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arXiv:cond-mat/0412013 · Applied Physics Letters

Photon-spin qubit-conversion based on Overhauser shift of Zeeman energies in quantum dots

S. Muto, S. Adachi, T. Yokoi, H. Sasakura, I. Suemune

Published Sep 8, 2005• 24 citations
arXivHTMLPDF

Abstract

We propose a method to realize the conversion of photon qubit and spin qubit using the effective magnetic field created by the nuclear polarization known as Overhauser field. We discuss the preliminary experiment on an InAlAs∕AlGaAs self-assembled quantum dot and also discuss the effects of electron-hole interaction on the conversion.
DOI
10.1063/1.2043229

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We consider two qubits interacting by means of an optical cavity, where each qubit is represented by a single-electron spin confined to a quantum dot. It is known that electron spins in III-V semiconductor quantum dots are affected by the decoherence due to the hyperfine interaction with nuclear spins. Here we show that the interaction between two qubits is influenced by the Overhauser field as well. Starting from an unpolarized nuclear ensemble, we investigate the dependance of the fidelities for two-qubit gates on the Overhauser field. We include the hyperfine interaction pertubatively to second order in our analytical results and to arbitrary precision numerically.
The motivating background for this thesis lies in the recent development in the coherent optical control of electron spin states in semiconductor quan- tum dots. One possible and attractive application for these achievements is a physical implementation of a quantum computer based on spin qubits (quan- tum bit) in quantum dots. However, one of the obstacles in building such quantum computer is decoherence caused by the interaction of the electron spins with nuclear spins of the host material. In this thesis we theoretically investigate the effects caused by the hyperfine interaction in optically active semiconductor quantum dots. In Chapter 2 we assume optically induced rotations of single electron spins in semiconductor quantum dots. The optical control of the electron spin states is considered to be conducted by means of Raman type optical transitions between electron spin states. We investigate the influence of nuclear spins on the performance of the single-qubit gates by incorporating the additional effect of the Overhauser field into the electron spin dynamics. To calculate the errors caused by the hyperfine interaction, we determine average fidelities of rotations around characteristic axes in the Bloch sphere in the presence of nuclear spins analytically with perturbation theory up to second order in the Overhauser field. By applying numerical averaging over the nuclear field distribution we find the average fidelity to the arbitrary orders of the hyper- fine interaction. In Chapter 3 we investigate the dynamics of spin qubits interacting by means of an optical cavity. The qubits are represented by a single electron spin each confined to a quantum dot. Knowing that electron spins in III-V semiconduc- tor quantum dots are affected by the decoherence due to the hyperfine inter- action with nuclear spins, we find that the interaction between two qubits is consequently influenced by the Overhauser field. Assuming an unpolarizied nuclear ensemble, we investigate the fidelities for two-qubit gates depending on the Overhauser field. We include the hyperfine interaction perturbatively to second order in our analytical results, and to arbitrary precision numeri cally. Quantum dots can be used not only as physical systems for qubits, but also as sources for entangled photons. In chapter 4 we consider an emission of entangled photons by spontaneous decay of the biexciton state to the ground state. Due to electron-hole exchange interaction, the intermediate excitonic states have a finite fine structure splitting. The electron spins of the excitons also interact via hyperfine interaction with the nuclear spins. We study the temporal and fine structure splitting dependance of the coherence measures considering the effect of the nuclear magnetic field. We find that the hy perfine interaction contributes considerably to the reduction of the photon coherence. One of the possibilities to minimize the decoherence effects of the hyperfine interaction is to polarize the nuclear spins to 100%. However, up to date it was not possible to reach such degree of the nuclear polarization in experi- ments. In a recent experiment by Chekhovich et al. it was shown that high nuclear spin polarization can be achieved in self-assembled quantum dots by exploiting an optically forbidden transition between a heavy hole and a trion state. A fully polarized state in this case was predicted by a classical rate equation, but could not be obtained experimentally. Therefore we theoret- ically investigate this problem with the help of a quantum master equation in Chapter 5, and we show that a fully polarized state cannot be achieved due to formation of a nuclear dark state. Moreover, we demonstrate that the maximal degree of polarization depends on the form of the electron wave function inside of the quantum dot.
