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arXiv:cond-mat/0401477 · Journal of the Physical Society of Japan

Static and Dynamic Properties of Antiferromagnetic Heisenberg Ladders: Fermionic versus Bosonic Approaches

宏光 堀, Shoji Yamamoto

Published Mar 15, 2004• 9 citations
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Abstract

In terms of spinless fermions via the Jordan-Wigner transformation along a snake-like path and spin waves modified so as to restore the sublattice symmetry, we investigate static and dynamic properties of two-leg antiferromagnetic Heisenberg ladders. The specific heat is finely reproduced by the spinless fermions, whereas the magnetic susceptibility is well described by the modified spin waves. The nuclear spin-lattice relaxation rate is discussed in detail with particular emphasis on its novel field dependence.

DOI
10.1143/jpsj.73.549

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In terms of spinless fermions via the Jordan-Wigner transformation along a snake-like path and spin waves modified so as to restore the sublattice symmetry, we investigate static and dynamic properties of two-leg antiferromagnetic Heisenberg ladders. The specific heat is finely reproduced by the spinless fermions, whereas the magnetic susceptibility is well described by the modified spin waves. The nuclear spin-lattice relaxation rate is discussed in detail with particular emphasis on its novel field dependence.
A Wigner-Jordan (WJ) transformation is used to study the one-dimensional (1D) and two-dimensional (2D) quantum antiferromagnetic Heisenberg model. The advantage of using the Wigner-Jordan transformation is that it preserves all spin-commutation relations as well as the spin on-site exclusion principle. In the 1D case a nearest-neighbor covalent-bonding state of the WJ fermions is found to have a ground-state energy (-0.4351J per site) comparable with that from the Bethe-ansatz solution (-0.4431J per site), and a linear energy spectrum at low energies with velocity 1.6366J, in close agreement with the velocity obtained by Haldane for the quantum antiferromagnetic Heisenberg model with 1/d2{\mathit{d}}^{2}d2 interaction (1.5708J). The method used for studying the 1D model is then applied to the 2D Heisenberg model in a square lattice. The resulting state at finite temperature is the in-phase flux state, i.e., a flux state of the Wigner-Jordan spinless fermions with an in-phase fermion orbital current circulating around each elementary plaquette.The single-particle excitation spectrum, i.e., the energy dispersion of reversing orientation of a spin in the system, of the in-phase flux state is overall similar to that of spin waves, with significant difference near the edge point k=(\ensuremath{\pi},0), at which the excitation energy of the WJ fermion is zero, whereas that of the spin-wave excitation is 2J. The specific heat of the in-phase flux state predicts a correct temperature dependence over the entire temperature range, namely a T2{\mathit{T}}^{2}T2 dependence at low temperature, a peak near T/J=0.6, and a 1/T2{\mathit{T}}^{2}T2 decreasing at high temperature. It also gives excellent agreement with the specific heat calculated from numerical methods. In contrast, the spin-wave theory only correctly predicts a T2{\mathit{T}}^{2}T2 dependence at low temperature. The Raman spectrum of the in-phase flux state is calculated and shows significant improvement over that from spin-wave theories compared with the experimental spectrum of La2{\mathrm{La}}_{2}La2​CuO4{\mathrm{CuO}}_{4}CuO4​. The exchange parameter, J, obtained from the comparison is 1060 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}1}$, in agreement with that obtained from analyzing the neutron-scattering data.
In terms of spinless fermions and spin waves, we describe magnetic properties of a spin-1/2 ferromagnetic– antiferromagnetic bond-alternating chain which behaves as a Haldane-gap antiferromagnet. On one hand, we employ the Jordan–Wigner transformation and treat the fermionic Hamiltonian within the Hartree–Fock approximation. On the other hand, we employ the Holstein– Primakoff transformation and modify the conventional spin-wave theory so as to restore the sublattice symmetry. We calculate the excitation gap, the specific heat, the magnetic susceptibility, magnetization curves, and the nuclear spin-lattice relaxation rate with varying bond alternation. These schemes are further applied to a bond-alternating tetramerized chain which behaves as a ferrimagnet. The fermionic language is particularly stressed as a useful tool to investigate one-dimensional spin-gapped antiferromagnets, while the bosonic one works better for ferrimagnets.
The temperature dependence of the static spin susceptibility, χ, and NMR relaxation rate, T 1 -1 , of S =1/2 Heisenberg two-leg ladder systems have been studied based on the Majorana fermion representation of the S =1/2 Heisenberg spin Hamiltonian introduced by Shelton, Nersesyan and Tsvelik (Phys. Rev. B 53 (1996) 8521). It is shown that in the case of SrCu 2 O 3 , we can fit the experimental data of χ and T 1 -1 in terms of the massive Majorana fermion excitation with mass m =440 K to resolve the apparent discrepancy of the spin gap activation energies between χ and T 1 -1 .
Using the recently developed transfer-matrix renormalization group method, we have studied the thermodynamic properties of two-leg antiferromagnetic ladders in a magnetic field. Based on different magnetization behaviors, we found a disordered spin liquid, the Luttinger liquid, spin-polarized phases, and a classical regime. Our calculations in the Luttinger liquid regime suggest that both the divergence of the NMR relaxation rate and the anomalous specific heat behavior observed on Cu2(C5H12N2)2Cl4 are due to a quasi-one-dimensional effect rather than three-dimensional ordering.