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arXiv:cond-mat/0603342 · Physical Review B

Critical charge instability on the verge of the Mott transition and the origin of quantum protection in high- Tc cuprates

T. K. Kopeć

Published Mar 10, 2006• 12 citations
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Abstract

The concept of topological excitations and the related ground state degeneracy are employed to establish an effective theory of the superconducting state evolving from the Mott insulator for high-${T}_{c}$ cuprates. The theory includes the effects of the relevant energy scales with the emphasis on the Coulomb interaction $U$ governed by the electromagnetic U(1) compact group. The results are obtained for the layered $t\ensuremath{-}{t}^{\ensuremath{'}}\ensuremath{-}{t}_{\ensuremath{\perp}}\ensuremath{-}U\ensuremath{-}J$ system of strongly correlated electrons relevant for cuprates. Casting the Coulomb interaction in terms of composite-fermions via the gauge flux attachment facility, we show that instanton events in the Matsubara ``imaginary time,'' labeled by topological winding numbers, are essential configurations of the phase field dual to the charge. This provides a nonperturbative concept of the topological quantization and displays the significance of discrete topological sectors in the theory governed by the global characteristics of the phase field. We show that for topologically ordered states these quantum numbers play the role of an order parameter in a way similar to the Landau order parameter for conventionally ordered states. In analogy to the usual phase transition that is characterized by a sudden change of the symmetry, the topological phase transitions are governed by a discontinuous change of the topological numbers signaled by the divergence of the zero-temperature topological susceptibility. This defines a quantum criticality ruled by topologically conserved numbers rather than the Landau principle of the symmetry breaking. We show that in the limit of strong correlations topological charge is linked to the average electronic filling number and the topological susceptibility to the electronic compressibility of the system. We exploit the impact of these nontrivial U(1) instanton phase field configurations for the cuprate phase diagram which displays the ``hidden'' quantum critical point covered by the superconducting lobe in addition to a sharp crossover between a compressible normal ``strange metal'' state and a region characterized by a vanishing compressibility, which marks the Mott insulator. Finally, we argue that the existence of robust quantum numbers explains the stability against small perturbation of the system and attributes to the topological ``quantum protectorate'' as observed in strongly correlated systems.