We study a large ensemble of nuclear spins interacting with a single electron spin in a quantum dot under optical excitation and photon detection. At the two-photon resonance between the two electron-spin states, the detection of light scattering from the intermediate exciton state acts as a weak quantum measurement of the effective magnetic (Overhauser) field due to the nuclear spins. In a coherent population trapping state without light scattering, the nuclear state is projected into an eigenstate of the Overhauser field operator, and electron decoherence due to nuclear spins is suppressed: We show that this limit can be approached by adapting the driving frequencies when a photon is detected. We use a Lindblad equation to describe the driven system under photon emission and detection. Numerically, we find an increase of the electron coherence time from 5 to 500 ns after a preparation time of 10 micros.
Summary form only given. Semiconductor quantum dots (QD) offer the current state-of-the-art in intensity and coherence for single photon generation, as well as serving as a testbed for various novel approaches to quantum networking. Their high brightness provides a means to produce high-bandwidth spin-photon entanglement [1]. However, the purity and usefulness of the generated entangled state is severely limited by the coherence time of the QD charge carrier spin, typically on the order of 2ns for electrons in a self-assembled InGaAs QD. This limit is imposed by low-frequency fluctuations of the Overhauser field generated by host nuclear spins, affecting the electron spin resonance frequency.Here, we measure an extension of T2 by over an order of magnitude, enabled by prior preparation of the surrounding nuclear spin bath. The interplay of dynamic nuclear polarization and coherent population trapping (CPT) can lead to a controllable mechanism that locks the nuclear spins, and thereby reduces the Overhauser field fluctuations [2,3]. We use the lambda-scheme formed by an optical transition between bound electron and negatively-charged exciton in Voigt geometry at a field of 5T. There, we use the CPT dark-state resonance as a means to lock the polarization state of the nuclear spins surrounding the electron spin. Using ultrafast optical spin rotations, we perform a Ramsey sequence following a CPT preparation of the nuclear spins, to measure the Free Induction Decay of the electron spin coherence [4]. With a pulse sequence composed of 70μs of CPT preparation, followed by 70μs of repeated Ramsey measurements, as shown in Fig. 1a, we observe coherent electron spin oscillations at a Ramsey delay of 29ns, as shown in Fig. 1b. The oscillations are free of the deleterious effects of nuclear polarization typical in such measurements [5], indicating the stabilization of the mean Overhauser field to a fixed value. The measured T2 of 39ns is over an order of magnitude longer than the Ti of 3ns measured on the system with unprepared nuclear spins, as shown in Fig. 1c.
Connecting quantum processors over long distances using photon qubits would enable more complex quantum computing architectures and quantum networks. Recently a protocol to transfer a quantum state from a photonic qubit to a singlet-triplet spin qubit in GaAs/AlGaAs heterostructure has been theoretically demonstrated. In practice, the coherent transfer is facilitated by a hybrid device where a GaAs/AlGaAs gate-defined quantum dot (GDQD) is tunnel coupled to a self-assembled quantum dot (SAQD), in which a conversion between a photon state and a spin state takes place. This work addressed the three requirements of the optical-interface devices based on tunnel coupling between the GDQD and the SAQD: (i) a properly designed GaAs/AlGaAs heterostructure where the two-dimensional electron gas (2DEG) can be electrically tuned into resonance with the InAs SAQD; (ii) high-mobility 2DEG to form and operate a GDQD; (iii) precise alignment between the SAQD and the GDQD. It is proven that the InAs SAQD can be tuned to be charged, discharged, and resonant with the 2DEG by applying a local electric field.
We analyzed the fidelity of the quantum state transfer (QST) from a photon-polarization qubit to an electron-spin-polarization qubit in a semiconductor quantum dot, with special attention to the exchange interaction between the electron and the simultaneously created hole. In order to realize a high-fidelity QST we had to separate the electron and hole as soon as possible, since the electron-hole exchange interaction modifies the orientation of the electron spin. Thus, we propose a double-dot structure to separate the electron and hole quickly, and show that the fidelity of the QST can reach as high as 0.996 if the resonant tunneling condition is satisfied.