New technologies based on the properties of quantum mechanics promise to revolutionise the way information is processed by outperforming what is possible using classical devices. Examples include massively parallel processing using quantum computers, verifiably secure communication using quantum cryptography, and measurement with sensitivity beyond classical limitation with quantum metrology. Realising the full potential of these technologies necessitates the ability to communicate quantum information over large distances, a key requirement for future quantum networks. However, developing practical implementations of long-distance quantum communication is challenging as it necessitates three major ingredients: light-matter interfaces, elementary quantum operations, and quantum memories. This thesis describes work that has been undertaken to address these requirements using semiconductor nanotechnology. We have first demonstrated that single InAs quantum dots embedded inside conventional diode structures constitute high-fidelity controllable interfaces between optical qubits and solid-state qubits. Indeed, the polarisation state of a photon was transferred into the spin state of an electron-hole pair and eventually restored through radiative recombination of the electron and the hole with a fidelity up to 95%. Moreover, spins were manipulated using subnanosecond modulation of a vertical electric field applied to the quantum dots. By controlling this electrical modulation, we demonstrated elementary phase-shift and spin-flip gate operations with near-unity fidelities. An electron-hole pair confi ned in a single quantum dot has a short radiative lifetime limiting therefore its use as an excitonic quantum memory. The solution we proposed was to use a quantum dot molecule to control the spatial separation of the electron and the hole and therefore prevent their recombination. Comprehensive studies of electric field eff ects upon the photoluminescence of quantum dot molecules lead to a clear understanding and a good control over their physical properties. Single photons were stored in individual quantum dot molecules up to 1μs and read out on a subnanosecond time scale. Moreover, the circular polarisation of individual photons was transferred into the spin state of electron-hole pairs with a fidelity above 90%, which does not degrade for storage times up to the 12.5 ns repetition period of the experiment. Our work on single quantum dots could be extended in the near future to allow for two-qubits quantum operations by con fining a second electron-hole pair to be electrically manipulated. Storage of a superposition of spin states in a quantum dot molecule should also be possible if the spin states are made degenerate, which is feasible using the electric fi eld dependence of the energy splitting between the spin states discussed in this thesis. We believe that combining both approaches will lead to the development of a controllable multi-qubit quantum memory for polarised light, a building block for long distance quantum communication based on semiconductor nanotechnology.
New technologies based on the properties of quantum mechanics promise to revolutionise the way information is processed by outperforming what is possible using classical devices. Examples include massively parallel processing using quantum computers, verifiably secure communication using quantum cryptography, and measurement with sensitivity beyond classical limitation with quantum metrology. Realising the full potential of these technologies necessitates the ability to communicate quantum information over large distances, a key requirement for future quantum networks. However, developing practical implementations of long-distance quantum communication is challenging as it necessitates three major ingredients: light-matter interfaces, elementary quantum operations, and quantum memories. This thesis describes work that has been undertaken to address these requirements using semiconductor nanotechnology. We have first demonstrated that single InAs quantum dots embedded inside conventional diode structures constitute high-fidelity controllable interfaces between optical qubits and solid-state qubits. Indeed, the polarisation state of a photon was transferred into the spin state of an electron-hole pair and eventually restored through radiative recombination of the electron and the hole with a fidelity up to 95%. Moreover, spins were manipulated using subnanosecond modulation of a vertical electric field applied to the quantum dots. By controlling this electrical modulation, we demonstrated elementary phase-shift and spin-flip gate operations with near-unity fidelities. An electron-hole pair confi ned in a single quantum dot has a short radiative lifetime limiting therefore its use as an excitonic quantum memory. The solution we proposed was to use a quantum dot molecule to control the spatial separation of the electron and the hole and therefore prevent their recombination. Comprehensive studies of electric field eff ects upon the photoluminescence of quantum dot molecules lead to a clear understanding and a good control over their physical properties. Single photons were stored in individual quantum dot molecules up to 1μs and read out on a subnanosecond time scale. Moreover, the circular polarisation of individual photons was transferred into the spin state of electron-hole pairs with a fidelity above 90%, which does not degrade for storage times up to the 12.5 ns repetition period of the experiment. Our work on single quantum dots could be extended in the near future to allow for two-qubits quantum operations by con fining a second electron-hole pair to be electrically manipulated. Storage of a superposition of spin states in a quantum dot molecule should also be possible if the spin states are made degenerate, which is feasible using the electric fi eld dependence of the energy splitting between the spin states discussed in this thesis. We believe that combining both approaches will lead to the development of a controllable multi-qubit quantum memory for polarised light, a building block for long distance quantum communication based on semiconductor nanotechnology.
