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arXiv:cond-mat/0303112 · Europhysics Letters (EPL)

Spectral scaling and quantum critical behaviour in the pseudogap Anderson model

Matthew T. Glossop, David E. Logan

Published Mar 1, 2003• 19 citations
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Abstract

The pseudogap Anderson impurity model provides a classic example of an essentially local quantum phase transition. Here we study its single-particle dynamics in the vicinity of the symmetric quantum critical point (QCP) separating generalized Fermi-liquid and local-moment phases, via the local-moment approach. Both phases are shown to be characterized by a low-energy scale that vanishes at the QCP; and the universal scaling spectra, on all energy scales, are obtained analytically. The spectrum precisely at the QCP is also obtained; its form showing clearly the non–Fermi-liquid, interacting nature of the fixed point.

DOI
10.1209/epl/i2003-00306-3

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The pseudogap Anderson impurity model provides a classic example of an essentially local quantum phase transition. Here we study its single-particle dynamics in the vicinity of the symmetric quantum critical point (QCP) separating generalized Fermi-liquid and local-moment phases, via the local-moment approach. Both phases are shown to be characterized by a low-energy scale that vanishes at the QCP; and the universal scaling spectra, on all energy scales, are obtained analytically. The spectrum precisely at the QCP is also obtained; its form showing clearly the non–Fermi-liquid, interacting nature of the fixed point.
The pseudogap Anderson impurity model provides a paradigm for understanding local quantum phase transitions, in this case between generalised Fermi liquid (GFL) and degenerate local moment phases. Here we develop a non-perturbative local moment approach to the generic asymmetric model, encompassing all energy scales and interaction strengths and leading thereby to a rich description of the problem. We investigate in particular underlying phase boundaries, the critical behaviour of relevant low-energy scales, and single-particle dynamics embodied in the local spectrum D (ω). Particular attention is given to the resultant universal scaling behaviour of dynamics close to the transition in both the GFL and LM phases, the scale-free physics characteristic of the quantum critical point itself, and the relation between the two.
We study correlated quantum impurity models that undergo a local quantum phase transition (QPT) from a strong coupling, Fermi liquid phase to a non-Fermi liquid phase with a globally doubly degenerate ground state. Our aim is to establish what can be shown exactly about such ``local moment'' (LM) phases, of which the permanent (zero-field) local magnetization is a hallmark, and an order parameter for the QPT. A description of the zero-field LM phase is shown to require two distinct self-energies, which reflect the broken symmetry nature of the phase and together determine the single self-energy of standard field theory. Distinct Friedel sum rules for each phase are obtained, via a Luttinger theorem embodied in the vanishing of appropriate Luttinger integrals. By contrast, the standard Luttinger integral is nonzero in the LM phase but found to have universal magnitude. A range of spin susceptibilites are also considered, including that corresponding to the local order parameter, whose exact form is shown to be RPA-like, and to diverge as the QPT is approached. Particular attention is given to the pseudogap Anderson model, including the basic physical picture of the transition, the low-energy behavior of single-particle dynamics, the quantum critical point itself, and the rather subtle effect of an applied local field. A two-level impurity model that undergoes a QPT (``singlet-triplet'') to an underscreened LM phase is also considered, for which we derive on general grounds some key results for the zero-bias conductance in both phases.
Local quantum criticality in itinerant fermion systems has been extensively investigated through the soft-gap Anderson impurity model, wherein a localized, correlated impurity hybridizes with a broad conduction band with a singular, ${|\ensuremath{\omega}|}^{r}$, density of states. However, lattice models hosting quantum critical points (QCPs) do not appear to have such a spectrum emerging at the QCP. In this work, we report the emergence of such a singular form of the density of states in a three-orbital lattice model, within dynamical mean field theory, precisely at a quantum critical point, separating a gapless, Fermi liquid (FL) metallic phase from a gapped, Mott insulating phase. A temperature-dependent exponent, $\ensuremath{\alpha}$, defined using the corresponding Matsubara self-energy, is found to vary from +1+1+1 deep in the FL regime, to $\ensuremath{-}1$ in the Mott insulator regime. Interestingly, we find that $\ensuremath{\alpha}$ becomes temperature-independent, and hence isosbestic, precisely at the QCP. The isosbestic exponent is shown to lead to an emergent soft-gap spectrum, ${|\ensuremath{\omega}|}^{r}$, at the QCP, where $r=|{\ensuremath{\alpha}}_{\mathrm{iso}}|$. We discuss the implications of our findings for non-Fermi-liquid behavior in the quantum critical region of the phase diagram.
