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arXiv:cond-mat/0606275 · Physical Review B

Cavity-assisted generation of entangled photon pairs by a quantum-dot cascade decay

Filippo Troiani, J. I. Perea, C. Tejedor

Published Dec 7, 2006• 69 citations
arXivHTMLPDF

Abstract

We compute the concurrence of the polarization-entangled photon pairs generated by the biexciton cascade decay of a semiconductor quantum dot. We show how a cavity-induced increase of the photon emission rate reduces the effect of dot dephasing and excitonic fine structure on the concurrence. However, strong dot-cavity couplings, as well as low detection efficiencies, increase the detrimental effect of multiple cascades. This affects the merits of the entangled photon-pair source, beyond what is estimated by quantum tomography.

DOI
10.1103/physrevb.74.235310

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We compute the concurrence of the polarization-entangled photon pairs generated by the biexciton cascade decay of a semiconductor quantum dot. We show how a cavity-induced increase of the photon emission rate reduces the effect of dot dephasing and excitonic fine structure on the concurrence. However, strong dot-cavity couplings, as well as low detection efficiencies, increase the detrimental effect of multiple cascades. This affects the merits of the entangled photon-pair source, beyond what is estimated by quantum tomography.
Semiconductor quantum dots are promising sources for polarization-entangled photons. As an alternative to the usual cascaded biexciton-exciton emission, direct two-photon emission from the biexciton can be used. With a high-quality optical resonator tuned to half the biexciton energy, a large proportion of the photons can be steered into the two-photon emission channel. In this case the degree of polarization entanglement is inherently insensitive to the exciton fine-structure splitting. In the present work we analyze the biexciton emission with particular emphasis on the influence of coupling of the quantum-dot cavity system to its environment. Especially for a high-quality cavity, the coupling to the surrounding semiconductor material can open up additional phonon-assisted decay channels. Our analysis demonstrates that with the cavity tuned to half the biexciton energy, the potentially detrimental influence of the phonons on the polarization entanglement is strongly suppressed---high degrees of entanglement can still be achieved. We further discuss spectral properties and statistics of the emitted twin photons.
Semiconductor quantum dots are among the best sources of on-demand entangled photon pairs. The degree of entanglement, however, is generally limited by the fine structure splitting of exciton states. In this paper, we theoretically investigate the generation of polarization-entangled photon pairs under two-photon excitation and cavity-assisted two-photon emission, both in the weak and strong cavity coupling regimes. We demonstrate and clarify that cavity coupling together with an excitation pulse reduces the degree of entanglement in three different ways. First, in a strong coupling regime, the cavity introduces the unequal ac-Stark shift of horizontally and vertically polarized exciton states, which results in the effective splitting of exciton states. Second, it induces the cross-coupling between the exciton states even in the weak coupling regime, causing the creation of unfavorable two-photon states. Finally, higher excited states of the cavity modes also contribute to the reduction of entanglement. Therefore, in the setting considered here, cavity coupling, which is generally required for the efficient collection of emitted photons, degrades the entanglement both in weak and strong coupling regimes.
We study the quantum properties and statistics of photons emitted by a quantum-dot biexciton inside a cavity. In the biexciton-exciton cascade, fine-structure splitting between exciton levels degrades polarization-entanglement for the emitted pair of photons. However, here we show that the polarization-entanglement can be preserved in such a system through simultaneous emission of two degenerate photons into cavity modes tuned to half the biexciton energy. Based on detailed theoretical calculations for realistic quantum-dot and cavity parameters, we quantify the degree of achievable entanglement.
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A fundamental approach to generate polarization-entangled photon pairs from solid-state devices is the biexciton cascade in semiconductor quantum dots. For efficient photon pair generation in the weak coupling regime, we present an analytical solution for the two-photon matrix elements (quantum-state tomography), including dephasing and relaxation mechanisms. In particular, we show that a pure dephasing mechanism does not affect the degree of entanglement for quantum dots with degenerated exciton levels.
We present a scheme for the fast cavity-assisted generation of entangled photon pairs from a single quantum dot coupled to a planar photonic crystal that support two orthogonally polarized cavity modes. We discuss ``within generation'' and ``across generation'' of entangled photons when both the biexciton to exciton, and the exciton to ground-state transitions, are coupled through cavity modes. In the across generation, the photon entanglement is restored through a time delay between the photons. The concurrence, which is a measure of the entanglement between two photons, is greater than 0.7 and 0.8 using experimentally achievable parameters in across generation and within generation, respectively. We also show that the entanglement can be distilled in both cases using a simple spectral filter.