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Physical review. B, Condensed matter

Electron paramagnetic resonance with parallel pumping in quantum spin chains with field-induced spin gap

Andrei A. Zvyagin, G. A. Zvyagina

Published Jul 19, 2002• 1 citation
Publisher

Abstract

Recently several compounds were observed to reveal properties of a one-dimensional spin-$\frac{1}{2}$ antiferromagnetic Heisenberg chain with gapless low-lying spin excitations in an absence of an external magnetic field. However even a very weak external magnetic field yields an onset of a spin gap for those low-lying excitations. Usually this onset of a field-induced spin gap is related to the presence of a staggered Dzyaloshinskii-Moriya interaction, or to the staggered effective g factors of magnetic ions. Experiments on thermodynamic properties cannot distinguish between those two origins for the spin-gap formation. Here we propose the setup for an experiment, in which one can clearly distinguish between the staggered Dzyaloshinskii-Moriya coupling and staggered external magnetic field: an electronic paramagnetic resonance in the parallel pumping geometry. The characteristics of the system under conditions of such an experiment, i.e., the renormalization of the homogeneous and staggered magnetizations, power of the microwave magnetic field, absorbed by the system, are calculated. Several important features of the solution are discussed.

DOI
10.1103/physrevb.66.014442

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Recently several compounds were observed to reveal properties of a one-dimensional spin-12\frac{1}{2}21​ antiferromagnetic Heisenberg chain with gapless low-lying spin excitations in an absence of an external magnetic field. However even a very weak external magnetic field yields an onset of a spin gap for those low-lying excitations. Usually this onset of a field-induced spin gap is related to the presence of a staggered Dzyaloshinskii-Moriya interaction, or to the staggered effective g factors of magnetic ions. Experiments on thermodynamic properties cannot distinguish between those two origins for the spin-gap formation. Here we propose the setup for an experiment, in which one can clearly distinguish between the staggered Dzyaloshinskii-Moriya coupling and staggered external magnetic field: an electronic paramagnetic resonance in the parallel pumping geometry. The characteristics of the system under conditions of such an experiment, i.e., the renormalization of the homogeneous and staggered magnetizations, power of the microwave magnetic field, absorbed by the system, are calculated. Several important features of the solution are discussed.
Abstract A spin-1/2 Heisenberg antiferromagnetic chain is one of the most important paradigmatic models in quantum magnetism. Its ground state is a spin singlet, while the excitation spectrum is formed by gapless fractional excitations, spinons. The presence of alternating g-tensors and/or the staggered Dzyaloshinskii-Moriya interaction results in opening the energy gap Δ∝H2/3\varDelta \propto H^{2/3}Δ∝H2/3 Δ ∝ H 2 / 3 , once the magnetic field H is applied. A fairly good understanding of this phenomenon was achieved in the framework of the sine-Gordon quantum-field theory, taking into account the effective transverse staggered field induced by the applied uniform field. The theory predicts solitons and antisolitons as elementary excitations, as well as their bound states, breathers. Here, I review recent high-field electron spin resonance spectroscopy studies of such systems, focusing on peculiarities of their spin dynamics in the sine-Gordon regime and beyond.
We investigated the thermodynamic properties of the spin-1/2 one-dimensional Heisenberg antiferromagnet KCuGaF6{}_{6}6​ by measuring the specific heat in magnetic fields. When this compound is subjected to a uniform magnetic field $\mathbit{H}$, a transverse staggered magnetic field $\mathbit{h}$ is induced in this compound owing to the staggered component of the $\mathbit{g}$ tensor and the Dzyaloshinskii-Moriya interaction with an alternating $\mathbit{D}$ vector. Consequently, the quantum sine-Gordon (SG) model is an effective model of this compound in a uniform magnetic field. In three different field directions, we observed a magnetic-field-induced gap, which increases with HHH. We analyzed experimental results using specific heat theory based on quantum SG theory. The thermodynamic property for $H\phantom{\rule{0.16em}{0ex}}\ensuremath{\parallel}\phantom{\rule{0.16em}{0ex}}c$ is very well described in terms of the elementary excitations characteristic of the quantum SG model, while for the other field directions significant contributions from other excitation modes beyond the framework of the quantum SG model were observed. For $H\phantom{\rule{0.16em}{0ex}}\ensuremath{\parallel}\phantom{\rule{0.16em}{0ex}}b$, a quantum phase transition between gapless and gapped ground states was observed.
Magnetic excitations in copper pyrimidine dinitrate, a spin-1/2 antiferromagnetic chain with alternating ggg-tensor and Dzyaloshinskii-Moriya interactions that exhibits a field-induced spin gap, are probed by means of pulsed-field electron-spin-resonance spectroscopy. In particular, we report on a minimum of the gap in the vicinity of the saturation field Hsat=48.5{H}_{\mathrm{sat}}=48.5Hsat​=48.5 T associated with a transition from the sine-Gordon region (with soliton-breather elementary excitations) to a spin-polarized state (with magnon excitations). This interpretation is fully confirmed by the quantitative agreement over the entire field range of the experimental data with the density matrix renormalization group calculations for a spin-1/2 Heisenberg chain with a staggered transverse field.
This article is a review of the recent achievements in experimental studies of magnetic excitations in the copper pyrimidine dinitrate [PM–Cu(NO3)2(H2O)2]n (PM = pyrimidine), an S = 1/2 antiferromagnetic chain material with an alternating g-tensor and the Dzyaloshinskii–Moriya interaction, by means of high-field electron spin resonance (ESR). Due to this alternation, in the 1D critical regime this material exhibits a field-induced gap. The excitation spectrum is formed by solitons and their bound states, breathers, and can be effectively described using the sine-Gordon model. With increasing temperature, the soliton-breather regime can be suppressed, resulting in a substantial evolution of ESR parameters. These changes can be described using a new theoretical concept recently proposed for S = 1/2 AF chains with a staggered transverse field. High magnetic field induces a transition into the spin-polarized state with the excitation spectrum formed by magnons. Nonmonotonous behavior of the field-induced gap is observed in vicinity of the saturation field. Experimental data are compared with results of existing theoretical approaches, revealing excellent agreement with predictions.
The magnetic-excitation spectrum of copper pyrimidine dinitrate, a material containing S = 1/2 antiferromagnetic chains with alternating g -tensor and the Dzyaloshinskii-Moriya interaction, and exhibiting a field-induced spin gap, is probed using tunable-frequency electron spin resonance spectroscopy in magnetic fields up to 25 T. The data are interpreted in frame of the sine-Gordon quantum-field theoretical concept proposed recently by Oshikawa and Affleck. The field-induced gap is measured directly ; signatures of soliton and three breather branches are identified.
We study magnetic excitations for anisotropic spin dimer systems. We present a theory that describes not only the lowest-lying excitation mode but also higher-lying modes of the spin dimers, where the latter modes are important for quantum phase transitions driven by magnetic field and pressure in spin-gapped systems. As the most intriguing application, we calculate electron spin resonance (ESR) intensity in the presence of Dzyaloshinskii–Moriya (DM) interaction, which couples the local triplet with the singlet states of the dimer. The ESR intensities under various configurations of the DM interactions are reported in both disordered and field-induced ordered phases, which are very useful for the analysis of high-field ESR data.