This manuscript summarizes my research activities devoted to the study of nonequilibrium phenomena in mesoscopic superconducting and semiconducting circuits. The work develops along two directions: the dynamics of metallic Josephson junctions driven out of equilibrium and the interaction between electrons and microwave photons in mesoscopic quantum circuits.The first part investigates diffusive superconductor–normal metal–superconductor Josephson junctions subjected to strong perturbations such as microwave irradiation or stochastic injection of high-energy quasiparticles. These experiments reveal how nonequilibrium excitations modify the Andreev spectrum and the phase dynamics of the junction. The second part addresses electron–photon coupling in mesoscopic circuits across different interaction regimes. Early work focused on semiconductor double quantum dots coupled to low-impedance microwave cavities in the weak coupling regime. Later work involved the fabrication and characterization of high-kineticinductance superconducting materials, allowing the realization of high-impedance resonators and stronger light-matter coupling. Finally, a superconducting tunnel junction coupled to a high-impedance granular aluminum cavity allowed bath engineering based on photo-assisted quasiparticle tunneling, efficient photon-toelectron conversion, and continuous single microwave photon detection.
This manuscript summarizes my research activities devoted to the study of nonequilibrium phenomena in mesoscopic superconducting and semiconducting circuits. The work develops along two directions: the dynamics of metallic Josephson junctions driven out of equilibrium and the interaction between electrons and microwave photons in mesoscopic quantum circuits.The first part investigates diffusive superconductor–normal metal–superconductor Josephson junctions subjected to strong perturbations such as microwave irradiation or stochastic injection of high-energy quasiparticles. These experiments reveal how nonequilibrium excitations modify the Andreev spectrum and the phase dynamics of the junction. The second part addresses electron–photon coupling in mesoscopic circuits across different interaction regimes. Early work focused on semiconductor double quantum dots coupled to low-impedance microwave cavities in the weak coupling regime. Later work involved the fabrication and characterization of high-kineticinductance superconducting materials, allowing the realization of high-impedance resonators and stronger light-matter coupling. Finally, a superconducting tunnel junction coupled to a high-impedance granular aluminum cavity allowed bath engineering based on photo-assisted quasiparticle tunneling, efficient photon-toelectron conversion, and continuous single microwave photon detection.
Circuit QED techniques have been instrumental in manipulating and probing with exquisite sensitivity the quantum state of superconducting quantum bits coupled to microwave cavities. Recently, it has become possible to fabricate new devices in which the superconducting quantum bits are replaced by hybrid mesoscopic circuits combining nanoconductors and metallic reservoirs. This mesoscopic QED provides a new experimental playground to study the light-matter interaction in electronic circuits. Here, we present the experimental state of the art of mesoscopic QED and its theoretical description. A first class of experiments focuses on the artificial atom limit, where some quasiparticles are trapped in nanocircuit bound states. In this limit, the circuit QED techniques can be used to manipulate and probe electronic degrees of freedom such as confined charges, spins, or Andreev pairs. A second class of experiments uses cavity photons to reveal the dynamics of electron tunneling between a nanoconductor and fermionic reservoirs. For instance, the Kondo effect, the charge relaxation caused by grounded metallic contacts, and the photo-emission caused by voltage-biased reservoirs have been studied. The tunnel coupling between nanoconductors and fermionic reservoirs also enable one to obtain split Cooper pairs, or Majorana bound states. Cavity photons represent a qualitatively new tool to study these exotic condensed matter states.
We review recent developments regarding the quantum dynamics and many-body physics with light, in superconducting circuits and Josephson analogues, by analogy with atomic physics. We start with quantum impurity models addressing dissipative and driven systems. Both theorists and experimentalists are making efforts towards the characterization of these non-equilibrium quantum systems. We show how Josephson junction systems can implement the equivalent of the Kondo effect with microwave photons. The Kondo effect can be characterized by a renormalized light frequency and a peak in the Rayleigh elastic transmission of a photon. We also address the physics of hybrid systems comprising mesoscopic quantum dot devices coupled with an electromagnetic resonator. Then, we discuss extensions to Quantum Electrodynamics (QED) Networks allowing one to engineer the Jaynes–Cummings lattice and Rabi lattice models through the presence of superconducting qubits in the cavities. This opens the door to novel many-body physics with light out of equilibrium, in relation with the Mott–superfluid transition observed with ultra-cold atoms in optical lattices. Then, we summarize recent theoretical predictions for realizing topological phases with light. Synthetic gauge fields and spin–orbit couplings have been successfully implemented in quantum materials and with ultra-cold atoms in optical lattices — using time-dependent Floquet perturbations periodic in time, for example — as well as in photonic lattice systems. Finally, we discuss the Josephson effect related to Bose–Hubbard models in ladder and two-dimensional geometries, producing phase coherence and Meissner currents. The Bose–Hubbard model is related to the Jaynes–Cummings lattice model in the large detuning limit between light and matter (the superconducting qubits). In the presence of synthetic gauge fields, we show that Meissner currents subsist in an insulating Mott phase.
