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Towards an optical interface to spin qubits

Zeng, Zheng

Published Jan 1, 2022• 0 citations
OpenAlex

Abstract

Connecting quantum processors over long distances using photon qubits would enable more complex quantum computing architectures and quantum networks. Recently a protocol to transfer a quantum state from a photonic qubit to a singlet-triplet spin qubit in GaAs/AlGaAs heterostructure has been theoretically demonstrated. In practice, the coherent transfer is facilitated by a hybrid device where a GaAs/AlGaAs gate-defined quantum dot (GDQD) is tunnel coupled to a self-assembled quantum dot (SAQD), in which a conversion between a photon state and a spin state takes place. This work addressed the three requirements of the optical-interface devices based on tunnel coupling between the GDQD and the SAQD: (i) a properly designed GaAs/AlGaAs heterostructure where the two-dimensional electron gas (2DEG) can be electrically tuned into resonance with the InAs SAQD; (ii) high-mobility 2DEG to form and operate a GDQD; (iii) precise alignment between the SAQD and the GDQD. It is proven that the InAs SAQD can be tuned to be charged, discharged, and resonant with the 2DEG by applying a local electric field.

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Connecting quantum processors over long distances using photon qubits would enable more complex quantum computing architectures and quantum networks. Recently a protocol to transfer a quantum state from a photonic qubit to a singlet-triplet spin qubit in GaAs/AlGaAs heterostructure has been theoretically demonstrated. In practice, the coherent transfer is facilitated by a hybrid device where a GaAs/AlGaAs gate-defined quantum dot (GDQD) is tunnel coupled to a self-assembled quantum dot (SAQD), in which a conversion between a photon state and a spin state takes place. This work addressed the three requirements of the optical-interface devices based on tunnel coupling between the GDQD and the SAQD: (i) a properly designed GaAs/AlGaAs heterostructure where the two-dimensional electron gas (2DEG) can be electrically tuned into resonance with the InAs SAQD; (ii) high-mobility 2DEG to form and operate a GDQD; (iii) precise alignment between the SAQD and the GDQD. It is proven that the InAs SAQD can be tuned to be charged, discharged, and resonant with the 2DEG by applying a local electric field.
We describe an opto-electronic structure in which charge and spin degrees of freedom in electrical gate-defined quantum dots can be coherently coupled to light. This is achieved via electron-electron interaction or via electron tunneling into a proximal self-assembled quantum dot. We illustrate potential applications of this approach by considering several quantum control techniques, including optical read-out of gate-controlled semiconductor quantum bits and controlled generation of entangled photon-spin pairs.
Interconnecting well-functioning, scalable stationary qubits and photonic qubits could substantially advance quantum communication applications and serve to link future quantum processors. Here, we present two protocols for transferring the state of a photonic qubit to a single-spin and to a two-spin qubit hosted in gate-defined quantum dots (GDQD). Both protocols are based on using a localized exciton as intermediary between the photonic and the spin qubit. We use effective Hamiltonian models to describe the hybrid systems formed by the exciton and the GDQDs and apply simple but realistic noise models to analyze the viability of the proposed protocols. Using realistic parameters, we find that the protocols can be completed with a success probability ranging between 84−−9684--96\phantom{\rule{0.16em}{0ex}}%84−−96.
Self-assembled quantum dots (QDs) containing a single electron are one of the leading candidate systems for the realization of a quantum computer. The spin states of charges confined in these dots have been shown to possess a number of qualities that are attractive for use as the quantum bits (qubits) in quantum computing implementations, particularly their long lifetimes and coherence times. In addition, these spin qubits may be controlled optically, offering the prospect of ultrafast qubit gate operations, a crucial necessity for the execution of quantum algorithms. Due to the weak interaction of self-assembled QDs with light, however, the coherent optical control and read-out of the spin states of charged self-assembled QDs has proven to be a considerable challenge. This thesis presents two sets of experiments demonstrating the coherent optical control and read-out of the quantum states of a self-assembled InAs QD containing a single electron. The first utilizes mode-locked picosecond optical pulses to control the optical transitions in the dot and to detect QD level occupations. These capabilities are used to observe transient