DOI
10.1103/physrevb.73.104505

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The concept of topological excitations and the related ground state degeneracy are employed to establish an effective theory of the superconducting state evolving from the Mott insulator for high-Tc{T}_{c}Tc​ cuprates. The theory includes the effects of the relevant energy scales with the emphasis on the Coulomb interaction UUU governed by the electromagnetic U(1) compact group. The results are obtained for the layered t\ensuremath−t\ensuremath′\ensuremath−t\ensuremath⊥\ensuremath−U\ensuremath−Jt\ensuremath{-}{t}^{\ensuremath{'}}\ensuremath{-}{t}_{\ensuremath{\perp}}\ensuremath{-}U\ensuremath{-}Jt\ensuremath−t\ensuremath′\ensuremath−t\ensuremath⊥​\ensuremath−U\ensuremath−J system of strongly correlated electrons relevant for cuprates. Casting the Coulomb interaction in terms of composite-fermions via the gauge flux attachment facility, we show that instanton events in the Matsubara imaginary time,'' labeled by topological winding numbers, are essential configurations of the phase field dual to the charge. This provides a nonperturbative concept of the topological quantization and displays the significance of discrete topological sectors in the theory governed by the global characteristics of the phase field. We show that for topologically ordered states these quantum numbers play the role of an order parameter in a way similar to the Landau order parameter for conventionally ordered states. In analogy to the usual phase transition that is characterized by a sudden change of the symmetry, the topological phase transitions are governed by a discontinuous change of the topological numbers signaled by the divergence of the zero-temperature topological susceptibility. This defines a quantum criticality ruled by topologically conserved numbers rather than the Landau principle of the symmetry breaking. We show that in the limit of strong correlations topological charge is linked to the average electronic filling number and the topological susceptibility to the electronic compressibility of the system. We exploit the impact of these nontrivial U(1) instanton phase field configurations for the cuprate phase diagram which displays the hidden'' quantum critical point covered by the superconducting lobe in addition to a sharp crossover between a compressible normal strange metal'' state and a region characterized by a vanishing compressibility, which marks the Mott insulator. Finally, we argue that the existence of robust quantum numbers explains the stability against small perturbation of the system and attributes to the topological quantum protectorate'' as observed in strongly correlated systems.
For strongly correlated electrons the relation between total number of charge carriers ne{n}_{e}ne​ and the chemical potential $\ensuremath{\mu}$ reveals for large Coulomb energy the apparently paradoxical pinning of $\ensuremath{\mu}$ within the Mott gap, as observed in high-Tc{T}_{c}Tc​ cuprates. By unraveling consequences of the nontrivial topology of the charge gauge U(1) group and the associated ground state degeneracy we found a close kinship between the pinning of $\ensuremath{\mu}$ and the zero-temperature divergence of the charge compressibility $\ensuremath{\kappa}\ensuremath{\sim}\ensuremath{\partial}{n}_{e}∕\ensuremath{\partial}\ensuremath{\mu}$, which marks a novel quantum criticality governed by topological charges rather than Landau principle of the symmetry breaking.
The electronic $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}U\text{\ensuremath{-}}J$ model for the CuO2\mathrm{Cu}{\mathrm{O}}_{2}CuO2​ plane in high-Tc{T}_{c}Tc​ superconducting cuprates is elaborated. It incorporates both charge transfer UUU and exchange correlation JJJ with direct ttt and diagonal ${t}^{\ensuremath{'}}$ hopping. Making use of the Yang concept of the off diagonal long range order (ODLRO) in the reduced density matrix of the electronic system we study the loss of quantum wave coherence (and thereby superconductivity) due to the Coulomb interaction. To this aim the second-quantized Hamiltonian of the model is translated to the phase representation with the help of the topologically constrained path integral formalism. As a result the electrons emerge as composite particles consisting of of spin-carrying neutral fermions and charged topological bosons in a form of ``flux tubes'' with the quantum phase variable dual to the local electron density. The charge carrying bose field forms a collective variable representing the correlated ``sliding'' motion of the entire electronic system. We found that the spin gap $\ensuremath{\Delta}$ which appears in one-particle spectrum is the result of valence bond pairing of neutral fermions without ODLRO and deduce the solution for $\ensuremath{\Delta}$ with ``ddd-wave'' symmetry. In the bosonic sector we derive the effective quantum rotor model along with microscopic phase stiffnesses setting the energy scale for superconductivity and point out the special role played by the diagonal hopping ${t}^{\ensuremath{'}}$. We explore the relationship of the quantum rotor phase model and the Bose-Hubbard system emphasizing the ring topology of quantum phase variable. Furthermore, we obtain the ground state phase diagrams which facilitate the Mott insulator-superconductor transition scenario. We elucidate the role of the chemical potential (doping) and the huge degeneracy of the effective bosonic system in achieving ODLRO with long-range phase coherence in the presence of large Coulomb repulsion. Finally, we discuss a number of relevant issues pertaining to the the present work which include: theoretical aspects of the hierarchy of the energy scales in cuprates, ``spin-charge separation'' concepts, ``local-pair'' and ``phase-fluctuation'' scenarios as well as experimental findings related to the role of the ``ddd-wave'' symmetry of the spin gap and diagonal hopping ${t}^{\ensuremath{'}}$ in cuprates.
Topological Mott Insulators and Discontinuous U(1)U(1)U(1) θθθ-Terms
We introduce a lattice field theory that describes the transition between a superfluid (SF) and a bosonic topological Mott Insulator (tMI) -- a U(1)U(1)U(1) symmetry protected topological phase labeled by an integer level kkk and possessing an even integer 2ke2h2k\frac{e^2}{h}2khe2​ quantized Hall conductance. Our model differs from the usual 2+12+12+1d XY model by a topological term that vanishes on closed manifolds and in the absence of an applied gauge field, which implies that the critical exponents of the SF-tMI transition are identical to those of the well-studied 2+12+12+1d XY transition. Our formalism predicts a "level-shift" symmetry: in the absence of an applied gauge field, the bulk correlation functions of all local operators are identical for models differing by the topological term. %, for example, near the SF-MI and SF-tMI transitions, and hence the extremely well-studied critical exponents of the 2+12+12+1d XY model apply to the SF-tMI transition. In the presence of a background gauge field, the topological term leads to a quantized Hall response in the tMI phase, and we argue that this quantized Hall effect persists in the vicinity of the phase transition into the SF phase. Our formalism paves the way for other exact lattice descriptions of symmetry-protected-topological (SPT) phases, and mappings of critical exponents between transitions from symmetry-breaking to trivial states and transitions from symmetry-breaking to SPT states. A similar "level shift" symmetry should appear between all group cohomology SPT states protected by the same symmetry.