Although Josephson junctions can be viewed as highly nonlinear impedances for superconducting quantum technologies, they also possess internal dynamics that may strongly affect their behavior. Here, we construct a computational framework that includes a microscopic description of the junction (full fledged treatment of both the superconducting condensate and the quasiparticles) in the presence of a surrounding electrical circuit. Our approach generalizes the standard resistor capacitor Josephson model to arbitrary junctions (including, e.g., multiterminal geometries and/or junctions that embed topological or magnetic elements) and arbitrary electric circuits treated at the classical level. By treating the superconducting condensate and quasiparticles on equal footings, we capture nonequilibrium phenomena such as multiple Andreev reflection. We show that the interplay between the quasiparticle dynamics and the electrical environment leads to the emergence of new phenomena. In a RC circuit connected to single channel Josephson junction, we find out-of-equilibrium current-phase relations that are strongly distorted with respect to the (almost sinusoidal) equilibrium one, revealing the presence of the high harmonic ac Josephson effect. In an RLC circuit connected to a junction, we find that the shape of the resonance is strongly modified by the quasiparticle dynamics: close to resonance, the current can be smaller than without the resonator. Our approach provides a route for the quantitative modeling of superconducting-based circuits.
Quasiparticle (QP) effects play a significant role in the coherence and fidelity of superconducting quantum circuits.The Andreev bound states of high-transparency Josephson junctions can act as low-energy traps for QPs, providing a mechanism for studying the dynamics and properties of both the QPs and the junction.Using locally injected and thermal QPs, we study QP loss and QP poisoning in epitaxial Al-InAs Josephson junctions incorporated in a superconducting quantum interference device (SQUID) galvanically shorting a superconducting resonator to ground.We observe changes in the resonance line shape and frequency shifts consistent with QP trapping into and clearing out of the ABSs of the junctions when the junctions are phase biased.By monitoring the QP trapping and clearing mechanisms in time, we find a time scale of O(1 µs) for these QP dynamics, consistent with the presence of phonon-mediated QP-QP interactions.Our measurements suggest that electron-phonon interactions play a significant role in the relaxation mechanisms of our system, while electron-photon interactions and electron-phonon interactions govern the clearing mechanisms.Our results highlight the QP-induced dissipation and complex QP dynamics in superconducting quantum circuits fabricated on superconductor-semiconductor heterostructures.
Conventional tunnel Josephson junctions form the basic building blocks of superconducting electronics. Their operation is based on comparatively simple dynamics where the superconducting phases across the junctions is the only dynamical degree of freedom. The goal of the project on which this thesis is based, is to understand the physics and develop a consistent theoretical description of the quantum dynamics of unconventional Josephson structures: spin active junctions, junctions containing low energy quasiparticles, and junctions composed of d-wave superconductors. Spin active Josephson junctions involve the additional degree of freedom of quasiparticle spin. Here we theoretically investigate the spin-structure of the current carrying interface bound states - Andreev Bound States (ABS), and induced ground state spin polarization of a short (shorter than the superconducting coherence length) nanowire junction containing a localized magnetic moment. We show that temporal variation of the superconducting phase difference and magnetic moment induce rotations in spin polarized and unpolarized subspaces respectively, which is manifested by temporal oscillation of the Josephson current.The interlevel transitions obey a selection rule that forbids manipulations in a certain region ofexternal parameters and results from specific properties of Andreev bound states in magnetic contacts where, in a certain regime of phase bias and strength of magnetic scatterer, ABS belong to different eigenstates of the combined charge and parity inversion symmetry operator.A general framework is developed to include low energy quasiparticle states into the dynamics of Josephson junctions. Such states exist in e.g. constriction type junctions with high transparency channels or resonant states, as well as in junctions of unconventional superconductors. The existence of such states prevent the separation of energy scales which in conventional tunnel junctions freezes out the quasiparticle degrees of freedom. We show that the resonant interaction with such low energy states rather than the Josephson potential defines the nonlinear Josephson dynamics at small amplitudes.The framework is applied to high temperature Josephson junctions, whose unconventional order parameter admits ABS with energies in the middle of the superconducting gap - Mid Gap States (MGS). In addition to the non-linear dynamics induced by the MGS, we identify a reentrance effect in the transition between thermal activation and macroscopic quantum tunneling associated with the MGS, and connect this phenomenon to experimental observations.
Properties of weak links between two superconductors, or Josephson junctions, make them interesting for fundamental physics research. Since their discovery over four decades ago, they have provided a unique way to study the behavior of the superconducting quantum phase. More recently, ultra small, or mesoscopic, Josephson junctions with substantial single Cooper pair charging energy have gained interest due to their behavior as macroscopic quantum objects. In addition to the theoretical interest, Josephson junctions can be used as active elements in circuit applications. Particularly, in this Thesis we study two different devices. We develop the required theoretical treatments, derive device properties, and compare the results with experimental data. The first application is a Josephson voltage standard based on externally damped Superconductor - Insulator - Superconductor junctions. It consists of an array of large Josephson junctions connected in series and irradiated with a 70 GHz microwave signal. Phase locking the Josephson dynamics into the signal leads to the quantization of the voltage. This is utilized in metrology. We introduce a new circuit solution based on frequency dependent damping of the junctions. Optimization and some designs for practical arrays are presented. The purpose is to find such a design that the array is fast, has low power consumption and is as stable as possible. Arrays able to generate DC voltages of order 1 volt with metrological accuracy are demonstrated experimentally and their applicability in AC voltage calibrations is analyzed. The second application is the Bloch Oscillating Transistor (BOT). The BOT is based on controlling the Cooper pair current in an ultra small Josephson junction by means of quasiparticles tunneling through a normal junction. As part of the thesis work, the principle of operation is first demonstrated computationally. The model is then refined to yield quantitative predictions of the characteristics. Finally, an analytic theory for the device is developed and the properties as an amplifier are derived.