The symmetric Anderson impurity model with a hybridization vanishing at the Fermi level, Δ I ∝|ω| r , is studied via the numerical renormalization group (NRG) at T = 0; and detailed comparison made with predictions arising from the local moment approach (LMA), a recently developed many-body theory which is found to provide a remarkably successful description of the problem. Results for the `normal' ( r = 0) impurity model are obtained as a specific case, and likewise compared. Particular emphasis is given both to single-particle excitation dynamics, and to the transition between the strong-coupling (SC) and local moment (LM) phases of the model. Scaling characteristics and asymptotic behaviour of the SC/LM phase boundaries are considered. Single-particle spectra D (ω) are investigated in some detail, for the SC phase in particular. Here, in accordance with a recently established result, the modified spectral functions ℱ(ω)∝|ω| r D (ω) are found to contain a generalized Kondo resonance that is ubiquitously pinned at the Fermi level; and which exhibits a characteristic low-energy Kondo scale, ω K ( r ), that narrows progressively upon approach to the SC→LM transition, where it vanishes. Universal scaling of the spectra as the transition is approached thus results. The scaling spectrum characteristic of the normal Anderson model is recovered as a particular case, that exemplifies behaviour characteristic of the SC phase generally, and which is captured quantitatively by the LMA. In all cases the r -dependent scaling spectra are found to possess characteristic low-energy asymptotics, but to be dominated by generalized Doniach-Sunjic tails, in agreement with LMA predictions.
The quantum criticality of the two-lead two-channel pseudogap Anderson impurity model is studied. Based on the non-crossing approximation (NCA) and numerical renormalization group (NRG) approaches, we calculate both the linear and nonlinear conductance of the model at finite temperatures with a voltage bias and a power-law vanishing conduction electron density of states, ρc(ω) proportional |ω − μF|(r) (0 < r < 1) near the Fermi energy μF. At a fixed lead-impurity hybridization, a quantum phase transition from the two-channel Kondo (2CK) to the local moment (LM) phase is observed with increasing r from r = 0 to r = rc < 1. Surprisingly, in the 2CK phase, different power-law scalings from the well-known [Formula: see text] or [Formula: see text] form is found. Moreover, novel power-law scalings in conductances at the 2CK-LM quantum critical point are identified. Clear distinctions are found on the critical exponents between linear and non-linear conductance at criticality. The implications of these two distinct quantum critical properties for the non-equilibrium quantum criticality in general are discussed.
A local moment approach is developed for single-particle excitations of a symmetric Anderson impurity model (AIM) with a soft-gap hybridization vanishing at the Fermi level: I | | r , with r >0. Local moments are introduced explicitly from the outset, and a two-self-energy description is employed in which single-particle excitations are coupled dynamically to low-energy transverse spin fluctuations. The resultant theory is applicable on all energy scales, and captures both the spin-fluctuation regime of strong coupling (large U ), as well as the weak-coupling regime where it is perturbatively exact for those r -domains in which perturbation theory in U is non-singular. While the primary emphasis is on single-particle dynamics, the quantum phase transition between strong-coupling (SC) and local moment (LM) phases can also be addressed directly; for the spin-fluctuation regime in particular a number of asymptotically exact results are thereby obtained, notably for the behaviour of the critical U c ( r ) separating SC/LM states and the Kondo scale m ( r ) characteristic of the SC phase. Results for both single-particle spectra and SC/LM phase boundaries are found to agree well with recent numerical renormalization group (NRG) studies; and a number of further testable predictions are made. Single-particle spectra are examined systematically for both SC and LM states; in particular, for all 0 r <½, spectra characteristic of the SC state are predicted to exhibit an r -dependent universal scaling form as the SC/LM phase boundary is approached and the Kondo scale vanishes. Results for the `normal' r = 0 AIM are moreover recovered smoothly from the limit r 0, where the resultant description of single-particle dynamics includes recovery of Doniach-Sunjic tails in the wings of the Kondo resonance, as well as characteristic low-energy Fermi liquid behaviour and the exponential diminution with U of the Kondo scale itself. The normal AIM is found to represent a particular case of more generic behaviour characteristic of the r >0 SC phase which, in agreement with conclusions drawn from recent NRG work, may be viewed as a non-trivial but natural generalization of Fermi liquid physics.