We present a full theoretical and experimental study of the dynamics and energy distribution of nonequilibrium quasiparticles in superconducting tunnel junctions (STJ's). STJ's are often used for single-photon spectrometers, where the numbers of quasiparticles excited by a photon provide a measure of the photon energy. The magnitude and fluctuations of the signal current in STJ detectors are in large part determined by the quasiparticle dynamics and energy distribution during the detection process. We use this as motivation to study the transport and energy distribution of nonequilibrium quasiparticles excited by x-ray photons in a lateral, imaging junction configuration. We present a full numerical model for the tunneling current of the major physical processes which determine the signal. We find that a diffusion framework models the quasiparticle dynamics well and that excited quasiparticles do not equilibrate to the lattice temperature during the time scales for tunneling. We extract physical time scales from the measured data, make comparisons with existing theories, and comment on implications for superconducting mesoscopic systems and single-photon detectors.
We present a full theoretical and experimental study of the dynamics and energy distribution of nonequilibrium quasiparticles in superconducting tunnel junctions (STJ's). STJ's are often used for single-photon spectrometers, where the numbers of quasiparticles excited by a photon provide a measure of the photon energy. The magnitude and fluctuations of the signal current in STJ detectors are in large part determined by the quasiparticle dynamics and energy distribution during the detection process. We use this as motivation to study the transport and energy distribution of nonequilibrium quasiparticles excited by x-ray photons in a lateral, imaging junction configuration. We present a full numerical model for the tunneling current of the major physical processes which determine the signal. We find that a diffusion framework models the quasiparticle dynamics well and that excited quasiparticles do not equilibrate to the lattice temperature during the time scales for tunneling. We extract physical time scales from the measured data, make comparisons with existing theories, and comment on implications for superconducting mesoscopic systems and single-photon detectors.
The latest generation of high quality, narrow gap, superconducting tunnel junctions (STJs) exhibits a steady-state and time-dependent behavior which cannot be described satisfactorily by previous treatments of nonequilibrium quasiparticle (qp) dynamics. These effects are particularly evident in experiments using STJs as detectors of photons, over the range from near infrared to x ray. In this paper, we present a detailed theoretical analysis of the spectral and temporal evolution of the nonequilibrium qp and phonon distributions in such STJs excited by single photons, over a wide range of excitation energy, bias voltage, and temperature. By solving the coupled set of kinetic equations describing the interacting excitations, we show that the nonequilibrium qp distribution created by the initial photoabsorption does not decay directly back to the initial undisturbed state in thermal equilibrium. Instead, it undergoes a rapid adiabatic relaxation to a long-lived, excited state, the spectral distribution of which is nonthermal, maintained by a balance between qp creation, recombination, and trapping. The model is able to describe successfully photoabsorption data taken on several different aluminum STJs, using a single set of parameters. Of particular note is the conclusion that the local traps responsible for qp loss are situated specifically in the region of Nb contacts.
Superconducting materials are useful for a wide range of applications, ranging from particle detectors to quantum computing. The presence of excitations (quasiparticles) in the superconductor can be a resource in some devices and a disturbance in others - in kinetic inductance detectors, the generation of quasiparticles by an incoming photon can be read out and used to calculate the energy of the photon, while the tunnelling of quasiparticles is a cause of decoherence in quantum computing. While early research mostly focused on superconductors close to the critical temperature, temperatures that are far below the critical temperatures are often used for current applications. At these low temperatures, the energy exchange between quasiparticles and phonons becomes slow, and even small disturbances may drive the energy distribution of the quasiparticles out of thermal equilibrium. In fact, experiments usually show a residual number of quasiparticles even at milikelvin temperatures, for which the thermal density of quasiparticles would be negligible. This thesis consists of two parts: In the first part, I model the energy distribution of quasiparticles in superconducting resonators: Quasiparticles absorb energy by absorbing photons and release it as phonons, which drives the superconductor out of thermal equilibrium. I solve a set of rate equations, both numerical and analytical, to calculate the energy distribution of the quasiparticles. For parameters typically used in kinetic inductance detectors made of aluminum, the microwave signal used to read out the resonator dominates the energy distribution of the quasiparticles, while their density is determined by other processes. At not too low temperatures, quasiparticles are mainly produced by thermal phonons, and my calculations reproduce recently measured quality factors of resonators at temperatures above 250 mK without free parameters. I show that even a very small number of photons of higher energy, which I ascribe to noise from the microwave generator, would dominate the quasiparticle density at lower temperatures. Under this assumption, my calculations also reproduce the quality factors at lower temperatures. In the second part of this thesis, I investigate the effects of spatial fluctuations of the superconducting energy gap on the dynamics of quasiparticles. Recently, it has been proposed that such fluctuations may lead to the localization of quasiparticles in states below the energy gap, which could cause a finite quasiparticle density even at very low temperatures. Using the Keldysh-Usadel formalism, I derive rates for the different processes (recombination/(de-) localization/generation) of quasiparticles in such systems. Using these rate equations I derive new upper limits for the quasiparticle density that could result from these localized states. These upper limits show that localization caused by weak magnetic impurities in typical aluminum systems does not lead to a relevant quasiparticle density. This contradicts previous theories, which only consider the recombination between two localized quasiparticles without examining their dynamics in detail.
