Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1212.0903 · Physical Review A

Feshbach-molecule formation in a Bose-Fermi mixture

Tyler D. Cumby, Ruth Shewmon, Ming-Guang Hu, John D. Perreault, Deborah Jin

Published Jan 7, 2013• 35 citations
arXivHTMLPDF

Abstract

We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of ${}^{40}$K and ${}^{87}$Rb atoms, where we can create ${}^{40}$K${}^{87}$Rb molecules with a conversion efficiency as high as 45%. In the limit of fast magnetic sweeps and small molecule fraction, we find that the time scale of molecule production is accurately predicted by a parameter-free model that uses only the atomic densities, masses, and the known Feshbach resonance parameters. We find that molecule production efficiency saturates for slower magnetic sweeps, at which point the maximum number of Feshbach molecules depends primarily on the atoms' phase-space density. At higher temperatures, our measurements agree with a phenomenological model that successfully describes the formation of bosonic molecules from either Bose or Fermi gases. However, for quantum degenerate atom gas mixtures, we measure significantly fewer molecules than this model predicts.

DOI
10.1103/physreva.87.012703

Related papers

Production Efficiency of Ultracold Feshbach Molecules in Bosonic and Fermionic Systems

E. Hodby, Sarah T. Thompson, Cindy A. Regal +5 more

We investigate the production efficiency of ultracold molecules in bosonic 85 Rb and fermionic 40 K when the magnetic field is swept across a Feshbach resonance.For adiabatic sweeps of the magnetic field, the conversion efficiency of each species is solely determined by the phase space density of the atomic cloud, in contrast to a number of theoretical predictions.Our novel model for the adiabatic pairing process, developed from general physical principles, accurately predicts the conversion efficiency for both ultracold gases of bosons and of fermions.In the non-adiabatic regime our measurements of the 85 Rb molecule conversion efficiency follow a Landau Zener model, with a conversion efficiency that is characterized by the density divided by the time derivative of the magnetic field.

WORLD SCIENTIFIC eBooks•Jan 1, 2008•1 citation

Production Efficiency of Ultracold Feshbach Molecules in Bosonic and Fermionic Systems

E. Hodby, Sarah T. Thompson, Cindy A. Regal +5 more

We investigate the production efficiency of ultracold molecules in bosonic 85Rb and fermionic 40K when the magnetic field is swept across a Feshbach resonance. For adiabatic sweeps of the magnetic field, our novel model shows that the conversion efficiency of both species is solely determined by the phase space density of the atomic cloud, in contrast with a number of theoretical predictions. In the nonadiabatic regime our measurements of the 85Rb molecule conversion efficiency follow a Landau-Zener model.

arXiv:cond-mat/0411487•Physical Review Letters•Mar 30, 2005•145 citations

Conversion Efficiency of Ultracold Fermionic Atoms to Bosonic Molecules via Feshbach Resonance Sweep Experiments

E. Pazy, Amichay Vardi, Y. B. Band

We explain why the experimental efficiency observed in the conversion of ultracold Fermi gases of 40K and 6Li atoms into diatomic Bose gases is limited to 0.5 when the Feshbach resonance sweep rate is sufficiently slow to pass adiabatically through the Landau-Zener transition but faster than "the collision rate" in the gas, and increases beyond 0.5 when it is slower. The 0.5 efficiency limit is due to the preparation of a statistical mixture of two spin states, required to enable s-wave scattering. By constructing the many-body state of the system we show that this preparation yields a mixture of even and odd parity pair states, where only even parity can produce molecules. The odd parity spin-symmetric states must decorrelate before the constituent atoms can further Feshbach scatter, thereby increasing the conversion efficiency; "the collision rate" is the pair decorrelation rate.

