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arXiv:cond-mat/0501697 · Journal of the Physical Society of Japan

Quantum vs Classical Magnetization Plateaus of S=1/2 Frustrated Heisenberg Chains

Kazuo Hida, Ian K. Affleck

Published Jun 1, 2005• 46 citations
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Abstract

The competition between quantum and classical magnetization plateaus of S=1/2 frustrated Heisenberg chains with modified exchange couplings is investigated. The conventional S=1/2 frustrated Heisenberg chains is known to exhibit a 3-fold degenerate udu-type classical plateau at 1/3 of the saturation magnetization accompanied by the spontaneous Z_3 translational symmetry breakdown. The stability of this plateau phase against period 3 exchange modulation which favors the 00u-type quantum plateau state (00= singlet dimer) is studied by bosonization, renormalization group and numerical diagonalization methods. The ground state phase diagram and the spin configuration in each phase are numerically determined. The translationally invariant Valence Bond Solid-type model with 4-spin and third neighbor interactions, which has the exact 00u-type quantum plateau state, is also presented. The phase transition to the classical udu-type ground state is also observed by varying the strength of 4-spin and third neighbor interactions. The relation between these two types of models with quantum plateau states is discussed.

DOI
10.1143/jpsj.74.1849

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The competition between quantum and classical magnetization plateaus of S=1/2 frustrated Heisenberg chains with modified exchange couplings is investigated. The conventional S=1/2 frustrated Heisenberg chains is known to exhibit a 3-fold degenerate udu-type classical plateau at 1/3 of the saturation magnetization accompanied by the spontaneous Z_3 translational symmetry breakdown. The stability of this plateau phase against period 3 exchange modulation which favors the 00u-type quantum plateau state (00= singlet dimer) is studied by bosonization, renormalization group and numerical diagonalization methods. The ground state phase diagram and the spin configuration in each phase are numerically determined. The translationally invariant Valence Bond Solid-type model with 4-spin and third neighbor interactions, which has the exact 00u-type quantum plateau state, is also presented. The phase transition to the classical udu-type ground state is also observed by varying the strength of 4-spin and third neighbor interactions. The relation between these two types of models with quantum plateau states is discussed.
The magnetization plateau of the S = 1/2 frustrated Heisenberg chain with period 3 parity invariant exchange modulation is investigated by the bosonization and numerical exact diagonalization method. The ground state phase diagram at 1/3 of the saturated magnetization is obtained. Among three degenerate ↑↑↓-type plateau states in the uniform chain, two of them (↓↑↑↓↑↑⋅⋅⋅ and ↑↓↑↑↓↑⋅⋅⋅) turned out to be robust against the period 3 exchange modulation which favors the phase up to a critical value of the modulation amplitude ( = singlet dimer) resulting in the Z2 symmetry broken phase. Another ↑↑↓-type state with ↑↑↓↑↑↓⋅⋅⋅ configuration is stabilized for period 3 modulation with opposite sign. The transition between the -phase and Z2-broken phase is the Ising transition and that between the ↑↑↓↑↑↓⋅⋅⋅ -phase and Z2 broken phase is the first order transition. The spin configuration in each phase is numerically verified by applying the local symmetry breaking field.
The spin-12\frac{1}{2}21​ Heisenberg model on a kagome lattice is a typical frustrated quantum spin system. The basic structure of a kagome lattice is also present in the kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-12\frac{1}{2}21​ Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions using the density-matrix renormalization-group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking translational and/or reflection symmetry spontaneously. The structures are classified by an array of five-site unit cells with specific bond-spin correlations. In a case with a nontrivial plateau, namely a 3/10 plateau, we find long-period magnetic structure with a period of four unit cells.
The ground state properties of the S = 1/ 2 frustrated Heisenberg chain with period 3 exchange modulation are investigated using the numerical diagonalization and density matrix renormalization group (DMRG) method. It is known that this model has a magnetization plateau at one third of the saturation magnetization Ms. On the other hand, the ground state is ferrimagnetic even in the absence of frustration if one of the nearest neighbour bond is ferromagnetic and the others are antiferromagnetic. In the present work, we show that this ferrimagnetic state continues to the region in which all bonds are antiferromagnetic if the frustration is strong. This state further continues to the above- mentioned 1/ 3 plateau state. In between, we also find the noncollinear ferrimagnetic phase in which the spontaneous magnetization is finite but less than Ms/ 3. The intuitive interpretation for the phase diagram is given and the physical properties of these phases are discussed.
We present a numerical study of the magnetization process of frustrated quantum spin-SSS chains with S=1,3∕2,2S=1,3∕2,2S=1,3∕2,2 as well as the classical limit. Using the exact diagonalization and density-matrix renormalization techniques, we provide evidence that a plateau at one third of the saturation magnetization exists in the magnetization curve of frustrated spin-SSS chains with S>1∕2S>1∕2S>1∕2. Similar to the case of S=1∕2S=1∕2S=1∕2, this plateau state breaks the translational symmetry of the Hamiltonian and realizes an up-up-down pattern in the spin component parallel to the external field. Our study further shows that this plateau exists both in the cases of an isotropic exchange and in the easy-axis regime for spin-S=1S=1S=1, 3∕23∕23∕2, and 2, but is absent in classical frustrated spin chains with isotropic interactions. We discuss the magnetic phase diagram of frustrated spin-1 and spin-3∕23∕23∕2 chains as well as other emergent features of the magnetization process such as kink singularities, jumps, and even-odd effects. A quantitative comparison of the one-third plateau in the easy-axis regime between spin-1 and spin-3∕23∕23∕2 chains on the one hand and the classical frustrated chain on the other hand indicates that the critical frustration and the phase boundaries of this state rapidly approach the classical result as the spin SSS increases.
The ground state properties of the S = 1/2 frustrated Heisenberg chain with period 3 exchange modulation are investigated using the numerical diagonalization and density matrix renormalization group (DMRG) method. It is known that this model has a magnetization plateau at one third of the saturation magnetization M s . On the other hand, the ground state is ferrimagnetic even in the absence of frustration if one of the nearest neighbour bond is ferromagnetic and the others are antiferromagnetic. In the present work, we show that this ferrimagnetic state continues to the region in which all bonds are antiferromagnetic if the frustration is strong. This state further continues to the above-mentioned 1/3 plateau state. In between, we also find the noncollinear ferrimagnetic phase in which the spontaneous magnetization is finite but less than M s /3. The intuitive interpretation for the phase diagram is given and the physical properties of these phases are discussed.
Magnetization plateaus in quantum spin systems emerges in two-dimensional frustrated systems such as kagome lattice. The spin-1/2 antiferromagnetic Heisenberg model on square-kagome lattice is also appropriate for the study of magnetization plateau. Motivated by recent experimental finding of such a square-kagome lattice with nonequivalent three bonds, we investigate the phase diagrams and magnetization plateaus of the lattice by the exact diagonalization method. In addition to previously reported the 1/3 and 2/3 plateaus in the model with two equivalent bonds, we find a new 2/3 plateau whose magnetic structure is characterized by spontaneously broken four-fold rotational symmetry. The plateau appears only in the case of three nonequivalent bonds. We propose the possibility of finding plateaus including the new one.