We study local and nonlocal correlations of light transmitted through active random media. The conventional approach results in divergence of ensemble-averaged correlation functions due to the existence of lasing realizations. We introduce a conditional average for correlation functions by omitting the divergent realizations. Our numerical simulation reveals that amplification does not affect local spatial correlation. The nonlocal intensity correlations are strongly magnified due to selective enhancement of the contributions from long propagation paths. We also show that by increasing gain, the average mode linewidth can be made comparable to the average mode spacing. This implies that light transport through a diffusive random system with gain may exhibit some similarities with that through a localized passive system.
We study local and nonlocal correlations of light transmitted through active random media. The conventional approach results in divergence of ensemble-averaged correlation functions due to the existence of lasing realizations. We introduce a conditional average for correlation functions by omitting the divergent realizations. Our numerical simulation reveals that amplification does not affect local spatial correlation. The nonlocal intensity correlations are strongly magnified due to selective enhancement of the contributions from long propagation paths. We also show that by increasing gain, the average mode linewidth can be made comparable to the average mode spacing. This implies that light transport through a diffusive random system with gain may exhibit some similarities with that through a localized passive system.
The model based on the method of finite-difference time-domain is applied to calculate the general feature of localized modes in active random media. The evolution of the localized modes from passive random media to active ones is investigated. By varying the gain lineshape for an active random medium, we have observed a selective excitation of localized modes, including both single-mode and multi-mode excitations. When the eigenfrequencies for some localized modes are near the centre of the gain spectrum, the optical gain offers coherent amplification to them so that they can obtain more amplification and have stronger field amplitude than other modes. The pumping level dependence of the field amplitude of the localized modes exhibits a threshold behaviour.
In the last decade Anderson Localization of Light and Random Lasing has attracted a variety of interest in the community of condensed matter theory. The fact that a system so inartificial as a thin layer consisting of dust particles, which have amplifying properties, can produce coherent laser emission, is of a simple elegance, which promises new insights in fundamental physics. There is no need of an external feedback mechanism, like in the system of a conventional laser. Whereas several attempts try to enter the subject numerically by considering cavity approximations, this thesis is concerned with building a microscopically self-consistent theory of random lasing. Designing this method, we had to study light localization effects in random media including absorption and gain. Incorporating interference effects by means of Cooperon contributions we derived Anderson localized states for passive media. Mapping this on a system which consists of laser active Mie-scatterers in a passive medium, we found that by incorporation of the Cooperon, we loose the Anderson localization, but the system is weakly localized, which is sufficient for population inversion and stimulated emission.
Light propagation in matter is described by vibration eigenstates, called modes, which characterize the light-matter interaction. In the specific case of random media, according to the strength of the disorder, the modes can be either extended over the whole system or spatially localized. This disorder-based confinement is called Anderson’s localization.In the first part, we introduce basic notions used along this manuscript. In particular the light-matter interaction requires a semiclassical approach: The electromagnetic field is described by Maxwell’s equations while the quantum nature of matter must be considered. In this thesis open media are studied. In such systems the modal description requires a specific analytic treatment different from closed problems. In the second part, we focus on Anderson-localized modes in open passive random media. Any change of the disorder induces modifications of modes. Therefore, it enables the control over the light properties. Moreover, when inserting an emitter inside an Anderson-localized mode, strong light-matter interaction regimes can be reached. In the third part, active random media, commonly called random lasers, are introduced. Using our experimental achievements, characteristics of random lasers are presented. The notion of mode enables us to describe complex mechanisms involved in the lasing emission. Last, we demonstrate both experimentally and numerically that a non-uniform excitation of random lasers can lead to a control of the properties of the emission. In particular a multimode spectrum for a uniform pumping can be turned into single-mode using an adapted pumping.
We study the dynamics of lasing from photonic paints excited by short, localized, optical pulses, using a time-dependent diffusion model for light propagating in the medium containing active atoms. The full time-dependent, nonadiabatic nonlinear response of the atomic system to the local optical field intensity is described using the Einstein rate equations for absorption and emission of light. Solving the time-dependent diffusion equation for the light intensity in the medium with nonlinear gain and loss, we derive detailed information on the spectral, spatial, and temporal properties of the emitted laser light. Our model recaptures the effects of scatterers to narrow the emission spectral linewidth and to narrow the emitted pulse duration, at a specific threshold pump intensity. Our model also describes how this threshold pump intensity decreases with scatterer density and excitation spot diameter, in excellent agreement with experimental results.
Amplification in random media is investigated from the perspective of diffuse photon density waves (DPDWs). These exponentially decaying waves, typical in absorbing media, exhibit significantly enhanced propagation characteristics in random amplifying media. Consequently, finite amplifying regions, embedded in an absorbing random medium, exhibit specific resonant features governed by the geometry of the amplifying region. For a spheroidal amplifying region, the scattered waves are dominated by the characteristic multipolar resonances, and the monopolar as well as the dipolar resonances are closely related to random lasing thresholds. The levels of amplification at which the resonance (or lasing) occurs can be used to identify the size, shape, and orientation of the amplifying region. These resonant modes are quite robust and survive, even as the modulation frequency of the DPDW is varied from about 100 MHz to zero, thereby indicating a deeper connection between random lasing path distributions and the appropriate gain profiles resulting in the associated intensity distribution of the DPDW modes.