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arXiv:cond-mat/0305165 · Physical Review B

Resonant nature of phonon-induced damping of Rabi oscillations in quantum dots

Paweł Machnikowski, Lucjan Jacak

Published May 4, 2004• 110 citations
arXivHTMLPDF

Abstract

Optically controlled coherent dynamics of charge (excitonic) degrees of freedom in a semiconductor quantum dot under the influence of lattice dynamics (phonons) is discussed theoretically. We show that the dynamics of the lattice response in the strongly nonlinear regime is governed by a semiclassical resonance between the phonon modes and the optically driven dynamics. We stress on the importance of the stability of intermediate states for the truly coherent control.

DOI
10.1103/physrevb.69.193302

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Optically controlled coherent dynamics of charge (excitonic) degrees of freedom in a semiconductor quantum dot under the influence of lattice dynamics (phonons) is discussed theoretically. We show that the dynamics of the lattice response in the strongly nonlinear regime is governed by a semiclassical resonance between the phonon modes and the optically driven dynamics. We stress on the importance of the stability of intermediate states for the truly coherent control.
We show that the interaction between carriers confined in a quantum dot and the surrounding lattice under external driving of carrier dynamics has a dynamical, resonant character. The quality of Rabi oscillations in such a system depends on the relation between nonlinear spectral characteristics of the driven dynamics and the spectral density of effectively coupled lattice modes (phonon frequencies and density of states). For a large number of Rabi oscillations within a fixed time (allowed by, e.g., exciton recombination) the spectrum of the dynamics extends towards high frequencies, coming into resonance with acoustic and optical phonons. Thus, this resonant lattice response strongly restricts the possibility of fully coherent control over the charge state in a quantum dot.
This chapter is devoted to the recent theoretical results on the optical quantum control over charges confined in quantum dots under influence of phonons. We show that lattice relaxation processes lead to decoherence of the confined carrier states. The theoretical approach leading to a uniform, compact description of the phonon impact on carrier dynamics, perturbative in phonon couplings but applicable to arbitrary unperturbed evolution, is described in detail. Next, some applications are presented: phonon damping of Rabi oscillations in quantum dots and phonon-induced error of a single-qubit gate for an excitonic quantum dot qubit as well as for a semiconductor quantum dot spin qubit operated via a STIRAP transfer.
Electron-phonon interaction is a major source of optical dephasing in semiconductor quantum dots. Within a density matrix theory the electron-phonon interaction is considered up to the second order of a correlation expansion, allowing the calculation of the quantum kinetic dephasing dynamics of optically induced nonlinearities in GaAs quantum dots for arbitrary pulse strengths and shapes. We find Rabi oscillations renormalized and a damping that depends on the input pulse strength, a behavior not known from exponential dephasing mechanisms.
The effect of strong exciton-phonon interaction on the excitonic Rabi oscillations in a coherently driven quantum dot in a high-Q single mode cavity is investigated theoretically. We show that the Rabi oscillation of exciton dressed by phonons can persists with the Rabi frequency ge -λ/2 at absolute zero temperature, where g is the single-photon Rabi frequency and λ is the Huang-Rhys factor. The results also present that such coherent oscillations can be modified by manipulating the Rabi frequency of the driving field.