The history of modern condensed matter physics may be regarded as the competition and reconciliation between Stoner’s and Anderson’s physical pictures, where the former is based on momentum–space descriptions focusing on long wave-length fluctuations while the latter is based on real-space physics emphasizing emergent localized excitations. In particular, these two view points compete with each other in various nonperturbative phenomena, which range from the problem of high [Formula: see text] superconductivity, quantum spin liquids in organic materials and frustrated spin systems, heavy-fermion quantum criticality, metal-insulator transitions in correlated electron systems such as doped silicons and two-dimensional electron systems, the fractional quantum Hall effect, to the recently discussed Fe-based superconductors. An approach to reconcile these competing frameworks is to introduce topologically nontrivial excitations into the Stoner’s description, which appear to be localized in either space or time and sometimes both, where scattering between itinerant electrons and topological excitations such as skyrmions, vortices, various forms of instantons, emergent magnetic monopoles, and etc. may catch nonperturbative local physics beyond the Stoner’s paradigm. In this review paper, we discuss nonperturbative effects of topological excitations on dynamics of correlated electrons. First, we focus on the problem of scattering between itinerant fermions and topological excitations in antiferromagnetic doped Mott insulators, expected to be relevant for the pseudogap phase of high [Formula: see text] cuprates. We propose that nonperturbative effects of topological excitations can be incorporated within the perturbative framework, where an enhanced global symmetry with a topological term plays an essential role. In the second part, we go on to discuss the subject of symmetry protected topological states in a largely similar light. While we do not introduce itinerant fermions here, the nonperturbative dynamics of topological excitations is again seen to be crucial in classifying topologically nontrivial gapped systems. We point to some hidden links between several effective field theories with topological terms, starting with one-dimensional physics, and subsequently finding natural generalizations to higher dimensions.
In this thesis, we investigate several topics pertaining to emergent collective quantum phenomena in the domain of correlated fermions, using the quantum Monte Carlo method. They display exotic low temperature phases as well as phase transitions which are beyond the Landau–Ginzburg theory. The interplay between three key points is crucial for us: fermion statistics, many body effects and topology. We highlight the following several achievements: 1. Successful modeling of continuum field theories with lattice Hamiltonians, 2. their sign-problem-free Monte Carlo simulations of these models, 3. and numerical results beyond mean field descriptions. First, we consider a model of Dirac fermions with a spin rotational invariant inter- action term that dynamically generates a quantum spin Hall insulator. Surprisingly, an s-wave superconducting phase emerges due to the condensation of topological de- fects of the spin Hall order parameter. When particle-hole symmetry is present, the phase transition between the topological insulator and the superconducting phase is an example of a deconfined quantum critical point(DQCP). Although its low energy effec- tive field theory is purely bosonic, the exact conservation law of the skyrmion number operator rules out the possibility of realizing this critical point in lattice boson models. This work is published in Ref. [1]. Second, we dope the dynamically generated quantum spin Hall insulator mentioned above. Hence it is described by a field theory without Lorentz invariance due to the lack of particle-hole symmetry. This sheds light on the extremely hot topic of twisted bilayergraphene: Why is superconductivity generated when the repulsive Coulomb interaction is much stronger than the electron-phonon coupling energy scale? In our case, Cooper pairs come from the topological skyrmion defects of the spin current order parameter, which are charged. Remarkably, the nature of the phase transition is highly non-mean-field-like: one is not allowed to simply view pairs of electrons as single bosons in a superfluid-Mott insulator transition, since the spin-current order parameter can not be ignored. Again, due to the aforementioned skyrmions, the two order parameters are intertwined: One phase transition occurs between the two symmetry breaking states. This work is summarized in Ref. [2]. Third, we investigate the 2 + 1 dimensional O(5) nonlinear sigma model with a topological Wess-Zumino-Witten term. Remarkably, we are able to perform Monte Carlo calculations with a UV cutoff given by the Dirac Landau level quantization. It is a successful example of simulating a continuous field theory without lattice regularization which leads to an additional symmetry breaking. The Dirac background and the five anti-commuting Dirac mass terms naturally introduce the picture of a non-trivial Berry phase contribution in the parameter space of the five component order parameter. Using the finite size scaling method given by the flux quantization, we find a stable critical phase in the low stiffness region of the sigma model. This is a candidate ground state of DQCP when the O(5) symmetry breaking terms are irrelevant at the critical point. Again, it has a bosonic low energy field theory which is seemingly unable to be realized in pure boson Hamiltonians. This work is summarized in Ref. [3].
Superfluids and superconductors can be either fully gapped or gapless with nodal structures in momentum space. Both the gapped and nodal phases can be topologically protected and possess nontrivial topological invariants. Topological quantum phase transitions exist at zero temperature between different gapped phases or between gapped and nodal phases. These phase transitions can be driven by chemical potential and/or spin exchange fields. The two phases separated by the phase transition can have the same local order but differ in global topology. Thus, these topological quantum phase transitions cannot be described by the Landau paradigm of symmetry breaking. Although some aspects of these transitions, such as the change of topological invariants and gapless boundary states, have been discussed before, a complete theory of these transitions has yet to be developed. In this dissertation, we construct effective field theories to study the universality and thermodynamic signatures of these transitions. We find four different universality classes in superfluids and superconductors. Certain thermodynamic quantities, such as compressibility or spin susceptibility, change non-analytically across the transitions. For certain time-reversal symmetry breaking fields that lead to bulk phase transitions, there also exist topological phase transitions on the surface. All the topological phase transitions studied in this dissertation only exist at zero temperature. At finite temperature, different states are connected by smooth crossovers. There exists a quantum critical region at finite temperature near the quantum critical point (QCP). In this quantum critical region, thermodynamic quantities have universal scaling dependence on temperature dictated by the universality class of the QCP. We argue that these scaling properties can be used to probe and differentiate these QCPs. These bulk and surface topological quantum phase transitions are discussed in various concrete models, such as chiral and time-reversal invariant p-wave superfluids, topological superconductors of emergent Dirac fermions, and topological superconducting model of CuₓBi₂Se₃.