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arXiv:cond-mat/0509617 · Physical Review B

Infrared catastrophe and tunneling into strongly correlated electron systems: Beyond the x-ray edge limit

Kelly R. Patton, Michael R. Geller

Published Mar 20, 2006• 3 citations
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Abstract

We develop a nonperturbative method to calculate the electron propagator in low-dimensional and strongly correlated electron systems. The method builds on our earlier work using a Hubbard-Stratonovich transformation to map the tunneling problem to the x-ray edge problem, which accounts for the infrared catastrophe caused by the sudden introduction of a new electron into a conductor during a tunneling event. Here we use a cumulant expansion to include fluctuations about this x-ray edge limit. We find that the dominant effect of electron-electron interaction at low energies is to correct the noninteracting Green's function by a factor ${e}^{\ensuremath{-}S∕\ensuremath{\hbar}}$, where $S$ can be interpreted as the Euclidean action for a density field describing the time-dependent charge distribution of the newly added electron. Initially localized, this charge distribution spreads in time as the electron is accommodated by the host conductor, and during this relaxation process action is accumulated according to classical electrostatics with a screened interaction. The theory applies to lattice or continuum models of any dimensionality, with or without translational invariance. In one dimension the method correctly predicts a power-law density of states for electrons with short-range interaction and no disorder, and when applied to the solvable Tomonaga-Luttinger model, the exact density of states is obtained.