We recently predicted the formation of a highly non-equilibrium quasiparticle (qp) distribution in low TC multiple tunnelling superconducting tunnel junctions (STJs) [1]. The situation arises through qp energy gain in cycles of successive forward and back tunnelling events in the absence of relaxation via sub-gap phonon emission. The qps can acquire sufficient energy to emit phonons, which break more Cooper pairs and release additional qps. In this paper we report theoretical and experimental studies of the effect of this process on photon detection by such an STJ. We derived a set of energy-dependent balance equations [2], which describe the kinetics of the qps and phonons, including the qp multiplication process described above. Solution of the balance equations gives the non-equilibrium distribution of the qps as a function of time and energy, and hence the responsivity of the STJ as a function of bias voltage. We compared the theoretical results with experiments on high quality, multiple-tunnelling Al STJs cooled to 35mK in an adiabatic demagnetisation refrigerator, and illuminated with monochromatic photons with wavelengths between 250 and 1000 nm. It was found that in the larger junctions with the longest qp loss time, both responsivity and signal decay time increased rapidly with bias voltage. Excellent agreement was obtained between the observed effects and theoretical modelling.
This manuscript summarizes my research activities devoted to the study of nonequilibrium phenomena in mesoscopic superconducting and semiconducting circuits. The work develops along two directions: the dynamics of metallic Josephson junctions driven out of equilibrium and the interaction between electrons and microwave photons in mesoscopic quantum circuits.The first part investigates diffusive superconductor–normal metal–superconductor Josephson junctions subjected to strong perturbations such as microwave irradiation or stochastic injection of high-energy quasiparticles. These experiments reveal how nonequilibrium excitations modify the Andreev spectrum and the phase dynamics of the junction. The second part addresses electron–photon coupling in mesoscopic circuits across different interaction regimes. Early work focused on semiconductor double quantum dots coupled to low-impedance microwave cavities in the weak coupling regime. Later work involved the fabrication and characterization of high-kineticinductance superconducting materials, allowing the realization of high-impedance resonators and stronger light-matter coupling. Finally, a superconducting tunnel junction coupled to a high-impedance granular aluminum cavity allowed bath engineering based on photo-assisted quasiparticle tunneling, efficient photon-toelectron conversion, and continuous single microwave photon detection.
Non-local conductance experiments using tunnel junctions can provide valuable spectroscopic information on both the transport and relaxation of quasiparticles in superconductors, as these techniques directly probe the quasiparticle charge and energy imbalance even at mK temperatures. In this work, we employ mesoscopic three terminal Cu and Al NIS devices to study non-local quasiparticle transport over length-scales on the order of the superconducting coherence length in this regime. Via a dual-bias scheme, which utilizes detector biases both above and below the superconducting gap, we are able to extract the effect of quasiparticle energy imbalance via its impact on the self consistent pair potential by symmetry considerations. We observe non-local conductance features due to pair-breaking which are anti-symmetric with respect to the polarity of the voltage bias, with a sharp onset during single electron tunneling at energies around 3Δ. We compare these findings with quasiclassical simulations including inelastic effects to obtain estimates of the energy dependent inelastic scattering time. In addition, we demonstrate kinetic effects due to a large applied supercurrent which can also be captured in this formalism and decomposed with respect to the particle-hole symmetry and supercurrent direction, and discuss further opportunities for the advancement of this method.
We recently predicted the formation of a highly non-equilibrium quasiparticle (qp) distribution in low TC multiple tunnelling superconducting tunnel junctions (STJs) [1]. The situation arises through qp energy gain in cycles of successive forward and back tunnelling events in the absence of relaxation via sub-gap phonon emission. The qps can acquire sufficient energy to emit phonons, which break more Cooper pairs and release additional qps. In this paper we report theoretical and experimental studies of the effect of this process on photon detection by such an STJ. We derived a set of energy-dependent balance equations [2], which describe the kinetics of the qps and phonons, including the qp multiplication process described above. Solution of the balance equations gives the non-equilibrium distribution of the qps as a function of time and energy, and hence the responsivity of the STJ as a function of bias voltage. We compared the theoretical results with experiments on high quality, multiple-tunnelling Al STJs cooled to 35mK in an adiabatic demagnetisation refrigerator, and illuminated with monochromatic photons with wavelengths between 250 and 1000 nm. It was found that in the larger junctions with the longest qp loss time, both responsivity and signal decay time increased rapidly with bias voltage. Excellent agreement was obtained between the observed effects and theoretical modelling.