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arXiv:cond-mat/0507619

One-magnon states and electron spin resonance in spin-ladders with singlet-rung ground statein a staggered magnetic field

P. N. Bibikov

Published Jul 26, 2005• 0 citations
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Abstract

One-magnon problem for spin-ladders with exact singlet-rung ground state in arbitrary oriented constant and staggered magnetic fields is studied. For two special configurations when the both fields are parallel or perpendicular to each other the exact formulas for eigenstates and eigenvectors are presented. In the parallel case the one-magnon contribution to the ESR absorption line shape is obtained. The latter is non-Lorentzian, has finite range and a gap around resonance. For low fields both the range of the spectrum and the width of the gap are controlled by the width of the one-magnon zone in zero magnetic field. Some other interactions usually contributing to the ESR line shape are also briefly discussed.

DOI
10.48550/arxiv.cond-mat/0507619

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One-magnon problem for spin-ladders with exact singlet-rung ground state in arbitrary oriented constant and staggered magnetic fields is studied. For two special configurations when the both fields are parallel or perpendicular to each other the exact formulas for eigenstates and eigenvectors are presented. In the parallel case the one-magnon contribution to the ESR absorption line shape is obtained. The latter is non-Lorentzian, has finite range and a gap around resonance. For low fields both the range of the spectrum and the width of the gap are controlled by the width of the one-magnon zone in zero magnetic field. Some other interactions usually contributing to the ESR line shape are also briefly discussed.
Recently several compounds were observed to reveal properties of a one-dimensional spin-12\frac{1}{2}21​ antiferromagnetic Heisenberg chain with gapless low-lying spin excitations in an absence of an external magnetic field. However even a very weak external magnetic field yields an onset of a spin gap for those low-lying excitations. Usually this onset of a field-induced spin gap is related to the presence of a staggered Dzyaloshinskii-Moriya interaction, or to the staggered effective g factors of magnetic ions. Experiments on thermodynamic properties cannot distinguish between those two origins for the spin-gap formation. Here we propose the setup for an experiment, in which one can clearly distinguish between the staggered Dzyaloshinskii-Moriya coupling and staggered external magnetic field: an electronic paramagnetic resonance in the parallel pumping geometry. The characteristics of the system under conditions of such an experiment, i.e., the renormalization of the homogeneous and staggered magnetizations, power of the microwave magnetic field, absorbed by the system, are calculated. Several important features of the solution are discussed.
Abstract A spin-1/2 Heisenberg antiferromagnetic chain is one of the most important paradigmatic models in quantum magnetism. Its ground state is a spin singlet, while the excitation spectrum is formed by gapless fractional excitations, spinons. The presence of alternating g-tensors and/or the staggered Dzyaloshinskii-Moriya interaction results in opening the energy gap Δ∝H2/3\varDelta \propto H^{2/3}Δ∝H2/3 Δ ∝ H 2 / 3 , once the magnetic field H is applied. A fairly good understanding of this phenomenon was achieved in the framework of the sine-Gordon quantum-field theory, taking into account the effective transverse staggered field induced by the applied uniform field. The theory predicts solitons and antisolitons as elementary excitations, as well as their bound states, breathers. Here, I review recent high-field electron spin resonance spectroscopy studies of such systems, focusing on peculiarities of their spin dynamics in the sine-Gordon regime and beyond.
We have studied the ground state phase diagram of a spin ladder with alternating rung exchange J⊥n=J⊥[1+(−1)nδ]J^{n}_{\perp} = J_{\perp}[1 + (-1)^{n} δ]J⊥n​=J⊥​[1+(−1)nδ] in a magnetic filed, in the limit where the rung coupling is dominant. In this limit the model is mapped onto an XXZXXZXXZ Heisenberg chain in a uniform and staggered longitudinal magnetic fields, where the amplitude of the staggered field is ∼δ\sim δ∼δ. We have shown that the magnetization curve of the system exhibits a plateau at magnetization equal to the half of the saturation value. The width of a plateau scales as δνδ^νδν, where ν=4/5ν=4/5ν=4/5 in the case of ladder with isotropic antiferromagnetic legs and ν=2ν=2ν=2 in the case of ladder with isotropic ferromagnetic legs. We have calculated four critical fields (Hc1±H^{\pm}_{c1}Hc1±​ and Hc2±H^{\pm}_{c2}Hc2±​) corresponding to transitions between different magnetic phases of the system. We have shown that these transitions belong to the universality class of the commensurate-incommensurate transition.
We construct a class of spin-1/2 antiferromagnetic two-chain ladder models consisting of blocks of n-spin tetrahedral clusters alternating with two-spin rungs. For n=4n=4n=4 and 6 and in extended parameter regimes, the exact ground state of the ladder is shown to be a product of the ground states of the rungs and the n-spin blocks, in both zero and finite magnetic fields. In the latter case, magnetization/site m versus magenetic field h plot exhibits well-defined magnetization plateaus.
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