We report on a single photon and spin storage device based on a semiconductor quantum dot molecule. Optically excited single electron-hole pairs are trapped within the molecule, and their recombination rate is electrically controlled over 3 orders of magnitude. Single photons are stored up to 1 μs and read out on a subnanosecond time scale. By using resonant excitation, the circular polarization of individual photons is transferred into the spin state of electron-hole pairs with a fidelity above 80%, which does not degrade for storage times up to the 12.5 ns repetition period of the experiment.
We demonstrate high-fidelity reversible transfer of quantum information from the polarization of photons into the spin state of an electron-hole pair in a semiconductor quantum dot. Moreover, spins are electrically manipulated on a subnanosecond time scale, allowing us to coherently control their evolution. By varying the area of the electrical pulse, we demonstrate phase-shift and spin-flip gate operations with near-unity fidelities. Our system constitutes a controllable quantum interface between flying and stationary qubits, an enabling technology for quantum logic in the solid state.
A fascinating dream in quantum information science is to build quantum computers with super-performance and quantum networks with unconditional security [1]. Quantum networks utilize static (matter) quantum bits (qubits) to store and process quantum information at local nodes, and photons as flying qubits for long-distance quantum state transmission between different nodes. To realize a quantum network, it is crucial to achieve light-matter entanglement and reversible quantum-state transfer between light and matter, i.e., the light-matter quantum interface, and the quantum repeater for large-scale quantum communications [2]. Recent experiments have shown that both electrons and holes confined in semiconductor quantum dots (QDs) have long spin relaxation time (T1e, T1h ~ ms) and long spin coherence time (T2e ~ microseconds, T2h > 100 ns). Moreover, fast spin cooling and ultra-fast spin manipulation as well as spin echoes to preserve the spin coherence have also been demonstrated. Undoubtedly these rapid progresses imply that the QD spin is a good candidate for matter qubit in quantum information processing. Furthermore, QD-based single photon sources have been also developed. Therefore, semiconductor QDs offer a good platform for solid-state quantum networking and quantum computation. Here we present two types of conditional quantum gates, i.e., the photon-spin entangling gates [3-4] using a single QD spin in a single-sided or double-sided optical microcavity. Both gates are universal and deterministic (if they are optimized). The spin-selective coherent photon-spin interaction enhanced by the cavity QED lead to giant circular birefringence, which allows us to build these gates. We will show the versatile spin-cavity systems can be applied in all aspects of quantum information science and technology, not only for large-scale quantum communication networks (solid-state quantum repeaters) [5], but also for scalable quantum computing with either photons or spins as qubits. We will also discuss other applications using these gates, such as photon-number resolving detection, quantum feed-back control, loss-resistant quantum metrology, and loophole-free Bell test [6], and other devices based on optical nonlinearity at single-photon levels in these gate structures. All these schemes are feasible with current semiconductor technology [7], and we have recently seen conditional phase shifts in uncharged QD-cavity systems [8]. References [1] H.J. Kimble, Nature (London) 453, 1023 (2008). [2] H.-J. Briegel et al., Phys. Rev. Lett. 81, 5932 (1998). [3] C.Y. Hu et al., Phys. Rev. B 78, 085307 (2008); ibid. 78, 125318 (2008). [4] C.Y. Hu et al., Phys. Rev. B 80, 205326 (2009). [5] C.Y. Hu and J.G. Rarity, Phys. Rev. B 83, 115303 (2011). [6] N. Brunner et al., Arxiv: quant-phys 1303.6522 (2013). [7] S. Reitzenstein et al., Appl. Phys. Lett. 90, 251109 (2007). [8] A.B. Young et al., Phys. Rev. A 84, 011803 (2011).
