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Physical Review B

Spin locking and freezing phenomena in the antiferromagnetic Heisenberg model on the three-leg ladder

Mohamed Moussadek Azzouz, K. A. Asante

Published Sep 27, 2005• 10 citations
Publisher

Abstract

The antiferromagnetic Heisenberg model on the three-leg ladder is studied using the generalized Jordan-Wigner transformation in dimensions higher than 1, and the bond-mean-field theory. The magnetic susceptibility and other thermodynamic quantities are analyzed as a function of the rung-to-leg coupling ratio $\ensuremath{\alpha}$ and temperature $T$. We fit the experimental susceptibility data of the three-leg material ${\mathrm{Sr}}_{2}{\mathrm{Cu}}_{3}{\mathrm{O}}_{5}$ of Azuma and co-workers with good agreement. One of the main findings of this work is the proposal that close to two-thirds of the spin degrees of freedom on each of the rungs of the ladder lock at low $T$ for small $\ensuremath{\alpha}$, then collectively almost $2∕3$ of the spin degrees of freedom on all the rungs freeze completely at low $T$ for $\ensuremath{\alpha}$ greater than a threshold value. The approach developed here can be used to study the three-leg ladder for all values of $\ensuremath{\alpha}$, and is thus suitable for the description of the crossover regime between the weak- and strong-coupling regimes.

