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arXiv:cond-mat/0506154 · Physical Review B

Spin dynamics and violation of the fluctuation dissipation theorem in a nonequilibrium ohmic spin-boson model

Aditi Mitra, Andrew J. Millis

Published Sep 14, 2005• 30 citations
arXivHTMLPDF

Abstract

We present results for the dynamics of an impurity spin coupled to a magnetic field and to two ohmic baths that are out of equilibrium due to the application of a bias voltage. Both the nonequilibrium steady state and the rate constants describing the approach to the steady state are found to depend sensitively on the relative strengths of a magnetic field and a voltage dependent decoherence rate. Computation of physical quantities, including the frequency dependent ratio of the response to the correlation functions and the probabilities of the two spin states, allows the extraction of voltage dependent effective temperatures. The temperatures extracted from different quantities differ from one another in magnitude and in their dependence on parameters, and, in general, are nonmonotonic.

DOI
10.1103/physrevb.72.121102

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We present results for the dynamics of an impurity spin coupled to a magnetic field and to two ohmic baths that are out of equilibrium due to the application of a bias voltage. Both the nonequilibrium steady state and the rate constants describing the approach to the steady state are found to depend sensitively on the relative strengths of a magnetic field and a voltage dependent decoherence rate. Computation of physical quantities, including the frequency dependent ratio of the response to the correlation functions and the probabilities of the two spin states, allows the extraction of voltage dependent effective temperatures. The temperatures extracted from different quantities differ from one another in magnitude and in their dependence on parameters, and, in general, are nonmonotonic.
The quantum dynamics of a two-level system coupled to an Ohmic spin bath is studied by means of the perturbation approach based on a unitary transformation. A scattering function xi(k) is introduced in the transformation to take into account quantum fluctuations. By the master equation within the Born approximation, nonequilibrium dynamics quantities are calculated. The method works well for the coupling constant 0<alpha<alpha(c) and a finite bare tunneling Delta. It is found that (i) only at zero temperature with small coupling or moderate one does the spin-spin-bath model display identical behavior as the well-known spin-boson-bath model; (ii) in comparison with the known results of spin-boson-bath model, the coherence-incoherence transition point, which occurs at alpha(c)=12[1+etaDelta/omega(c)], is temperature independent; and (iii) the nonequilibrium correlation function P(t)=tau(z)(t), evolves without temperature dependence, while tau(x)(t) depends on temperature. Both P(t) and tau(x)(t) not only satisfy their initial conditions, respectively, and also have correct long time limits. Besides, the Shiba relation and sum rule are exactly satisfied in the coherent regime for this method. Our results show that increasing temperature does not help the system suppress decoherence in the coherent regime, i.e., finite temperature does not favor the coherent dynamics in this regime. Thus, the finite-temperature dynamics induced by two kinds of baths (spin-bath and boson-bath) exhibit distinctly different physics.
Dissipative processes in nonequilibrium many-body systems are fundamentally different than their equilibrium counterparts. Such processes are of great importance for the understanding of relaxation in single-molecule devices. As a detailed case study, we investigate here a generic spin-fermion model, where a two-level system couples to two metallic leads with different chemical potentials. We present results for the spin relaxation rate in the nonadiabatic limit for an arbitrary coupling to the leads using both analytical and exact numerical methods. The nonequilibrium dynamics is reflected by an exponential relaxation at long times and via complex phase shifts, leading in some cases to an ``antiorthogonality'' effect. In the limit of strong system-lead coupling at zero temperature we demonstrate the onset of a Marcus-like Gaussian decay with voltage difference activation. This is analogous to the equilibrium spin-boson model, where at strong coupling and high temperatures, the spin excitation rate manifests temperature activated Gaussian behavior. We find that there is no simple linear relationship between the role of the temperature in the bosonic system and a voltage drop in a nonequilibrium electronic case. The two models also differ by the orthogonality-catastrophe factor existing in a fermionic system, which modifies the resulting line shapes. Implications for current characteristics are discussed. We demonstrate the violation of pairwise Coulomb gas behavior for strong coupling to the leads. The results presented in this paper form the basis of an exact, nonperturbative description of steady-state quantum dissipative systems.
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We derive a consistent two-loop scaling picture for a Kondo dot in both equilibrium and nonequilibrium situations using the flow equation method. Our analysis incorporates the important decoherence effects from both thermal and nonequilibrium noise in a common setting. In the weak-coupling regime we calculate the spin-spin correlation function, the T-matrix, and the magnetization as functions of applied magnetic field, dc-voltage bias and temperature. In all these quantities we observe characteristic nonequilibrium features for a nonvanishing external voltage bias such as Kondo splitting and strongly enhanced logarithmic corrections.
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We investigate the effect of dissipation in a Bose Josephson junction (BJJ) coupled to bath of bosons at two sites as an application of the generalized spin-boson model. Apart from the dynamical transition due to repulsive interactions, the BJJ undergoes a quantum phase transition by increasing the coupling strength with the bath modes. We analyze this system by mapping to an equivalent spin model coupled to the bosonic modes. The excitation energies and fluctuation of number imbalance are obtained within Holstein-Primakoff approximation, which exhibits vanishing of energy gap and enhanced quantum fluctuations at the critical coupling. We study the dynamics of BJJ using time-dependent variational method and analyze stability of different types of steady states. As a special case, we study in details the phase space dynamics of BJJ coupled to a single-mode, which reveals diffusive and incoherent behaviour with increasing coupling to the bath mode. The dynamical steady states corresponding to the Pi-oscillation and self-trapped state become unstable in the region where their oscillation frequencies are in resonance with the bath modes. We investigate the time evolution of number imbalance and relative phase in presence of Ohmic bath with Gaussian noise to incorporate thermal fluctuations. Apart from the damping of Josephson oscillations and transition to symmetry broken state for strong coupling, we observe the decay of Pi-oscillation and self-trapped state to the ground state as a result of dissipation. Variation of phase fluctuation with temperature of the bath shows similar behaviour as observed in the experiments.