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arXiv:cond-mat/0406129 · Physical Review Letters

Observation of Feshbach Resonances between Two Different Atomic Species

Claudiu A. Stan, Martin W. Zwierlein, Christian H. Schunck, S. M. F. Raupach, Wolfgang Ketterle

Published Sep 30, 2004• 270 citations
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Abstract

We have observed three Feshbach resonances in collisions between $^{6}\mathrm{L}\mathrm{i}$ and $^{23}\mathrm{N}\mathrm{a}$ atoms. The resonances were identified as narrow loss features when the magnetic field was varied. The molecular states causing these resonances have been identified, and additional $^{6}\mathrm{L}\mathrm{i}\mathrm{\text{\ensuremath{-}}}^{23}\mathrm{N}\mathrm{a}$ resonances are predicted. These resonances will allow the study of degenerate Bose-Fermi mixtures with adjustable interactions and could be used to generate ultracold heteronuclear molecules.

DOI
10.1103/physrevlett.93.143001

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We have observed three Feshbach resonances in collisions between 6Li^{6}\mathrm{L}\mathrm{i}6Li and 23Na^{23}\mathrm{N}\mathrm{a}23Na atoms. The resonances were identified as narrow loss features when the magnetic field was varied. The molecular states causing these resonances have been identified, and additional 6Li\ensuremath-23Na^{6}\mathrm{L}\mathrm{i}\mathrm{\text{\ensuremath{-}}}^{23}\mathrm{N}\mathrm{a}6Li\ensuremath-23Na resonances are predicted. These resonances will allow the study of degenerate Bose-Fermi mixtures with adjustable interactions and could be used to generate ultracold heteronuclear molecules.
Three magnetic-field induced heteronuclear Feshbach resonances were identified in collisions between bosonic 87Rb^{87}\mathrm{R}\mathrm{b}87Rb and fermionic 40K^{40}\mathrm{K}40K atoms in their absolute ground states. Strong inelastic loss from an optically trapped mixture was observed at the resonance positions of 492, 512, and $543\ifmmode\pm\else\textpm\fi{}2\text{ }\text{ }\mathrm{G}$. The magnetic-field locations of these resonances place a tight constraint on the triplet and singlet cross-species scattering lengths, yielding $(\ensuremath{-}281\ifmmode\pm\else\textpm\fi{}15){a}_{0}$ and $(\ensuremath{-}54\ifmmode\pm\else\textpm\fi{}12){a}_{0}$, respectively. The width of the loss feature at 543 G is $3.7\ifmmode\pm\else\textpm\fi{}1.5\text{ }\text{ }\mathrm{G}$ wide; this broad Feshbach resonance should enable experimental control of the interspecies interactions.
We report on the observation of two Feshbach resonances in collisions between ultracold 6Li^{6}\mathrm{Li}6Li and 87Rb^{87}\mathrm{Rb}87Rb atoms in their respective hyperfine ground states $\ensuremath{\mid}F,{m}_{F}⟩=\ensuremath{\mid}1∕2,1∕2⟩$ and \ensuremath{\mid}1,1⟩. The resonances show up as trap losses for the 6Li^{6}\mathrm{Li}6Li cloud induced by inelastic Li-Rb-Rb three-body collisions. The magnetic field values where they occur represent important benchmarks for an accurate determination of the interspecies interaction potentials. A broad Feshbach resonance located at 1066.92G1066.92\phantom{\rule{0.3em}{0ex}}\mathrm{G}1066.92G opens interesting prospects for the creation of ultracold heteronuclear molecules. We furthermore observe a strong enhancement of the narrow ppp-wave Feshbach resonance in collisions of 6Li^{6}\mathrm{Li}6Li atoms at 158.55G158.55\phantom{\rule{0.3em}{0ex}}\mathrm{G}158.55G in the presence of a dense 87Rb^{87}\mathrm{Rb}87Rb cloud. The effect of the 87Rb^{87}\mathrm{Rb}87Rb cloud is to introduce Li-Li-Rb three-body collisions occurring at a higher rate than Li-Li-Li collisions.
We report on the observation of five Feshbach resonances in collisions between ultracold 7Li^{7}\mathrm{Li}7Li and 87Rb^{87}\mathrm{Rb}87Rb atoms in the absolute ground-state mixture where both species are in their $\ensuremath{\mid}f,{m}_{f}⟩=\ensuremath{\mid}1,1⟩$ hyperfine states. The resonances appear as trap losses for the 7Li^{7}\mathrm{Li}7Li cloud induced by inelastic heteronuclear three-body collisions. The magnetic field values where they occur are important quantities for an accurate determination of the interspecies interaction potentials. Results of coupled channels calculations based on the observed resonances are presented and refined potential parameters are given. A very broad Feshbach resonance centered around 649G649\phantom{\rule{0.3em}{0ex}}\mathrm{G}649G should allow for fine-tuning of the interaction strength in future experiments.
We have observed 28 heteronuclear Feshbach resonances in ten spin combinations of the hyperfine ground states of a $^{40}\mathrm{K}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ mixture. The measurements were performed by observing the loss rates from an atomic mixture at magnetic fields between 000 and 700G700\phantom{\rule{0.3em}{0ex}}\mathrm{G}700G. These data were used to significantly refine an interatomic potential derived from molecular spectroscopy, yielding a highly consistent model of the $^{40}\mathrm{K}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ interaction. Thus, the measured resonances can be assigned to the corresponding molecular states. In addition, this potential allows for an accurate calculation of the energy differences between highly excited levels and the rovibrational ground level. This information is of particular relevance for the formation of deeply bound heteronuclear molecules. Finally, the model is used to predict Feshbach resonances in mixtures of 87Rb^{87}\mathrm{Rb}87Rb combined with 39K^{39}\mathrm{K}39K or 41K^{41}\mathrm{K}41K.
We have successfully prepared an optically trapped ultracold mixture of 23{}^{23}23Na and 87{}^{87}87Rb atoms and studied their interspecies Feshbach resonances. Using two different spin combinations, several sss- and ppp-wave resonances are identified by observing high inelastic losses and temperature increases for both species near resonant magnetic field values. The two sss-wave resonances observed below 500 G between atoms in their lowest-energy levels are possible candidates for Feshbach molecule association. Our results are well characterized by a coupled-channel model which also refines the ground-state interaction potentials between 23{}^{23}23Na and 87{}^{87}87Rb. This work opens up the prospect for preparing ultracold ensembles of ground-state bosonic NaRb molecules which are chemically stable and can provide strong dipolar interactions.
K) molecules in the rovibrational ground state. We prepare the atoms and molecules in various hyperfine levels of their ground states and observe the loss of molecules as a function of the magnetic field. The atom-molecule Feshbach resonances are identified by observing an enhancement of the loss. We have observed 11 resonances in the magnetic field range of 43 to 120 gauss. The observed atom-molecule Feshbach resonances at ultralow temperatures probe the three-body potential energy surface with exceptional resolution and will help to improve understanding of ultracold collisions.