DOI
10.1103/physrevb.72.094433

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The antiferromagnetic Heisenberg model on the three-leg ladder is studied using the generalized Jordan-Wigner transformation in dimensions higher than 1, and the bond-mean-field theory. The magnetic susceptibility and other thermodynamic quantities are analyzed as a function of the rung-to-leg coupling ratio \ensuremathα\ensuremath{\alpha}\ensuremathα and temperature TTT. We fit the experimental susceptibility data of the three-leg material Sr2Cu3O5{\mathrm{Sr}}_{2}{\mathrm{Cu}}_{3}{\mathrm{O}}_{5}Sr2​Cu3​O5​ of Azuma and co-workers with good agreement. One of the main findings of this work is the proposal that close to two-thirds of the spin degrees of freedom on each of the rungs of the ladder lock at low TTT for small \ensuremathα\ensuremath{\alpha}\ensuremathα, then collectively almost 2∕32∕32∕3 of the spin degrees of freedom on all the rungs freeze completely at low TTT for \ensuremathα\ensuremath{\alpha}\ensuremathα greater than a threshold value. The approach developed here can be used to study the three-leg ladder for all values of \ensuremathα\ensuremath{\alpha}\ensuremathα, and is thus suitable for the description of the crossover regime between the weak- and strong-coupling regimes.
This paper is about the frustration-induced criticality in the antiferromagnetic Heisenberg model on the two-leg ladder with exchange interactions along the chains, rungs, and diagonals, and also about the effect of thermal fluctuations on this criticality. The method used is the bond-mean-field theory, which is based on the Jordan–Wigner transformation in dimensions higher than one. In this paper, we will summarize the main results presented in a talk, and report on new results about the couplings and temperature dependences of the spin susceptibility.PACS Nos.: 75.10.Jm, 75.10.Dg, 75.50.Ee
Field-induced quantum (zero temperature) criticality described using parameters that are not associated with a symmetry-breaking long-range order is found in the spin-12\frac{1}{2}21​ antiferromagnetic three-leg Heisenberg ladder. These parameters represent the spin bond order, which is a consequence of the probability for spins on adjacent sites to be bound in a singletlike arrangement. They underwent two phase transitions, one at the lower critical field hc1{h}_{c1}hc1​ and the other at the upper critical field hc2{h}_{c2}hc2​. The field dependence of these bond parameters and of the magnetization is calculated for several values of the rung coupling in all regimes. This yields the coupling field phase diagram. It is found that the rung coupling must exceed a threshold value for the plateau, at one third of the saturation magnetization, to appear. The results obtained here within the bond mean-field theory compare well with existing numerical data.
The antiferromagnetic Heisenberg model on the two-leg ladder with exchange interactions along the chains, rungs, and diagonals is studied using the Jordan-Wigner transformation and bond-mean-field theory. The inclusion of all three couplings introduces frustration to the system and depending on their relative strengths the ladder can adopt one of three possible magnetically disordered gapped states. The phase diagram found in this mean-field approach is in very good agreement with the one calculated by Weihong et al. [Phys. Rev. B 57, 11439 (1998)] using the Lanczos exact diagonalization method. By analyzing the ground-state energy, we study quantum criticality when the coupling parameters are varied at zero temperature. We study the effect of temperature on the phase boundaries and find that the system shows thermally induced criticality for some values of the rung and diagonal coupling constants. All the phase transitions encountered in this system occur between disordered phases and are all caused by frustration.
Using the density matrix renormalization group method, we have obtained the ground-state phase diagram of a spin-1/2 two-leg antiferromagnetic Heisenberg ladder with a ferromagnetic diagonal interaction ${J}_{\ifmmode\times\else\texttimes\fi{}}.$ The boundary between the two phases found in the system, the Haldane phase and the singlet phase, lies in the frustrated area of the parameter space, i.e., both the rung coupling ${J}_{\ensuremath{\perp}}$ and the diagonal coupling ${J}_{\ifmmode\times\else\texttimes\fi{}}$ are ferromagnetic. The spin gap is found to be insensitive to the change of the ferromagnetic diagonal coupling strength when the ratio of the rung coupling constant ${J}_{\ensuremath{\perp}}$ to the leg coupling constant ${J}_{\ensuremath{\Vert}}$ is 0.5, in agreement with the analysis of recent experimental spin susceptibility data.
Extraction of antiferromagnetic (AF) exchange constants J and J\ensuremath{'} in two-leg spin-1/2 nearest-neighbor (NN) Heisenberg ladders from experimental magnetic spin susceptibility \ensuremath{\chi}(T) data is studied, where J\ensuremath{'} is the NN exchange constant in the rungs and J is that in the legs. Two low-T (T\ensuremath{\ll}J/kB{\mathit{k}}_{\mathit{B}}kB​) approximations of Troyer, Tsunetsugu, and W\"urtz [Phys. Rev. B 50, 13 515 (1994)] for \ensuremath{\chi}(T) of the isolated spin-1/2 two-leg ladder with J\ensuremath{'}/J=1 are shown to be accurate to \ensuremath{\sim}10% when extrapolated to T\ensuremath{\sim}J\ensuremath{'}/kB{\mathit{k}}_{\mathit{B}}kB​. The variations in the magnetic excitation dispersion relation parameters [which enter the low-T expression of Troyer et al. for \ensuremath{\chi}(T)] for J\ensuremath{'}/J1 are inferred from previous theoretical results. Next, the values of the maxima in \ensuremath{\chi}(T)\ensuremath{\equiv}${\mathrm{\ensuremath{\chi}}}^{\mathrm{max}}$ from many numerical calculations in the literature for various nonfrustrated spin-1/2 NN Heisenberg antiferromagnets are considered. The values of the product ${\mathrm{\ensuremath{\chi}}}^{\mathrm{max}}$zeff{\mathit{z}}_{\mathrm{eff}}zeff​ are found to depend systematically and almost uniqely on an effective magnetic coordination number zeff{\mathit{z}}_{\mathrm{eff}}zeff​, defined in the text, but are nearly independent of the dimensionality of the spin lattice and of the magnitude of any gap in the magnetic excitation spectrum. This observation allows accurate bounds on the exchange coupling constants in arbitrary quasi-low-dimensional spin-1/2 antiferromagnets to be inferred from experimental ${\mathrm{\ensuremath{\chi}}}^{\mathrm{max}}$ values. Finally, a mean-field-type expression for \ensuremath{\chi}(T) for arbitrary quasi-low-dimensional spin-1/2 Heisenberg antiferromagnets is derived, using the above ${\mathrm{\ensuremath{\chi}}}^{\mathrm{max}}$ phenomenology as input, which allows the influence of intersystem coupling on \ensuremath{\chi}(T) to be evaluated. These results, and the \ensuremath{\chi}(T) calculations of Barnes and Riera [Phys. Rev. B 50, 6817 (1994)] for isolated two-leg spin-1/2 Heisenberg ladders, are used to analyze the experimental \ensuremath{\chi}(T) data of Azuma et al. [Phys. Rev. Lett. 73, 3463 (1994)] for the spin-1/2 two-leg ladder compound SrCu2{\mathrm{SrCu}}_{2}SrCu2​O3{\mathrm{O}}_{3}O3​. The analyses together suggest that J\ensuremath{'}/J\ensuremath{\sim}0.5, contrary to the expectation that J\ensuremath{'}/J\ensuremath{\approxeq}1, and that J is very large (\ensuremath{\sim}2000 K), similar to the value of J in the linear-chain cuprate Sr2{\mathrm{Sr}}_{2}Sr2​CuO3{\mathrm{CuO}}_{3}CuO3​. \textcopyright{} 1996 The American Physical Society.
The antiferromagnetic Heisenberg two-leg ladder in the presence of frustration and an external magnetic field is a system that is characterized by two sorts of quantum criticalities, not only one. One criticality is the consequence of intrinsic frustration, and the other one is a result of the external magnetic field. So the behaviour of each of them in the presence of the other deserves to be studied. Using the Jordan–Wigner transformation in dimensions higher than one and the bond-mean-field theory we examine the interplay between the field-induced and frustration-induced quantum criticalities in this system. The present work could constitute a prototype for those systems showing multiple, perhaps sometimes competing, quantum criticalities. We calculate several physical quantities such as magnetization and spin susceptibility as functions of field and temperature.PACS Nos.: 75.10.Jm 73.43.Nq 75.10.Pq 75.10.Dg