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arXiv:cond-mat/0401109 · Physical Review Letters

Crossover from a Molecular Bose-Einstein Condensate to a Degenerate Fermi Gas

M. Bartenstein, A. Altmeyer, S. Riedl, Selim Jochim, Cheng Chin, Johannes Hecker Denschlag, Rudolf Grimm

Published Mar 23, 2004• 695 citations
arXivHTMLPDF

Abstract

We demonstrate a reversible conversion of a 6Li2 molecular Bose-Einstein condensate to a degenerate Fermi gas of atoms by adiabatically crossing a Feshbach resonance. By optical in situ imaging, we observe a smooth change of the cloud size in the crossover regime. On the Feshbach resonance, the ensemble is strongly interacting and the measured cloud size is 75(7)% of the one of a noninteracting zero-temperature Fermi gas. The high condensate fraction of more than 90% and the adiabatic crossover suggest our Fermi gas to be cold enough to form a superfluid.

DOI
10.1103/physrevlett.92.120401

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We demonstrate a reversible conversion of a 6Li2 molecular Bose-Einstein condensate to a degenerate Fermi gas of atoms by adiabatically crossing a Feshbach resonance. By optical in situ imaging, we observe a smooth change of the cloud size in the crossover regime. On the Feshbach resonance, the ensemble is strongly interacting and the measured cloud size is 75(7)% of the one of a noninteracting zero-temperature Fermi gas. The high condensate fraction of more than 90% and the adiabatic crossover suggest our Fermi gas to be cold enough to form a superfluid.
Atomic Feshbach resonances have recently been used to produce a strongly interacting Fermi gas, where the BCS/BEC crossover can be explored. We have used both narrow and broad Feshbach resonances to convert a quantum degenerate Fermi gas of 6Li atoms into an ultracold gas of Li2 molecules. For the narrow resonances, the molecules are formed by coherent adiabatic passage through the resonance. We find that 50% of the atoms are converted to molecules. Furthermore, the lifetime of these molecules was measured to be surprisingly long, 1 s. We will discuss these measurements in the context of the present theoretical understanding. Molecules can also be formed using static fields near the broad Feshbach resonance. The lifetime of these molecules is again long, and sufficient to enable their evaporation to a Bose‐Einstein condensate. Phase contrast images of the molecular condensate are presented. The BCS/BEC crossover may be explored by starting with a pure molecular condensate on the low‐field side of the Feshbach resonance, and adiabatically changing the field to any final value around resonance. We combine this ability with optical spectroscopy on a bound‐bound molecular transition to probe the nature of the many‐body wavefunction in the crossover regime.
We have observed Bose-Einstein condensation of pairs of fermionic atoms in an ultracold 6Li gas at magnetic fields above a Feshbach resonance, where no stable 6Li2 molecules would exist in vacuum. We accurately determined the position of the resonance to be 822+/-3 G. Molecular Bose-Einstein condensates were detected after a fast magnetic field ramp, which transferred pairs of atoms at close distances into bound molecules. Condensate fractions as high as 80% were obtained. The large condensate fractions are interpreted in terms of preexisting molecules which are quasistable even above the two-body Feshbach resonance due to the presence of the degenerate Fermi gas.
We consider a single vortex in a superfluid Fermi gas in the BCS-BEC crossover regime near a Feshbach resonance. The effect of the molecular Bose-Einstein condensate upon the vortex structure is discussed within the mean field approximation at zero temperature. Using the self-consistent Bogoliubov-de Gennes equation of the fermion-boson coupled model, we calculate density distributions of atoms and molecules. As the number of the molecules increases, both atomic and molecular density changes from BCS-like distribution to BEC-like. We also study the change of the vortex core size in the crossover regime.
The realization of fermionic superfluidity in a dilute gas of atoms, analogous to superconductivity in metals, is a long-standing goal of ultracold gas research. Beyond being a new example of this fascinating quantum phenomenon, fermionic superfluidity in an atomic gas holds the promise of adjustable interactions and the ability to tune continuously from BCS-type superfluidity to Bose-Einstein condensation (BEC). This crossover between BCS superfluidity of correlated atom pairs in momentum space and BEC of local pairs has long been of theoretical interest, motivated in part by the discovery of high Tc superconductors. In atomic Fermi gas experiments superfluidity has not yet been demonstrated; however recent experiments have made remarkable progress toward this goal. Starting from an ultracold Fermi gas experimenters have used Feshbach resonances to reversibly create molecules, i.e. composite bosons consisting of local fermion pairs. Furthermore, the experiments have shown that the resulting diatomic molecules can have surprisingly long lifetimes. Here we report the conversion of a Fermi sea of atoms into a molecular BEC. In addition to being the first molecular condensate in thermal equilibrium, this BEC represents one extreme of the predicted BCS-BEC continuum.
We observe characteristic atomic behaviors in the Bose–Einstein-condensation-Bardeen–Cooper–Schrieffer (BECBCS) crossover, by accurately tuning the magnetic field across the Feshbach resonance of lithium atoms. The magnetic field is calibrated by measuring the Zeeman shift of the optical transition. A non-monotonic anisotropic expansion is observed across the Feshbach resonance. The density distribution is explored in different interacting regimes, where a condensate of diatomic molecules forms in the BEC limit with the indication of a bimodal distribution. We also measure the three-body recombination atom loss in the BEC-BCS crossover, and find that the magnetic field of the maximum atom loss is in the BEC limit and gets closer to the Feshbach resonance when decreasing the atom temperature, which agrees with previous experiments and theoretical prediction. This work builds up a controllable platform for the study on the strongly interacting Fermi gas.
We consider the superfluid phase transition that arises when a Feshbach resonance pairing occurs in a dilute Fermi gas. We apply our theory to consider a specific resonance in potassium ((40)K), and find that for achievable experimental conditions, the transition to a superfluid phase is possible at the high critical temperature of about 0.5T(F). Observation of superfluidity in this regime would provide the opportunity to experimentally study the crossover from the superfluid phase of weakly coupled fermions to the Bose-Einstein condensation of strongly bound composite bosons.