phenomena in a singly charged InAs QD such as the generation and decay of excited state population and spin precession. Further, Rabi oscillations between the electron and the lowest-lying excited state are observed, demonstrating the ability to coherently control the optical transitions of the QD, a prerequisite for spin control. These results are built upon in the second set of experiments, in which a combination of optical pulses, an externally applied DC magnetic field and a continuous-wave (CW) optical field are employed to initialize and completely control the states of a QD confined electron spin. Spin control by the use of pulse-driven two-photon Raman processes, spin precession about the external magnetic field and geometric phases generated by CW-driven cyclic evolutions in the dot is demonstrated. A number of spin qubit gate operations are shown for these spin control mechanisms, forming a foundational set of single qubit gates required for the implementation of quantum computing with singly charged self-assembled QDs.
New technologies based on the properties of quantum mechanics promise to revolutionise the way information is processed by outperforming what is possible using classical devices. Examples include massively parallel processing using quantum computers, verifiably secure communication using quantum cryptography, and measurement with sensitivity beyond classical limitation with quantum metrology. Realising the full potential of these technologies necessitates the ability to communicate quantum information over large distances, a key requirement for future quantum networks. However, developing practical implementations of long-distance quantum communication is challenging as it necessitates three major ingredients: light-matter interfaces, elementary quantum operations, and quantum memories. This thesis describes work that has been undertaken to address these requirements using semiconductor nanotechnology. We have first demonstrated that single InAs quantum dots embedded inside conventional diode structures constitute high-fidelity controllable interfaces between optical qubits and solid-state qubits. Indeed, the polarisation state of a photon was transferred into the spin state of an electron-hole pair and eventually restored through radiative recombination of the electron and the hole with a fidelity up to 95%. Moreover, spins were manipulated using subnanosecond modulation of a vertical electric field applied to the quantum dots. By controlling this electrical modulation, we demonstrated elementary phase-shift and spin-flip gate operations with near-unity fidelities. An electron-hole pair confi ned in a single quantum dot has a short radiative lifetime limiting therefore its use as an excitonic quantum memory. The solution we proposed was to use a quantum dot molecule to control the spatial separation of the electron and the hole and therefore prevent their recombination. Comprehensive studies of electric field eff ects upon the photoluminescence of quantum dot molecules lead to a clear understanding and a good control over their physical properties. Single photons were stored in individual quantum dot molecules up to 1μs and read out on a subnanosecond time scale. Moreover, the circular polarisation of individual photons was transferred into the spin state of electron-hole pairs with a fidelity above 90%, which does not degrade for storage times up to the 12.5 ns repetition period of the experiment. Our work on single quantum dots could be extended in the near future to allow for two-qubits quantum operations by con fining a second electron-hole pair to be electrically manipulated. Storage of a superposition of spin states in a quantum dot molecule should also be possible if the spin states are made degenerate, which is feasible using the electric fi eld dependence of the energy splitting between the spin states discussed in this thesis. We believe that combining both approaches will lead to the development of a controllable multi-qubit quantum memory for polarised light, a building block for long distance quantum communication based on semiconductor nanotechnology.
We analyze and give estimates for the long-distance coupling via floating metallic gates between different types of spin qubits in quantum dots made of different commonly used materials. In particular, we consider the hybrid, the singlet-triplet, and the spin-12\frac{1}{2}21​ qubits, and the pairwise coupling between each type of these qubits with another hybrid qubit in GaAs, InAs, Si, and Si0.9Ge0.1{\mathrm{Si}}_{0.9}{\mathrm{Ge}}_{0.1}Si0.9​Ge0.1​. We show that hybrid qubits can be capacitively coupled strongly enough to implement two-qubit gates, as long as the distance of the dots from the metallic gates is small enough. Thus, hybrid qubits are good candidates for scalable implementations of quantum computing in semiconducting nanostructures.