Single spins in semiconductor quantum dots form a promising platform for solid-state quantum information processing. The spin-up and spin-down states of a single electron or hole, trapped inside a quantum dot, can represent a single qubit with a reasonably long decoherence time. The spin qubit can be optically coupled to excited (charged exciton) states that are also trapped in the quantum dot, which provides a mechanism to quickly initialize, manipulate and measure the spin state with optical pulses, and to interface between a stationary matter qubit and a 'flying' photonic qubit for quantum communication and distributed quantum information processing. The interaction of the spin qubit with light may be enhanced by placing the quantum dot inside a monolithic microcavity. An entire system, consisting of a two-dimensional array of quantum dots and a planar microcavity, may plausibly be constructed by modern semiconductor nano-fabrication technology and could offer a path toward chip-sized scalable quantum repeaters and quantum computers. This article reviews the recent experimental developments in optical control of single quantum dot spins for quantum information processing. We highlight demonstrations of a complete set of all-optical single-qubit operations on a single quantum dot spin: initialization, an arbitrary SU(2) gate, and measurement. We review the decoherence and dephasing mechanisms due to hyperfine interaction with the nuclear-spin bath, and show how the single-qubit operations can be combined to perform spin echo sequences that extend the qubit decoherence from a few nanoseconds to several microseconds, more than 5 orders of magnitude longer than the single-qubit gate time. Two-qubit coupling is discussed, both within a single chip by means of exchange coupling of nearby spins and optically induced geometric phases, as well as over longer-distances. Long-distance spin-spin entanglement can be generated if each spin can emit a photon that is entangled with the spin, and these photons are then interfered. We review recent work demonstrating entanglement between a stationary spin qubit and a flying photonic qubit. These experiments utilize the polarization- and frequency-dependent spontaneous emission from the lowest charged exciton state to single spin Zeeman sublevels.
InAs quantum dots (QDs) can be used as optically coupled quantum storage devices for quantum information applications. The QD can be charged with a single electron, where the spin state (up or down) provides a long lived quantum bit (qubit). The QD's optically excited states are used to initialize, manipulate, and read out the electron spin state with laser pulses. However, most practical quantum information applications require many interacting qubits, forming a quantum network. Since QDs are based on semiconductor technology, and are compatible with standard nano-fabrication processing, there is promise that they can provide a solid state platform where a scalable quantum information architecture is realizable. We focus on scaling the QD system to multiple qubits using intermediate spin-photon entangled states. In this work, experimental and theoretical techniques are developed to study the QD-light matter interaction at the single photon level. Resonance fluorescence from a single QD is experimentally realized, and the single photon nature of the scattered radiation is verified through intensity correlation experiments. Transient fluorescence measurements on resonantly excited QDs are performed using time correlated single photon counting techniques to measure the excited state lifetime. High speed electro-optic modulators are used to time gate narrow bandwidth lasers, so that a QD can be driven under step-wise excitation, allowing for the direct observation of time-dependent optical Rabi oscillations. From these measurements, we are able to extract a decoherence rate which is consistent with the lifetime limit, indicating that pure dephasing is negligible in this system. These techniques are applied to the QD spin system to demonstrate a spin-photon entangled state, by performing correlation measurements on the spin and photon state in two bases. A lower bound on the entanglement fidelity of 0.59(4) is achieved, which exceeds the classical limit of 0.5 by more than two standard deviations. The entanglement fidelity is limited primarily by the finite timing resolution of available single photon detectors. Taking this into account, we achieve 84% of the apparatus limited fidelity. These spin-entangled photons can be used to mediate entanglement between distant QD spins, providing the basis of an optically coupled QD spin network.
We present an exciton-spin memory scheme using a single QDM consisting of two InAs QDs separated by a thin GaAs tunnelling barrier. Electrical control of the electron-hole spatial separation allowed the exciton lifetime to be tuned in the 1-1000 ns range. Storage and read-out operations were implemented using sub nanosecond modulation of the lifetime and photon storage up to 1μs was demonstrated. Using resonant excitation the circular polarisation of photons was transferred and stored in the exciton Zeeman states of a QDM under a magnetic field. The delayed emission was clearly co-polarised with the excitation light and a combined fidelity of 80% for the write and read operations was achieved.