arXiv:cond-mat/0403362•Physical Review Letters•Sep 16, 2004•23 citations

Formation of ultracold fermionic NaLi Feshbach molecules

Myoung-Sun Heo, Tout T. Wang, Caleb A. Christensen +5 more

We describe the formation of fermionic NaLi Feshbach molecules from an ultracold mixture of bosonic ${}^{23}$Na and fermionic ${}^{6}$Li. Precise magnetic field sweeps across a narrow Feshbach resonance at 745 G result in a molecule conversion fraction of $5%$ for our experimental densities and temperatures, corresponding to a molecule number of $5\ifmmode\times\else\texttimes\fi{}{10}^{4}$. The observed molecular decay lifetime is $1.3$ ms after removing free Li and Na atoms from the trap. Due to its extremely low reactivity, NaLi molecules in the ground state will have a much longer lifetime than KRb.

arXiv:1205.5304•Physical Review A•Aug 6, 2012•112 citations

Enhanced magnetoassociation of $^6$Li in the quantum degenerate regime

Vineetha Naniyil, Yijia Zhou, Guy Simmonds +3 more

We study magnetic Feshbach resonance of ultracold $^6$Li atoms in a dipole trap close to quantum degeneracy. The experiment is carried out by linearly ramping down the magnetic field from the BCS to the BEC side around the broad resonance at $B_r=834.1$G. The Feshbach molecule formation efficiency depends strongly on the temperature of the atomic gas and the rate at which the magnetic field is ramped across the Feshbach resonance. The molecular association process is well described by the Landau-Zener transition while above the Fermi temperature, such that two-body physics dominates the dynamics. However, we observe an enhancement of the atom-molecule coupling as the Fermionic atoms reach degeneracy, demonstrating the importance of many-body coherence not captured by the conventional Landau-Zener model. We develop a theoretical model that explains the temperature dependence of the atom-molecule coupling. Furthermore, we characterize this dependence experimentally and extract the atom-molecule coupling coefficient as a function of temperature, finding qualitative agreement between our model and experimental results. Accurate measurement of this coupling coefficient is important for both theoretical and experimental studies of atom-molecule association dynamics.

•Feb 3, 2021•0 citations

Formation of ultracold NaRb Feshbach molecules

Fudong Wang, Xiaodong He, Xiaoke Li +3 more

We report the creation of ultracold bosonic 23 Na 87 Rb Feshbach molecules via magneto-association. By ramping the magnetic field across an interspecies Feshbach resonance (FR), at least 4000 molecules can be produced out of the near degenerate ultracold mixture. Fast loss due to inelastic atom–molecule collisions is observed, which limits the pure molecule number, after residual atoms removal, to 1700. The pure molecule sample can live for 21.8(8) ms in the optical trap, long enough for future molecular spectroscopy studies toward coherently transferring to the singlet ro-vibrational ground state, where these molecules are stable against chemical reaction and have a permanent electric dipole moment of 3.3 Debye. We have also measured the Feshbach molecule's binding energy near the FR by the oscillating magnetic field method and found these molecules have a large closed-channel fraction.

