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arXiv:cond-mat/0404021 · Physical Review B

Nonequilibrium transfer and decoherence in quantum impurity problems

Holger Baur, Andrea Fubini, Ulrich Weiß

Published Jul 21, 2004• 9 citations
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Abstract

Using detailed balance and scaling properties of integrals that appear in the Coulomb gas reformulation of quantum impurity problems, we establish exact relations between the nonequilibrium transfer rates of the boundary sine-Gordon and the anisotropic Kondo model at zero temperature. Combining these results with findings from the thermodynamic Bethe ansatz, we derive exact closed form expressions for the transfer rate in the biased spin-boson model in the scaling limit. They illustrate how the crossover from weak to strong tunneling takes place. Using a conjectured correspondence between the transfer and the decoherence rate, we also determine the exact lower bound for damping of the coherent oscillation as a function of bias and dissipation strength in this paradigmic model for nuclear magnetic resonance and superposition of macroscopically distinct states (qubits).

DOI
10.1103/physrevb.70.024302

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Using detailed balance and scaling properties of integrals that appear in the Coulomb gas reformulation of quantum impurity problems, we establish exact relations between the nonequilibrium transfer rates of the boundary sine-Gordon and the anisotropic Kondo model at zero temperature. Combining these results with findings from the thermodynamic Bethe ansatz, we derive exact closed form expressions for the transfer rate in the biased spin-boson model in the scaling limit. They illustrate how the crossover from weak to strong tunneling takes place. Using a conjectured correspondence between the transfer and the decoherence rate, we also determine the exact lower bound for damping of the coherent oscillation as a function of bias and dissipation strength in this paradigmic model for nuclear magnetic resonance and superposition of macroscopically distinct states (qubits).
Using detailed balance and scaling properties of integrals that appear in the Coulomb gas reformulation of quantum impurity problems, we establish exact relations between the nonequilibrium quantum decay rates of the boundary sine-Gordon and the anisotropic Kondo model at zero temperature. Combining these results with findings from the thermodynamic Bethe ansatz, we derive exact closed form expressions for the quantum decay rate of the dissipative two-state system in the scaling limit. These expressions illustrate how the crossover from weak to strong tunneling takes place. We trace out the regimes in which the usually applied Golden Rule (nonadiabatic) rate expression fails. Using a conjectured correspondence between the relaxation and dephasing rate, we obtain the exact lower bound of the dephasing rate as a function of bias and dissipation strength.
We study the transfer of heat in the nonequilibrium spin-boson model with an Ohmic dissipation. In the nonadiabatic limit we derive a formula for the thermal conductance based on a rate equation formalism at the level of the noninteracting blip approximation, valid for temperatures T>T(K), with T(K) as the Kondo temperature. We evaluate this expression analytically assuming either weak or strong couplings, and demonstrate that our results agree with exact relations. Far-from-equilibrium situations are further examined, showing a close correspondence to the linear response limit.
Based on the recent paper [Phys. Rev. Lett. 102, 216803 (2009)], we study the nonequilibrium occupation number nd{n}_{d}nd​ and charge susceptibility $\ensuremath{\chi}$ of a resonance level close to dissipative quantum phase transition of the Kosterlitz-Thouless (KT) type between a delocalized phase for weak dissipation and a localized phase for strong dissipation. The resonance level is coupled to two spinless fermionic baths with a finite bias voltage and an Ohmic bosonic bath representing the dissipative environment. The system is equivalent to an effective anisotropic Kondo model out of equilibrium. Within the nonequilibrium renormalization-group approach, we calculate nonequilibrium magnetization MMM and spin susceptibility $\ensuremath{\chi}$ in the effective Kondo model, corresponding to $2{n}_{d}\ensuremath{-}1$ and $\ensuremath{\chi}$ of a resonance level, respectively. We demonstrate the smearing of the KT transition in the nonequilibrium magnetization MMM as a function of the effective anisotropic Kondo couplings, in contrast to a perfect jump in MMM at the transition in equilibrium. In the limit of large bias voltages, we find MMM and $\ensuremath{\chi}$ at the KT transition and in the localized phase show deviations from the equilibrium Curie-law behavior. As the system gets deeper in the localized phase, both ${n}_{d}\ensuremath{-}1/2$ and $\ensuremath{\chi}$ decrease more rapidly to zero with increasing bias voltages.
We develop a unified theoretical framework for the anisotropic Kondo model and the boundary sine-Gordon model. They are both boundary integrable quantum field theories with a quantum-group spin at the boundary which takes values, respectively, in standard or cyclic representations of the quantum groupSU(2) q. This unification is powerful, and allows us to find new results for both models. For the anisotropic Kondo problem, we find exact expressions (in the presence of a magnetic field) for all the coefficients in the Anderson-Yuval perturbative expansion. Our expressions hold initially in the very anisotropic regime, but we show how to continue them beyond the Toulouse point all the way to the isotropic point using an analog of dimensional regularization. The analytic structure is transparent, involving only simple poles which we determine exactly, together with their residues. For the boundary sine-Gordon model, which describes an impurity in a Luttinger liquid, we find the nonequilibrium conductance for all values of the Luttinger coupling. This is an intricate computation because the voltage operator and the boundary scattering do not commute with each other.
We study the nonequilibrium transport properties of fully (exactly) screened Kondo quantum dots subject to a finite bias voltage or a finite temperature. First, we calculate the Fermi-liquid coefficients of the conductance for models with arbitrary spin, i.e., its leading behavior for small bias voltages or temperatures. Second, we determine the low-temperature behavior of the static susceptibility from the exactly known Bethe ansatz results for the magnetization. Third, we study the crossover from strong to weak coupling in the spin-1/2 and the spin-1 models coupled to one or two screening channels, respectively. Using a real-time renormalization group method we calculate the static and dynamical spin-spin correlation functions for the spin-1/2 model as well as the linear and differential conductance and the static susceptibility for the spin-1 model. We define various Kondo scales and discuss their relations. We assess the validity of the renormalization-group treatment by comparing with known results for the temperature dependence of the linear conductance and static susceptibility as well as the Fermi-liquid behavior at low energies.
The dynamical decoherence rate and charge susceptibility of a nonequilibrium quantum dot close to a dissipative quantum phase transition are calculated. The setup concerns a resonance-level quantum dot coupled to two spinless fermionic baths with a finite bias voltage and an ohmic bosonic bath representing a dissipative environment. The system is equivalent to an anisotropic Kondo model. As dissipation strength increases, the system at zero temperature and zero bias exhibits a quantum phase transition of the Kosterlitz-Thouless (KT) type between a conducting delocalized phase and an insulating localized phase. Within the nonequilibrium frequency-dependent renormalization group (RG) approach, the finite bias crossover in dynamical decoherence rate and charge susceptibility close to the transition are addressed. The dynamical decoherence rate is found to increase with increasing frequency. In the delocalized phase, it shows a singularity at frequencies equal to positive or negative bias voltage. As the system cross overs to the localized phase, the decoherence rate at low frequencies gets progressively smaller and the singular feature is gradually smeared out, leading to a single linear frequency dependence. The dynamical charge susceptibility at low frequencies shows a dip-to-peak crossover across the transition. Relevance of these results to the experiments is discussed.