarized Fermi gases across a narrow Feshbach resonance starting from the problem of a single down-spin fermion immersed in a Fermi sea of up spins. Both polaron and pairing states are considered using the variational wave function approach, and we find that the polaron-to-pairing transition will take place on the BCS side of the resonance, strongly in contrast to a wide resonance where the transition is located at the BEC side. For the pairing phase, we find the critical strength of the repulsive interaction between pairs above which the mixture of pairs and fermions will not phase separate. Therefore, nearby a narrow resonance, it is quite likely that magnetism can coexist with sss-wave BCS superfluidity at large Zeeman fields, which is a remarkable property absent in conventional BCS superconductors (or fermion-pair superfluids).