arXiv:1502.03869•New Journal of Physics•Mar 6, 2015•53 citations
We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of 40{}^{40}40K and 87{}^{87}87Rb atoms, where we can create 40{}^{40}40K87{}^{87}87Rb molecules with a conversion efficiency as high as 45%. In the limit of fast magnetic sweeps and small molecule fraction, we find that the time scale of molecule production is accurately predicted by a parameter-free model that uses only the atomic densities, masses, and the known Feshbach resonance parameters. We find that molecule production efficiency saturates for slower magnetic sweeps, at which point the maximum number of Feshbach molecules depends primarily on the atoms' phase-space density. At higher temperatures, our measurements agree with a phenomenological model that successfully describes the formation of bosonic molecules from either Bose or Fermi gases. However, for quantum degenerate atom gas mixtures, we measure significantly fewer molecules than this model predicts.
We investigate the production efficiency of ultracold molecules in bosonic 85 Rb and fermionic 40 K when the magnetic field is swept across a Feshbach resonance.For adiabatic sweeps of the magnetic field, the conversion efficiency of each species is solely determined by the phase space density of the atomic cloud, in contrast to a number of theoretical predictions.Our novel model for the adiabatic pairing process, developed from general physical principles, accurately predicts the conversion efficiency for both ultracold gases of bosons and of fermions.In the non-adiabatic regime our measurements of the 85 Rb molecule conversion efficiency follow a Landau Zener model, with a conversion efficiency that is characterized by the density divided by the time derivative of the magnetic field.
We investigate the production efficiency of ultracold molecules in bosonic 85Rb and fermionic 40K when the magnetic field is swept across a Feshbach resonance. For adiabatic sweeps of the magnetic field, our novel model shows that the conversion efficiency of both species is solely determined by the phase space density of the atomic cloud, in contrast with a number of theoretical predictions. In the nonadiabatic regime our measurements of the 85Rb molecule conversion efficiency follow a Landau-Zener model.
We explain why the experimental efficiency observed in the conversion of ultracold Fermi gases of 40K and 6Li atoms into diatomic Bose gases is limited to 0.5 when the Feshbach resonance sweep rate is sufficiently slow to pass adiabatically through the Landau-Zener transition but faster than "the collision rate" in the gas, and increases beyond 0.5 when it is slower. The 0.5 efficiency limit is due to the preparation of a statistical mixture of two spin states, required to enable s-wave scattering. By constructing the many-body state of the system we show that this preparation yields a mixture of even and odd parity pair states, where only even parity can produce molecules. The odd parity spin-symmetric states must decorrelate before the constituent atoms can further Feshbach scatter, thereby increasing the conversion efficiency; "the collision rate" is the pair decorrelation rate.
We describe the formation of fermionic NaLi Feshbach molecules from an ultracold mixture of bosonic 23{}^{23}23Na and fermionic 6{}^{6}6Li. Precise magnetic field sweeps across a narrow Feshbach resonance at 745 G result in a molecule conversion fraction of 55%5 for our experimental densities and temperatures, corresponding to a molecule number of $5\ifmmode\times\else\texttimes\fi{}{10}^{4}$. The observed molecular decay lifetime is 1.31.31.3 ms after removing free Li and Na atoms from the trap. Due to its extremely low reactivity, NaLi molecules in the ground state will have a much longer lifetime than KRb.
Enhanced magnetoassociation of 6^66Li in the quantum degenerate regime
We study magnetic Feshbach resonance of ultracold 6^66Li atoms in a dipole trap close to quantum degeneracy. The experiment is carried out by linearly ramping down the magnetic field from the BCS to the BEC side around the broad resonance at Br=834.1B_r=834.1Br​=834.1G. The Feshbach molecule formation efficiency depends strongly on the temperature of the atomic gas and the rate at which the magnetic field is ramped across the Feshbach resonance. The molecular association process is well described by the Landau-Zener transition while above the Fermi temperature, such that two-body physics dominates the dynamics. However, we observe an enhancement of the atom-molecule coupling as the Fermionic atoms reach degeneracy, demonstrating the importance of many-body coherence not captured by the conventional Landau-Zener model. We develop a theoretical model that explains the temperature dependence of the atom-molecule coupling. Furthermore, we characterize this dependence experimentally and extract the atom-molecule coupling coefficient as a function of temperature, finding qualitative agreement between our model and experimental results. Accurate measurement of this coupling coefficient is important for both theoretical and experimental studies of atom-molecule association dynamics.
We report the creation of ultracold bosonic 23 Na 87 Rb Feshbach molecules via magneto-association. By ramping the magnetic field across an interspecies Feshbach resonance (FR), at least 4000 molecules can be produced out of the near degenerate ultracold mixture. Fast loss due to inelastic atom–molecule collisions is observed, which limits the pure molecule number, after residual atoms removal, to 1700. The pure molecule sample can live for 21.8(8) ms in the optical trap, long enough for future molecular spectroscopy studies toward coherently transferring to the singlet ro-vibrational ground state, where these molecules are stable against chemical reaction and have a permanent electric dipole moment of 3.3 Debye. We have also measured the Feshbach molecule's binding energy near the FR by the oscillating magnetic field method and found these molecules have a large closed-channel fraction.