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arXiv:cond-mat/0311085 · Physical Review B

Quantum criticality and deconfinement in phase transitions between valence bond solids

Ashvin Vishwanath, Leon Balents, T. Senthil

Published Jun 30, 2004• 141 citations
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Abstract

We consider spin-half quantum antiferromagnets in two spatial dimensions in the quantum limit, where the spins are in a valence bond solid (VBS) phase. The transition between two such VBS phases is studied. In some cases, an interesting second-order transition controlled by a fixed line with varying critical exponents is found. A specific example is provided by an antiferromagnetically coupled bilayer system on the honeycomb lattice where a continuous quantum phase transition can generically exist between two VBS phases. Furthermore, these critical points are deconfined, in the sense that gapped spin-$1∕2$ spinon excitations emerge right at the transition. The low-energy physics of this critical point (up to marginally irrelevant interactions) contains just a free quadratically dispersing ``photon.'' The phase structure on one side of this continuous transition is very intricate, consisting of a series of infinitely closely spaced further transitions in a ``devil's staircase'' form. Analogies with previous examples of deconfined quantum criticality are emphasized. Closely related transitions in single layer systems are explored. These are second order only at some multicritical points. The solvable Rokshar-Kivelson point of quantum dimer models of single layer systems is found to correspond to a nongeneric multicritical point.

