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arXiv:cond-mat/0304489 · Physical Review Letters

Molecular Kondo Resonance in Atomic Fermi Gases

G. M. Falco, R. A. Duine, Henk T. C. Stoof

Published Apr 8, 2004• 30 citations
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Abstract

The usual Kondo effect is associated with the formation of a many-body ground state that contains a quantum-mechanical entanglement between a (localized) fermion and the free fermions. We show, however, that also a bosonic form of the Kondo effect can occur in degenerate atomic Fermi gases near a Feshbach resonance, if the energy of the diatomic molecular level associated with the Feshbach resonance approaches twice the Fermi energy of the atoms.

DOI
10.1103/physrevlett.92.140402

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The usual Kondo effect is associated with the formation of a many-body ground state that contains a quantum-mechanical entanglement between a (localized) fermion and the free fermions. We show, however, that also a bosonic form of the Kondo effect can occur in degenerate atomic Fermi gases near a Feshbach resonance, if the energy of the diatomic molecular level associated with the Feshbach resonance approaches twice the Fermi energy of the atoms.
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The use of Feshbach resonances for tuning the interparticle interaction in ultracold Fermi gases has led to remarkable developments, in particular to the creation and Bose-Einstein condensation of weakly bound diatomic molecules of fermionic atoms.These are the largest diatomic molecules obtained so far, with a size of the order of thousands of angstroms.They represent novel composite bosons, which exhibit features of Fermi statistics at short intermolecular distances.Being highly excited, these molecules are remarkably stable with respect to collisional relaxation, which is a consequence of the Pauli exclusion principle for identical fermionic atoms.The purpose of this review is to introduce theoretical approaches and describe the physics of molecular regimes in two-component Fermi gases and Fermi-Fermi mixtures, focusing attention on quantum statistical effects.
We propose a simple but novel scheme to realize the Kondo effect with ultracold atoms. Our system consists of a Fermi sea of spinless fermions interacting with an impurity atom of different species which is confined by an isotropic potential. The interspecies attraction can be tuned with an s-wave Feshbach resonance so that the impurity atom and a spinless fermion form a bound dimer that occupies a threefold-degenerate p orbital of the confinement potential. Many-body scatterings of this dimer and surrounding spinless fermions occur with exchanging their angular momenta and thus exhibit the SU(3) orbital Kondo effect. The associated Kondo temperature has a universal leading exponent given by TK∝exp[-π/(3apkF3)] that depends only on an effective p-wave scattering volume ap and a Fermi wave vector kF. We also elucidate a Kondo singlet formation at zero temperature and an anisotropic interdimer interaction mediated by surrounding spinless fermions. The Kondo effect thus realized in ultracold atom experiments may be observed as an increasing atom loss by lowering the temperature or with radio-frequency spectroscopy. Our scheme and its extension to a dense Kondo lattice will be useful to develop new insights into yet unresolved aspects of Kondo physics.
For calculating low-energy properties of a dilute gas of atoms interacting via a Feshbach resonance, we develop an effective theory in which the parameters that enter are an atom-molecule coupling strength and the magnetic moment of the molecular resonance. We demonstrate that, for resonances in the fermionic systems 6Li and 40K that are under experimental investigation, the coupling is so strong that many-body effects are appreciable even when the resonance lies at an energy large compared with the Fermi energy. We calculate a number of many-body effects, including the effective mass and the lifetime of atomic quasiparticles in the gas.
We propose a novel realization of Kondo physics with ultracold atomic gases. It is based on a Fermi sea of two different hyperfine states of one atom species forming bound states with a different species, which is spatially confined in a trapping potential. We show that different situations displaying Kondo physics can be realized when Feshbach resonances between the species are tuned by a magnetic field and the trapping frequency is varied. We illustrate that a mixture of 40K and 23Na atoms can be used to generate a Kondo-correlated state and that momentum resolved radio frequency spectroscopy can provide unambiguous signatures of the formation of Kondo resonances at the Fermi energy. We discuss how tools of atomic physics can be used to investigate open questions for Kondo physics, such as the extension of the Kondo screening cloud.