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arXiv:cond-mat/0401399

A method for direct observation of quantum tunneling in a single molecule

Anatoly Yu. Smirnov

Published Jan 21, 2004• 0 citations
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Abstract

An application of impedance measurement technique (IMT) for a detection of quantum tunneling in molecular structures is investigated. A charged particle which tunnels in a two-well potential is electrically coupled to a high-quality superconducting LC-circuit(tank) that makes possible a measurement of the electric susceptibility of the molecule at the resonant frequency of the tank. The real part of this susceptibility bears information about the tunneling rate through a measurable parameter - a phase angle between the tank voltage and a bias current applied to the tank. It is shown that the present approach is highly sensitive and allows the monitoring of the tunnel motion of charged nuclei in a single molecule.

DOI
10.48550/arxiv.cond-mat/0401399

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An application of impedance measurement technique (IMT) for a detection of quantum tunneling in molecular structures is investigated. A charged particle which tunnels in a two-well potential is electrically coupled to a high-quality superconducting LC-circuit(tank) that makes possible a measurement of the electric susceptibility of the molecule at the resonant frequency of the tank. The real part of this susceptibility bears information about the tunneling rate through a measurable parameter - a phase angle between the tank voltage and a bias current applied to the tank. It is shown that the present approach is highly sensitive and allows the monitoring of the tunnel motion of charged nuclei in a single molecule.
We propose to investigate flux qubits by the impedance measurement technique (IMT), currently used to determine the current-phase relation in Josephson junctions. We analyze in detail the case of a high-quality tank circuit coupled to a persistent-current qubit, to which the IMT was successfully applied in the classical regime. It is shown that the low-frequency IMT can give considerable information about the level anticrossing, in particular the value of the tunneling amplitude. An interesting difference exists between applying the ac bias directly to the tank and indirectly via the qubit. In the latter case, a convenient way to find the degeneracy point in situ is described. Our design only involves existing technology, and its noise tolerance is quantitatively estimated to be realistic.
We have studied the low-frequency magnetic susceptibility of two inductively coupled flux qubits using the impedance measurement technique (IMT), through their influence on the resonant properties of a weakly coupled high-quality tank circuit. In a single qubit, an IMT dip in the tank's current-voltage phase angle at the level anticrossing yields the amplitude of coherent flux tunneling. For two qubits, the difference (IMT deficit) between the sum of single-qubit dips and the dip amplitude when both qubits are at degeneracy shows that the system is in a mixture of entangled states (a necessary condition for entanglement). The dependence on temperature and relative bias between the qubits allows one to determine all the parameters of the effective Hamiltonian and equilibrium density matrix, and confirms the formation of entangled eigenstates.
A quantum electrometer is proposed which is based on charge modulation of the Josephson supercurrent in the Bloch transistor inserted in a superconducting ring. As this ring is inductively coupled to a high- Q resonance tank circuit, the variations of the charge on the transistor island are converted into variations of amplitude and phase of oscillations in the tank. These variations are amplified and then detected. At sufficiently low temperature of the tank the device sensitivity is determined by the energy resolution of the amplifier, that can be reduced down to the standard quantum limit of 1 / 2Planck's over 2pi. A "back-action-evading" scheme of subquantum limit measurements is proposed.
Time-domain observations of coherent oscillations between quantum states in mesoscopic superconducting systems have so far been restricted to restoring the time-dependent probability distribution from the readout statistics. We propose a method for direct observation of Rabi oscillations in a phase qubit. The external source, typically in the GHz range, induces transitions between the qubit levels. The resulting Rabi oscillations of supercurrent in the qubit loop are detected by a high-quality resonant tank circuit, inductively coupled to the phase qubit. Here we present the results of detailed computer simulations of the interaction of a classical object (resonant tank circuit) with a quantum object (phase qubit), which explicitly account for the back action of a tank circuit. According to the results of our simulations the Rabi oscillations in the MHz range can be detected using the conventional NMR pulse Fourier technique.