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arXiv:cond-mat/0504123 · Journal of the Physical Society of Japan

Effective Interaction between Molecules in the Strong-Coupling BEC Regime of a Superfluid Fermi Gas

Yoji Ohashi

Published Oct 1, 2005• 17 citations
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Abstract

We investigate the effective interaction between Cooper-pair molecules in the st rong-coupling BEC regime of a superfluid Fermi gas with a Feshbach resonance. Our work uses a path integral formulation and a renormalization group (RG) analy sis of fluctuations in a single-channel model. We show that a physical cutoff en ergy $ω_c$ originating from the finite molecular binding energy is the key to understanding the interaction between molecules in the BEC regime. Our work t hus clarifies recent results by showing that $a_{\rm M}=2a_{\rm F}$ is a {\it ba re} molecular scattering length while $a_{\rm M}=(0.6\sim0.75) a_{\rm F}$ is the low energy molecular scattering length renormalized to include high-energy scat tering up to $ω_c$ (here $a_{\rm F}$ is the scattering length between Fermi atoms). We also include many-body effects at finite temperatures. We find that $a_{\rm M}$ is strongly dependent on temperature, vanishing at $T_{\rm c}$, consistent with the earlier Bose gas results of Bijlsma and Stoof.

DOI
10.1143/jpsj.74.2659

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We investigate the effective interaction between Cooper-pair molecules in the st rong-coupling BEC regime of a superfluid Fermi gas with a Feshbach resonance. Our work uses a path integral formulation and a renormalization group (RG) analy sis of fluctuations in a single-channel model. We show that a physical cutoff en ergy ωcω_cωc​ originating from the finite molecular binding energy is the key to understanding the interaction between molecules in the BEC regime. Our work t hus clarifies recent results by showing that aM=2aFa_{\rm M}=2a_{\rm F}aM​=2aF​ is a {\it ba re} molecular scattering length while aM=(0.6∼0.75)aFa_{\rm M}=(0.6\sim0.75) a_{\rm F}aM​=(0.6∼0.75)aF​ is the low energy molecular scattering length renormalized to include high-energy scat tering up to ωcω_cωc​ (here aFa_{\rm F}aF​ is the scattering length between Fermi atoms). We also include many-body effects at finite temperatures. We find that aMa_{\rm M}aM​ is strongly dependent on temperature, vanishing at TcT_{\rm c}Tc​, consistent with the earlier Bose gas results of Bijlsma and Stoof.
We study the system of a dilute gas of fermions in 3-dimensions, with attractive interactions tuned to the unitarity point, using the non-perturbative Restricted Path Integral Monte Carlo (R-PIMC) method. The pairing and superfluid properties of this system are calculated at finite temperature. The total energy at very low temperature from our results agrees closely with that of previous ground-state Quantum Monte Carlo calculations. We identify the temperature T � � 0.70ǫF below which pairing correlations develop, and estimate the critical temperature for the superfluid transition Tc � 0.25ǫF from a finite size scaling analysis of the superfluid density. PACS numbers: The recent experiments, starting with generating a degenerate gas of cold atoms[3], the use of Feshbach resonance to tune the effective interaction between the fermions[4, 5], the measurements of the gap to identify a pairing scale[6] and the measurements of vortices[7] to identify the superfluid state, have all given an impetus to the study of superfluidity in the BCS-BEC crossover regime. The nature of superconductivity or superfluidity in a many-particle system with an increasing pairing attraction was shown [1, 2] to interpolate smoothly between the BCS regime for weak attraction between the fermions, and the Bose-Einstein condensation (BEC) regime for strong coupling. In the weak coupling regime, the Cooper pair size is much larger than the interparticle spacing, and the simultaneous pairing and condensation of fermions is well described by the BCS theory. In the strong coupling regime, fermions form strongly bound bosonic molecules at a pairing temperature scale T ∗ that is considerably higher than the BEC temperature Tc. In a two species system of fermions with an attractive interaction between them, the unitary point is defined by the divergence of the zero energy s-channel scattering length, as, for two particles in free space. The unitary point is interesting since it describes a strongly correlated system with universal properties[8]. In general, there are two length scales that define the system: the interparticle spacing ∝ n −1/3 , and the scattering length as which contains information about the interaction potential. At the unitary point however, since as diverges, all the properties of the system are described by a single length scale k −1
With help of a Feshbach scattering resonance it is possible to change the effective two-body interaction of ultra-cold atoms from repulsive to attractive, from weak to strong. Regular field theory for the description of Bose-Einstein condensates is based on a single interaction parameter only, the scattering length. Such a description, however, is not valid anymore for the resonance regime. We formulated a field-theory that incorporated the microscopic energy-dependent two-body interactions, that also takes pair correlations into account. This theory allowed us to explain an experiment at JILA where Ramsey fringes were observed in a ^85Rb Bose-Einstein condensate by making use of a Feshbach resonance. The theory and experiment show that coherent molecules are created, a first step in the direction of molecular BEC. For non-resonant interactions, the self-energy corresponding to the atom-atom interactions is proportional to the scattering length. Close to resonance, however, this relationship no longer applies, and the energy will level off to a finite value on resonance. We investigate this resonance self-energy, and compare it with experimental results from strongly interacting Fermi systems.
