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arXiv:cond-mat/0505353 · Physical Review Letters

Molecular Probe of Pairing in the BEC-BCS Crossover

Guthrie B. Partridge, Kevin E. Strecker, Ramsey I. Kamar, Michael W. Jack, Randall G. Hulet

Published Jul 7, 2005• 414 citations
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Abstract

We have used optical molecular spectroscopy to probe the many-body state of paired 6Li atoms near a broad Feshbach resonance. The optical probe projects pairs of atoms onto a vibrational level of an excited molecule. The rate of excitation enables a precise measurement of the closed-channel contribution to the paired state. This contribution is found to be quite small, supporting the concept of universality for the description of broad Feshbach resonances. The dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover and into the weakly interacting BCS regime.

DOI
10.1103/physrevlett.95.020404

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We have used optical molecular spectroscopy to probe the many-body state of paired 6Li atoms near a broad Feshbach resonance. The optical probe projects pairs of atoms onto a vibrational level of an excited molecule. The rate of excitation enables a precise measurement of the closed-channel contribution to the paired state. This contribution is found to be quite small, supporting the concept of universality for the description of broad Feshbach resonances. The dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover and into the weakly interacting BCS regime.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.
Atomic Feshbach resonances have recently been used to produce a strongly interacting Fermi gas, where the BCS/BEC crossover can be explored. We have used both narrow and broad Feshbach resonances to convert a quantum degenerate Fermi gas of 6Li atoms into an ultracold gas of Li2 molecules. For the narrow resonances, the molecules are formed by coherent adiabatic passage through the resonance. We find that 50% of the atoms are converted to molecules. Furthermore, the lifetime of these molecules was measured to be surprisingly long, 1 s. We will discuss these measurements in the context of the present theoretical understanding. Molecules can also be formed using static fields near the broad Feshbach resonance. The lifetime of these molecules is again long, and sufficient to enable their evaporation to a Bose‐Einstein condensate. Phase contrast images of the molecular condensate are presented. The BCS/BEC crossover may be explored by starting with a pure molecular condensate on the low‐field side of the Feshbach resonance, and adiabatically changing the field to any final value around resonance. We combine this ability with optical spectroscopy on a bound‐bound molecular transition to probe the nature of the many‐body wavefunction in the crossover regime.
We present a comprehensive study of the Bose-Einstein condensate to Bardeen-Cooper-Schrieffer (BEC-BCS) crossover in fermionic 6Li using Bragg spectroscopy. A smooth transition from molecular to atomic spectra is observed with a clear signature of pairing at and above unitarity. These spectra probe the dynamic and static structure factors of the gas and provide a direct link to two-body correlations. We have characterized these correlations and measured their density dependence across the broad Feshbach resonance at 834 G.
Understanding the effects of interactions on the ground-state of a paired degenerate Fermi gas throughout the BEC-BCS crossover has been a long standing physical quest for which countless papers have been written. The crossover describes the smooth transition of the physics of a BEC of tightly bound dimers to that of a paired BCS superfluid. A Feshbach resonance is used to tune the interactions necessary to study the crossover. Right around resonance the interactions are expected to be parameterized by a single universal parameter beta [1--3]. This thesis describes a measurement of the axial size of paired, 6Li clouds in the BEC-BCS crossover and provides a comparison with theory. In the BEC regime, absolute measurements of the molecular scattering length are compared with the atomic scattering length and the ratio is compared with theory. Finally, a measurement of beta is made and compared with theory.
We present an overview of our recent measurements on the crossover from a Bose‐Einstein condensate of molecules to a Bardeen‐Cooper‐Schrieffer superfluid. The experiments are performed on a two‐component spin‐mixture of 6Li atoms, where a Feshbach resonance serves as the experimental key to tune the s‐wave scattering length and thus to explore the various interaction regimes. In the BEC‐BCS crossover, we have characterized the interaction energy by measuring the size of the trapped gas, we have studied collective excitation modes, and we have observed the pairing gap. Our observations provide strong evidence for superfluidity in the strongly interacting Fermi gas.
We measure excitation spectra of an ultracold gas of fermionic (40)K atoms in the BCS-Bose-Einstein-condensation (BEC) crossover regime. The measurements are performed with a novel spectroscopy that employs a small modulation of the B field close to a Feshbach resonance to give rise to a modulation of the interaction strength. With this method we observe both a collective excitation as well as the dissociation of fermionic atom pairs in the strongly interacting regime. The excitation spectra reveal the binding energy or excitation gap for pairs in the crossover region.