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arXiv:cond-mat/0403553 · Physical Review Letters

Correlations in Atomic Systems: Diagnosing Coherent Superpositions

Radka Bach, Kazimierz Rza̧żewski

Published May 17, 2004• 38 citations
arXivHTMLPDF

Abstract

While investigating quantum correlations in atomic systems, we note that single measurements contain information about these correlations. Using a simple model of measurement-analogous to the one used in quantum optics-we show how to extract higher-order correlation functions from individual "photographs" of the atomic sample. As a possible application, we apply the method to detect a subtle phase coherence in mesoscopic superpositions.

DOI
10.1103/physrevlett.92.200401

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While investigating quantum correlations in atomic systems, we note that single measurements contain information about these correlations. Using a simple model of measurement-analogous to the one used in quantum optics-we show how to extract higher-order correlation functions from individual "photographs" of the atomic sample. As a possible application, we apply the method to detect a subtle phase coherence in mesoscopic superpositions.
This thesis fathoms the possibilities and limitations of measurements in quantum optics. After a short introduction to the general aspects of measurements in quantum mechanics, it presents three examples of a measurement process in concrete applications to quantum optics. For one, while operators describing quantities of interest might have a simple theoretical form, it is often hard to actually implement a measurement of their expectation values experimentally. This situation is encountered in the first part which is devoted to the measurement of quantum statistical properties of a light beam. In contrast to classical optics, these statistics are not fully determined by first- and second-order correlations. Instead, higher-order correlations, usually described by non-Hermitian operators, are necessary to characterize the quantum state completely. A particular example is the N-photon Fock state, for which only a measurement of the Nth-order correlations allows for a full characterization. Here, we present a new method how to measure an important class of Nth-order correlations for arbitrary N in a single spatial mode with two polarizations with limited experimental resources. The second part is again centered around the realization of specific measurement operators for photon correlation measurements. However, in contrast to the previous chapter, these measurements are not an end in their own, but are designed to create specific quantum states as a consequence of the measurement process: A suitable measurement of photons emitted by a number of atoms allows to transfer the atoms into long-lived entangled states. We find that with this method it is possible to entangle two remote atomic qubits to an arbitrary and well-defined degree. Furthermore, we show how to generate two families of quantum states in an arbitrary number of remote atomic qubits: one family consists of all -- symmetric and non-symmetric -- total angular momentum eigenstates in N remote qubits, the other is a family of cluster states. It is also systematically investigated whether the technique of quantum state engineering by projective measurements allows for the creation of any arbitrary state. We find explicit solutions for the case of two and three qubits, while it is shown that no solution exist for N > 6. We conclude the section by proving that with some changes in the setup, this measurement-based quantum state engineering technique allows to create the same states among the scattered photons themselves rather than among the emitting atoms. The last part is devoted to the amount of information one is able to gain about a given system when performing a measurement. The corresponding limits of information are investigated at the example of the duality that arises in a two-way interferometer between the visibility of the interference pattern and the knowledge about the path of the interfering object. We show that there exist correlations between the phase difference the interfering object acquires on its way through the interferometer and the amount of which-way information retrievable from certain observables of the which-way detector. In this way, the which-way information becomes a phase-dependent quantity. In particular, we find that for certain values of the phase shift, the amount of extractable which-way information can be larger than allowed by phase-independent measurement. This property is put to use to find the optimal observable for the which-way detector readout in dependence on the phase of the interfering object. Following this strategy, we are able to gain more which-way information than previously thought possible.
Quantum correlations are correlations that arise from a unique feature in quantum mechanics: quantum superposition. The most famous example of quantum superposition is the Schrodinger’s cat state, where a cat is in a state of neither dead nor alive before an observer determines the cat’s status. This is not what we expect. Nevertheless, quantum superposition and correlations are routinely created in the laboratories with microscopic systems involving atoms and light particles. Can this counterintuitive notion be realised in the macroscopic world? This thesis investigates this question by devising criteria that certify the existence of quantum correlations in mesoscopic/macroscopic systems. Powerful mathematical tools are used to simulate two quantum protocols in a mesoscopic system which have applications in quantum communication and computation.
The concept of coherence which has conventionally been used in optics is found to be inadequate to the needs of recently opened areas of experiment. To provide a fuller discussion of coherence, a succession of correlation functions for the complex field strengths is defined. The nthn\mathrm{th}nth order function expresses the correlation of values of the fields at 2n2n2n different points of space and time. Certain values of these functions are measurable by means of nnn-fold delayed coincidence detection of photons. A fully coherent field is defined as one whose correlation functions satisfy an infinite succession of stated conditions. Various orders of incomplete coherence are distinguished, according to the number of coherence conditions actually satisfied. It is noted that the fields historically described as coherent in optics have only first-order coherence. On the other hand, the existence, in principle, of fields coherent to all orders is shown both in quantum theory and classical theory. The methods used in these discussions apply to fields of arbitrary time dependence. It is shown, as a result, that coherence does not require monochromaticity. Coherent fields can be generated with arbitrary spectra.
The concept of coherence which has conventionally been used in optics is found to be inadequate to the needs of recently opened areas of experiment. To provide a fuller discussion of coherence, a succession of correlation functions for the complex field strengths is defined. The nthn\mathrm{th}nth order function expresses the correlation of values of the fields at 2n2n2n different points of space and time. Certain values of these functions are measurable by means of nnn-fold delayed coincidence detection of photons. A fully coherent field is defined as one whose correlation functions satisfy an infinite succession of stated conditions. Various orders of incomplete coherence are distinguished, according to the number of coherence conditions actually satisfied. It is noted that the fields historically described as coherent in optics have only first-order coherence. On the other hand, the existence, in principle, of fields coherent to all orders is shown both in quantum theory and classical theory. The methods used in these discussions apply to fields of arbitrary time dependence. It is shown, as a result, that coherence does not require monochromaticity. Coherent fields can be generated with arbitrary spectra.