A self-consistent theory is derived to describe the BCS--Bose-Einstein-condensate crossover for a strongly interacting Fermi gas with a Feshbach resonance. In the theory the fluctuation of the dressed molecules, consisting of both preformed Cooper pairs and ``bare'' Feshbach molecules, has been included within a self-consistent TTT-matrix approximation, beyond the Nozi\`eres and Schmitt-Rink strategy considered by Ohashi and Griffin. The resulting self-consistent equations are solved numerically to investigate the normal-state properties of the crossover at various resonance widths. It is found that the superfluid transition temperature Tc{T}_{c}Tc​ increases monotonically at all widths as the effective interaction between atoms becomes more attractive. Furthermore, a residue factor Zm{Z}_{m}Zm​ of the molecule's Green function and a complex effective mass have been determined to characterize the fraction and lifetime of Feshbach molecules at Tc{T}_{c}Tc​. Our many-body calculations of Zm{Z}_{m}Zm​ agree qualitatively well with recent measurments of the gas of 6Li^{6}\mathrm{Li}6Li atoms near the broad resonance at 834G834\phantom{\rule{0.3em}{0ex}}\mathrm{G}834G. The crossover from narrow to broad resonances has also been studied.
We investigate strong-coupling superfluidity in a uniform two-component gas of ultracold Fermi atoms attractively interacting via quasimolecular bosons associated with a Feshbach resonance. This interaction is tunable by the threshold energy $2\ensuremath{\nu}$ of the Feshbach resonance, becoming large as $2\ensuremath{\nu}$ is decreased (relative to $2{\ensuremath{\varepsilon}}_{\mathrm{F}},$ where ${\ensuremath{\varepsilon}}_{\mathrm{F}}$ is the Fermi energy of one component). In recent work, we showed that the enhancement of this tunable pairing interaction naturally leads to the BCS-BEC (Bose-Einstein condensation) crossover, where the character of the superfluid phase transition changes from the BCS type to a BEC of composite bosons consisting of preformed Cooper-pairs and Feshbach-induced molecules. In this paper, we extend our previous work and study both the quasiparticles and the collective dynamics of the superfluid phase below the phase-transition temperature Tc,{T}_{\mathrm{c}},Tc​, limiting ourselves to a uniform gas. We show how the superfluid order parameter changes from the Cooper-pair amplitude $\ensuremath{\Delta}$ to the square root of the number of condensed molecules $({\ensuremath{\varphi}}_{\mathrm{m}})$ associated with the Feshbach resonance, as the threshold energy $2\ensuremath{\nu}$ is lowered. In the intermediate coupling regime, the superfluidity is shown to be characterized by an order parameter consisting of a superposition of $\ensuremath{\Delta}$ and ${\ensuremath{\varphi}}_{\mathrm{m}}.$ We also discuss the Goldstone mode associated with superfluidity, and show how its character smoothly changes from the Anderson-Bogoliubov phonon in the BCS regime to the Bogoliubov phonon in the BEC regime in the BCS-BEC crossover. The velocity of this Goldstone phonon mode is shown to strongly depend on the value of $2\ensuremath{\nu}.$ We also show that this Goldstone mode appears as a resonance in the spectrum of the density-density correlation function, which is experimentally accessible.
Bose-Einstein condensation (BEC) of Feshbach molecules in a homogeneous Bose gas is studied at finite temperatures in a single-channel mean-field approach where the Hartree-Fock energy and pairing gap are determined self-consistently. In the molecular-BEC state, the atomic excitation is gapped and the molecular excitation is gapless. The binding energy of Feshbach molecules is shifted from the vacuum value by many-body effects. When the scattering length as{a}_{s}as​ of the atoms is negative, the system is subject to mechanical collapse due to negative compressibility. The system is stable in most regions with positive scattering lengths. However, at low temperatures near the resonance, the molecular-BEC state vanishes, and the coherent mixture of atomic and molecular BEC is subject to mechanical collapse.
We theoretically investigate the isothermal compressibility ${\ensuremath{\kappa}}_{T}$ in the normal state of an ultracold Fermi gas. Including pairing fluctuations, as well as preformed-pair formations, within the framework of the self-consistent TTT-matrix approximation, we evaluate the temperature dependence of this thermodynamic quantity over the entire BCS (Bardeen-Cooper-Schrieffer)-BEC (Bose-Einstein condensation) crossover region. While ${\ensuremath{\kappa}}_{T}$ in the weak-coupling BCS regime is dominated by Fermi atoms near the Fermi surface, correlations between tightly bound Cooper-pair molecules are found to play crucial roles in the strong-coupling BEC regime. In the latter region, besides a two-body molecular interaction, a three-body one is shown to sizably affect ${\ensuremath{\kappa}}_{T}$ near the superfluid phase-transition temperature. Our results indicate that the strong-coupling BEC regime of an ultracold Fermi gas would provide a unique opportunity to study multibody correlations between Cooper-pair molecules.