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arXiv:cond-mat/0506323

Dynamical projection of atoms to Feshbach molecules at strong coupling

Roman A. Barankov, Leonid S Levitov

Published Jun 14, 2005• 7 citations
arXivHTMLPDF

Abstract

The dynamical atom/molecule projection, recently used to probe fermion pairing, is fast compared to collective fermion times, but slow on the Feshbach resonance width scale. Theory of detuning-induced dynamics of molecules coupled to resonantly associating atom pairs, employing a time-dependent many-body Green's function approach, is presented. An exact solution is found, predicting a 1/3 power law for molecule production efficiency at fast sweep. The results for $s$- and p-wave resonances are obtained and compared. The predicted production efficiency agrees with experimental observations for both condensed and incoherent molecules away from saturation.

DOI
10.48550/arxiv.cond-mat/0506323

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The dynamical atom/molecule projection, recently used to probe fermion pairing, is fast compared to collective fermion times, but slow on the Feshbach resonance width scale. Theory of detuning-induced dynamics of molecules coupled to resonantly associating atom pairs, employing a time-dependent many-body Green's function approach, is presented. An exact solution is found, predicting a 1/3 power law for molecule production efficiency at fast sweep. The results for sss- and p-wave resonances are obtained and compared. The predicted production efficiency agrees with experimental observations for both condensed and incoherent molecules away from saturation.
Fast sweep projection onto Feshbach molecules has been widely used as a probe to explore the properties of fermionic condensates, in particular the condensate fraction. By determining the exact dynamics of a pair of atoms in time varying magnetic fields across a Feshbach resonance, we calculate the number of condensed and noncondensed molecules created after fast magnetic field sweeps from the BCS to the BEC side of the resonance. We analyse the dependence of the molecular conversion efficiency for condensed and noncondensed molecules on the sweep rate, and on the initial and final magnetic fields, for 40^{40}40K and 6^{6}6Li resonances; and discuss the relation between the initial fermionic condensate fraction and the molecular condensate fraction measured after the sweep.
Fast-sweep projection onto Feshbach molecules has been widely used as a probe of fermionic condensates. By determining the exact dynamics of a pair of atoms in time-varying magnetic fields, we calculate the number of condensed and noncondensed molecules created after fast magnetic field sweeps from the BCS to the Bose-Einstein condensate side of the resonances in 40K and 6Li, for different sweep rates and a range of initial and final fields. We discuss the relation between the initial fermionic condensate fraction and the molecular condensate fraction measured after the sweep.
We describe and justify a simple model for the dynamics associated with rapid sweeps across a Feshbach resonance, from the atomic to the molecular side, in an ultracold Fermi system. The model allows us to relate the observed molecule momentum distribution to equilibrium properties of the initial state. In particular, the dependence of the total molecule number on the sweep rate is found to be a sensitive probe of pairing in the initial state, whether condensed or not. This can be used to establish the presence of a phase fluctuation induced "pseudogap" phase in these systems.
The variation of a magnetic field in the vicinity of a zero-energy resonance allows highly vibrationally excited molecules (‘Feshbach molecules’) to be produced from an ultracold atomic gas. In this thesis, we study the dynamics of this process. We begin by studying the dissociation of Feshbach molecules, showing that in the limit of a sudden jump the shape of the spectrum of dissociated atoms can act as a probe of the zero-energy resonance. For some resonances, such jumps are within reach of current experiments. We also study the intermediate region between sudden jumps and asymptotically wide, linear ramps. It is shown from a precise derivation how the latter limit leads to a universal spectrum with a shape independent of the implementation of the two-body physics, provided that the near-resonant scattering properties are correctly modelled. We then turn to the dynamics of Feshbach molecule production from thermal and condensed gases. Our microscopic quantum dynamics approach includes the exact twobody evolution as an input to the many-body calculations. We show that in the long-time limit, and the Markov limit for the interactions, the non-Markovian Boltzmann equation (NMBE) we derive for the one-body density matrix reduces to the normal Boltzmann equation. In the limit of short times and small depletion of the atomic gas, the molecule production efficiency can be calculated by thermally averaging the two-body transition probability density. This thermal averaging technique is applied to studies of the formation of Feshbach molecules using a magnetic field modulation that is near-resonant with the molecular bound state energy. The continuum is shown to have a significant effect on both the dynamics and efficiency of this process. We examine the dependence of the molecule production efficiency on the duration, amplitude and frequency of the modulation, as well as the temperature and density of the gas. This method of producing molecules is effective for a wide range of bound state energies, but requires sufficient variation of the two-body energy levels with magnetic field. Lastly, we implement the NMBE for the case of a fast linear ramp across a Feshbach resonance. The solution of this equation is made feasible by including a large part of the required computation in the kernel, which is calculated in advance. The NMBE allows predictions of the molecule production efficiency which go beyond the thermal averaging technique by accounting for the depletion and rethermalisation of the continuum. In the limit of small depletions, the two approaches give the same results. As the depletion increases, the two approaches differ due to many-body effects limiting the maximum possible molecule production efficiency. We have observed this in our simulations by considering higher-density gases. We have therefore shown the suitability and practicability of this beyond mean-field approach for application to further problems in the production of Feshbach molecules from ultracold gases.
The dynamics of pair condensate formation in a strongly interacting Fermi gas close to a Feshbach resonance was studied. We employed a phase-shift method in which the delayed response of the many-body system to a modulation of the interaction strength was recorded. The observable was the fraction of condensed molecules in the cloud after a rapid magnetic field ramp across the Feshbach resonance. The measured response time was slow compared to the rapid ramp, which provides final proof that the molecular condensates reflect the presence of fermion pair condensates before the ramp.
We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of 40{}^{40}40K and 87{}^{87}87Rb atoms, where we can create 40{}^{40}40K87{}^{87}87Rb molecules with a conversion efficiency as high as 45%. In the limit of fast magnetic sweeps and small molecule fraction, we find that the time scale of molecule production is accurately predicted by a parameter-free model that uses only the atomic densities, masses, and the known Feshbach resonance parameters. We find that molecule production efficiency saturates for slower magnetic sweeps, at which point the maximum number of Feshbach molecules depends primarily on the atoms' phase-space density. At higher temperatures, our measurements agree with a phenomenological model that successfully describes the formation of bosonic molecules from either Bose or Fermi gases. However, for quantum degenerate atom gas mixtures, we measure significantly fewer molecules than this model predicts.