DOI
10.1103/physrevb.69.224416

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We consider spin-half quantum antiferromagnets in two spatial dimensions in the quantum limit, where the spins are in a valence bond solid (VBS) phase. The transition between two such VBS phases is studied. In some cases, an interesting second-order transition controlled by a fixed line with varying critical exponents is found. A specific example is provided by an antiferromagnetically coupled bilayer system on the honeycomb lattice where a continuous quantum phase transition can generically exist between two VBS phases. Furthermore, these critical points are deconfined, in the sense that gapped spin-1∕21∕21∕2 spinon excitations emerge right at the transition. The low-energy physics of this critical point (up to marginally irrelevant interactions) contains just a free quadratically dispersing photon.'' The phase structure on one side of this continuous transition is very intricate, consisting of a series of infinitely closely spaced further transitions in a devil's staircase'' form. Analogies with previous examples of deconfined quantum criticality are emphasized. Closely related transitions in single layer systems are explored. These are second order only at some multicritical points. The solvable Rokshar-Kivelson point of quantum dimer models of single layer systems is found to correspond to a nongeneric multicritical point.
We perform a numerical study of a spin-1/2 model with ${\mathbb{Z}}_{2}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{2}$ symmetry in one dimension which demonstrates an interesting similarity to the physics of two-dimensional deconfined quantum critical points (DQCP). Specifically, we investigate the quantum phase transition between Ising ferromagnetic and valence bond solid (VBS) symmetry-breaking phases. Working directly in the thermodynamic limit using uniform matrix product states, we find evidence for a direct continuous phase transition that lies outside of the Landau-Ginzburg-Wilson paradigm. In our model, the continuous transition is found everywhere on the phase boundary. We find that the magnetic and VBS correlations show very close power-law exponents, which is expected from the self-duality of the parton description of this DQCP. Critical exponents vary continuously along the phase boundary in a manner consistent with the predictions of the field theory for this transition. We also find a regime where the phase boundary splits, as suggested by the theory, introducing an intermediate phase of coexisting ferromagnetic and VBS order parameters. Interestingly, we discover a transition involving this coexistence phase which is similar to the DQCP, being also disallowed by the Landau-Ginzburg-Wilson symmetry-breaking theory.
Deconfined quantum critical points (DQCPs) are putative phase transitions beyond the Landau paradigm with emergent fractionalized degrees of freedom. The original example of a DQCP is the spin-12\frac{1}{2}21​ quantum antiferromagnet on the square lattice which features a second-order transition between valence bond solid (VBS) and N\'eel order. The VBS order breaks a lattice symmetry, and the corresponding VBS order parameter may couple to lattice distortion modes (phonons) at appropriate momenta. We investigate a field-theoretic description of the DQCP in the presence of such a spin-lattice coupling. We show that treating phonons as classical lattice distortions leads to a relevant monopole-phonon interaction inducing an instability towards a distorted lattice by an analogous mechanism to the spin-Peierls instability in one dimension. Consequently, there is a breakdown of the DQCP which generally becomes a strong first-order transition. Taking into account the full quantum nature of the phonons, we argue that the continuous DQCP persists above a critical phonon frequency. Lastly, we comment on the connection to general gapless, deconfined gauge theories.
We study a spin-1/2 SU(2) model on the honeycomb lattice with nearest-neighbor antiferromagnetic exchange J that favors Néel order and competing six-spin interactions Q that favor a valence-bond-solid (VBS) state in which the bond energies order at the "columnar" wave vector K=(2π/3,-2π/3). We present quantum Monte Carlo evidence for a direct continuous quantum phase transition between Néel and VBS states, with exponents and logarithmic violations of scaling consistent with those at analogous deconfined critical points on the square lattice. Although this strongly suggests a description in terms of deconfined criticality, the measured threefold anisotropy of the phase of the VBS order parameter shows unusual near-marginal behavior at the critical point.
We discuss zero‐temperature phase transititions from an antiferromagnetic ground state into a valence‐bond‐solid (VBS) in two different square‐lattice quantum spin models. In one limit these models reduce to the standard S = 1/2 XY and Heisenberg models, respectively, which have long‐range antiferromagnetic order at T = 0. Introducing particular types of four‐spin interactions, amenable to quantum Monte Carlo (QMC) simulation without negative‐sign problems, drives phase transitions into VBS states with broken Z4 symmetry. It has recently been argued that continuous quantum phase transitions of this nature represent a new class of deconfined quantum‐critical points [Senthil et al., Science 303, 1490 (2004)], which are not captured within the standard Ginzburg‐Landau framework of phase transitions. Here we discuss a QMC study aimed at accurately characterizing the transition in the XY model. We find some evidence that the transition is actually weakly first‐order, but other scenarios, such as a continuous transition violating hyperscaling, also cannot be completely ruled out. For the Heisenberg model with four‐spin interactions we have confirmed that a VBS state exists. Preliminary finite‐size scaling results show consistency with a continuous transition into the Néel state, with dynamic exponent z = 1. This model is thus a candidate for deconfined quantum criticality.
We report large-scale quantum Monte Carlo calculations at the T=0 antiferromagnetic to valence-bond-solid (VBS) transition of a two-dimensional S=1/2 XY model with four-spin interactions. Finite-size scaling suggests a discontinuous spin stiffness, but a continuous VBS order-parameter. We propose that this is a continuous VBS transition without critical spin fluctuations. We also argue that the system is close to a point, in an extended parameter space, where both the magnetic and VBS fluctuations are critical--possibly a deconfined quantum-critical point.
We continue recent efforts to discover examples of deconfined quantum criticality in one-dimensional models. In this work we investigate the transition between a Z3{\mathbb{Z}}_{3}Z3​ ferromagnet and a phase with valence bond solid (VBS) order in a spin chain with ${\mathbb{Z}}_{3}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{3}$ global symmetry. We study a model with alternating projective representations on the sites of the two sublattices, allowing the Hamiltonian to connect to an exactly solvable point having VBS order with the character of SU(3)SU(3)SU(3)-invariant singlets. Such a model does not admit a Lieb-Schultz-Mattis theorem typical of systems realizing deconfined critical points. Nevertheless, we find evidence for a direct transition from the VBS phase to a Z3{\mathbb{Z}}_{3}Z3​ ferromagnet. Finite-entanglement scaling data are consistent with a second-order or weakly first-order transition. We find in our parameter space an integrable lattice model apparently describing the phase transition, with a very long, finite, correlation length of 190878 lattice spacings. Based on exact results for this model, we propose that the transition is extremely weakly first order and is part of a family of deconfined quantum critical points described by walking of renormalization group flows.