DOI
10.1103/physrevb.73.125416

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We develop a nonperturbative method to calculate the electron propagator in low-dimensional and strongly correlated electron systems. The method builds on our earlier work using a Hubbard-Stratonovich transformation to map the tunneling problem to the x-ray edge problem, which accounts for the infrared catastrophe caused by the sudden introduction of a new electron into a conductor during a tunneling event. Here we use a cumulant expansion to include fluctuations about this x-ray edge limit. We find that the dominant effect of electron-electron interaction at low energies is to correct the noninteracting Green's function by a factor e\ensuremath−S∕\ensuremathℏ{e}^{\ensuremath{-}S∕\ensuremath{\hbar}}e\ensuremath−S∕\ensuremathℏ, where SSS can be interpreted as the Euclidean action for a density field describing the time-dependent charge distribution of the newly added electron. Initially localized, this charge distribution spreads in time as the electron is accommodated by the host conductor, and during this relaxation process action is accumulated according to classical electrostatics with a screened interaction. The theory applies to lattice or continuum models of any dimensionality, with or without translational invariance. In one dimension the method correctly predicts a power-law density of states for electrons with short-range interaction and no disorder, and when applied to the solvable Tomonaga-Luttinger model, the exact density of states is obtained.
The tunneling density of states exhibits anomalies (cusps, algebraic suppressions, and pseudogaps) at the Fermi energy in a wide variety of low-dimensional and strongly correlated electron systems. We argue that in many cases these spectral anomalies are caused by an infrared catastrophe in the screening response to the sudden introduction of a new electron into the system during a tunneling event. A nonperturbative functional integral method is introduced to account for this effect, making use of methods developed for the x-ray edge singularity problem. The formalism is applicable to lattice or continuum models of any dimensionality, with or without translational invariance. An approximate version of the technique is applied to the 1D electron gas and the 2D Hall fluid, yielding qualitatively correct results.
A general nonperturbative theory of the low-energy electron propagator is developed and used to calculate the single-particle density of states in a variety of systems. This method involves the decoupling of the electron-electron interaction through a Hubbard-Stratonovich transformation, followed by a saddle-point approximation of the remaining functional integral. The final expression is found to be the tunneling analog of the infrared catastrophe that occurs in the x-ray edge problem; here, the host system responds to the potential produced by the abrupt addition of an electron during a tunneling event. This response can lead to a suppression in the tunneling density of states near the Fermi energy. This method is adaptable to lattice or continuum models of any dimensionality, with or without translational invariance. When applied, the exact density of states is obtained for the Tomonaga-Luttinger model, and the pseudogap of a fractional quantum Hall fluid is recovered.
In previous work [K. R. Patton and M. R. Geller, Phys. Rev. B 72, 125108 (2005)] we have proposed that the non-Fermi-liquid spectral properties in a variety of low-dimensional and strongly correlated electron systems are caused by the infrared catastrophe, and we used an exact functional integral representation for the interacting Green's function to map the tunneling problem onto the x-ray edge problem, plus corrections. The corrections are caused by the recoil of the tunneling particle, and, in systems where the method is applicable, are not expected to change the qualitative form of the tunneling density of states (DOS). Qualitatively correct results were obtained for the DOS of the one-dimensional electron gas and two-dimensional Hall fluid when the corrections to the x-ray edge limit were neglected and when the corresponding Nozi\`eres-De Dominicis integral equations were solved by resummation of a divergent perturbation series. Here we reexamine the x-ray edge limit for these two models by solving these integral equations exactly, finding the expected modifications of the DOS exponent in the one-dimensional case but finding no changes in the DOS of the two-dimensional Hall fluid with short-range interaction. Our analysis provides an exact solution of the Nozi\`eres-De Dominicis equation for the two-dimensional electron gas in the lowest Landau level.
The theoretical model of the short-range interacting Luttinger liquid predicts a power-law scaling of the density of states and the momentum distribution function around the Fermi surface, which can be readily tested through tunneling experiments. However, some physical systems have long-range interaction, most notably the Coulomb interaction, leading to significantly different behaviors from the short-range interacting system. In this paper, we revisit the tunneling theory for the one-dimensional electrons interacting via the long-range Coulomb force. We show that even though in a small dynamic range of temperature and bias voltage, the tunneling conductance may appear to have a power-law decay similar to short-range interacting systems, the effective exponent is scale-dependent and slowly increases with decreasing energy. This factor may lead to the sample-to-sample variation in the measured tunneling exponents. We also discuss the crossover to a free Fermi gas at high energy and the effect of the finite size. Our work demonstrates that experimental tunneling measurements in one-dimensional electron systems should be interpreted with great caution when the system is a Coulomb Luttinger liquid.
Recent advances of experimental nanofabrication techniques draw increasing attention to the non-equilibrium behavior of low dimensional systems. Of particular interest are the strongly interacting one dimensional systems whose description in out of equilibrium situations remains a theoretical challenge. This thesis contributes to the understanding of important elementary processes in the non-equilibrium physics of one dimensional electron systems. Tunneling of an electron into a Luttinger liquid leads to partitioning of its charge and energy into counter-propagating modes. This thesis studies the partitioning of the energy which had previously remained unexplored. It turns out that energy partitioning is essentially independent of the charge partitioning and one can even reach conditions such that energy and charge propagate in opposite directions. Another important difference is their experimental accessibility. In contrast to the charge, energy partitioning provides a measurable characteristic of the tunneling process even in dc setups and we propose experimental geometries that allow for tuning and detecting energy partitioning. At higher excitation energies it becomes necessary to include curvature effects of the electron dispersion. Another part of this thesis discusses the consequences of curvature induced three-body collisions on the relaxation in quantum wires. This is particularly interesting due to the integrability of the Luttinger model which does not allow for thermalization within this paradigm of one dimensional systems. In this thesis we derive energy relaxation rates due to three-body processes beyond the Luttinger model within a well-defined perturbative approach. It turns out that the electron spin and the long range Coulomb interaction are important ingredients for a quantitative description of recent experiments which we provide in this thesis. Furthermore, we study the influence of three-body collisions on the energy relaxation in integer quantum Hall edge states. We specifically address different interaction induced edge reconstruction scenarios and find that edge reconstruction strongly enhances the energy relaxation. This is particularly pronounced when the reconstruction creates additional counter-propagating modes. Finally, we discuss another system which is crucially controlled by non-equilibrium effects. The so called nanoelectromechanical systems show a coupling between the electronic and mechanical degrees of freedom. The electron current can thus influence the mechanical motion which leads to a number of interesting applications. Previous theoretical studies on the basis of non-equilibrium Green's functions showed that these current induced forces can be expressed in terms of intuitive scattering matrix expressions. This thesis sheds considerable light on this observation by providing a much more satisfactory and concise derivation of the scattering theory of current induced forces.
This dissertation examines the impact of long-range interactions in lattice models of low-dimensional strongly correlated systems with a focus on their relevance to anomalous electronic transport. Traditionally, the Hubbard model forms the basis of theoretical and numerical investigations of strongly correlated quantum matter. This effective model constitutes the simplest model of electronic correlation and relies on an approximation that truncates electron-electron interactions to a local, on-site potential. While this approximation has proved valid in several instances, certain unexplained phenomena in correlated materials challenge us to develop new perspectives and approaches.In the first part of this thesis, we discuss the historical motivation for our current work from both a theoretical and an experimental viewpoint. In particular, we cover the discovery of bad metallic transport and the associated breakdown of Boltzmann theory of electron transport. We further review examples of strongly correlated systems that exhibit bad metallic transport and other exotic phenomena that suggest the possibility of poorly screened electronic interactions acting as a common microscopic mechanism. This general feature justifies the development of a theoretical framework that is capable of examining long-range interactions in a controlled, systematic manner.Motivated by this, we analyze a long-range interacting lattice model for spinless electrons in two dimensions via exact diagonalization on a finite cluster in real space. As this method is susceptible to finite-size errors, we discuss at length its implementation and technical details designed specifically to reduce these errors, namely the use of twisted boundary conditions and the Ewald summation. We determine the phase diagram at zero temperature and demonstrate that the long-range interactions act as a source of self-generated disorder that drives the development of a strongly correlated pseudogap phase, in a manner reminiscent of the classical Efros-Shklovskii Coulomb gap. Furthermore, we establish that this phenomenon is independent of lattice geometry, a fact that represents the broad potential of long-range interactions in giving rise to a novel form of strongly correlated behavior.Following our zero-temperature study, we address the question of whether this self-generated disorder can survive in the presence of thermal fluctuations and local Coulomb repulsion (Hubbard terms) relevant in Mott systems, a situation closer to those in experimental systems. By means of classical Monte Carlo calculations, we show that not only does the self-generated disorder survive, but that it also acts as a microscopic mechanism that generates bad metallic transport. Upon further investigation, we determine that the long-range interactions, in combination with quantum fluctuations, cause a transient localization of the charge carriers, thereby suppressing the conductivity values below those predicted in conventional Boltzmann theory, as observed experimentally.In conclusion, we have established that long-range interactions in electronic models act as a microscopic mechanism that is capable of causing exotic phenomena in numerous materials. We conclude that a proper treatment of both quantum fluctuations and long-range interactions should next be studied with the finite temperature Lanczos method, which will act as a bridge between our exact diagonalization and Monte Carlo studies. Overall, this dissertation emphasizes the capability of long-range interactions to produce novel phenomena and elicits further thought-provoking questions concerning the interplay with Mott-Hubbard physics and external disorder, crucial in metallic systems.