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arXiv:cond-mat/0302334 · Physical review. B, Condensed matter

Orbital Kondo behavior from dynamical structural defects

L. Borda, A. Zawadowski, Gergely Zaránd

Published Jul 29, 2003• 14 citations
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Abstract

The interaction between an atom moving in a model double-well potential and the conduction electrons is treated using renormalization-group methods in next-to-leading logarithmic order. A large number of excited states is taken into account and the Kondo temperature ${T}_{K}$ is computed as a function of barrier parameters. We find that for special parameters ${T}_{K}$ can be close to 1 K and it can be of the same order of magnitude as the renormalized splitting $\ensuremath{\Delta}.$ However, in the perturbative regime we always find that ${T}_{K}\ensuremath{\lesssim}\ensuremath{\Delta}$ with ${T}_{K}\ensuremath{\lesssim}1\mathrm{K}$ [I. L. Aleiner et al., Phys. Rev. Lett. 86, 2629 (2001)]. We also find that $\ensuremath{\Delta}$ remains unrenormalized at energies above the Debye frequency, ${\ensuremath{\omega}}_{\mathrm{Debye}}.$

DOI
10.1103/physrevb.68.045114

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Correlations are a central ingredient of modern condensed matter physics. With the advent of mesoscopic physics, it became possible to study correlated systems in non-equilibrium situations, which can be reached by e.g. driving a constant current through a quantum dot. A basic question is how correlations on the one hand and a non-equilibrium current on the other hand influence each other. Here this interplay is studied for the model system of a quantum dot in the Kondo regime using the real time renormalization group (RTRG) method. This method is a functional renormalization group (RG) method allowing a non-perturbative description of correlated systems in non-equilibrium. For the Kondo quantum dot the method is generalized to the case of double vertices. The RTRG method not only provides equations for the calculation of the renormalized coupling between the quantum dot spin and the reservoir electrons, but also equations for the calculation of the non-equilibrium decoherence rate and the non-equilibrium current.The RG equations are derived to second order. This approximation is expected to be valid as long as the quantum dot does not enter the strong coupling regime, i.e. the effective coupling strength between the quantum dot spin and the electrons does not become too large. It is found that this is the case if the bias voltage applied to the dot or the temperature is much larger than the Kondo temperature.It is shown that the RG equations lead to coupling functions depending on the energy of the incident and the scattered electron. This dependence is simplified to the dependence on the average energy of the incident and the scattered electron in the weak coupling regime.A closer inspection of the RG equations for the couplings shows that they not only contain terms leading to a logarithmic increase of the coupling strength but also subleading terms which are unimportant in the weak coupling regime. The RG equations are solved analytically for the case where the subleading terms are neglected. It is found that the coupling functions develop resonances at energies associated with the chemical potentials of the reservoirs. The height of these resonances is determined by the decoherence rate. However, for bias voltages much larger than the Kondo temperature these resonances do not affect the conductance for a two terminal setup, so the conductance does not provide a measure for the decoherence rate in this case. It is found that the conductance for the two terminal setup is a universal function of voltage/Kondo temperature and temperature/Kondo temperature in the weak coupling regime. This function is calculated analytically in the limits of vanishing voltage or temperature. Furthermore, it is found that for zero temperature the decoherence rate is proportional to the non-equilibrium current flowing through the system. This supports the physical picture that a non-equilibrium current is associated with a decoherence rate, which cuts the logarithmic scaling of the coupling strength.Finally, the RG equations are solved numerically for zero temperature including the subleading corrections found before. As expected, the subleading corrections have no impact on the decoherence rate and the conductance in the weak coupling regime. On the other hand, it is found that they lead to strong deviations from the results of the analytic leading logarithmic approximation if the bias voltage approaches the Kondo temperature. Generally, it is found that the subleading corrections lead to a saturation of the decoherence rate and the conductance to some finite value. However, for the numerical solution a numerical regularization parameter has to be introduced. It turns out that the saturation value found depends on its value, so no statements on the precise value of the decoherence rate and the current can be made in this regime.

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The interaction between an atom moving in a model double-well potential and the conduction electrons is treated using renormalization-group methods in next-to-leading logarithmic order. A large number of excited states is taken into account and the Kondo temperature TK{T}_{K}TK​ is computed as a function of barrier parameters. We find that for special parameters TK{T}_{K}TK​ can be close to 1 K and it can be of the same order of magnitude as the renormalized splitting \ensuremathΔ.\ensuremath{\Delta}.\ensuremathΔ. However, in the perturbative regime we always find that TK\ensuremath≲\ensuremathΔ{T}_{K}\ensuremath{\lesssim}\ensuremath{\Delta}TK​\ensuremath≲\ensuremathΔ with TK\ensuremath≲1K{T}_{K}\ensuremath{\lesssim}1\mathrm{K}TK​\ensuremath≲1K [I. L. Aleiner et al., Phys. Rev. Lett. 86, 2629 (2001)]. We also find that \ensuremathΔ\ensuremath{\Delta}\ensuremathΔ remains unrenormalized at energies above the Debye frequency, \ensuremathωDebye.{\ensuremath{\omega}}_{\mathrm{Debye}}.\ensuremathωDebye​.
We consider an atom in a double-well potential [parametrized by a two-level system (TLS)] interacting with screened conduction electrons. The tunneling of the TLS is assisted by the Fermi gas. Close to the strong-coupling fixed point the renormalization-group equations for the noncommutative model in the case of spinless fermions, but an arbitrary number of relevant orbital channels, lead to the n-channel Kondo problem with S=1/2. By solving the thermodynamic Bethe-ansatz equations for the n-channel Kondo problem numerically in the presence of a magnetic field, we discuss the low-temperature properties of the TLS close to the fixed point. The Zeeman splitting corresponds to the energy difference between the two positions of the tunneling atom. The atom is not localized at one of the potential minima. The susceptibility diverges as H\ensuremath{\rightarrow}0 and T\ensuremath{\rightarrow}0, indicating that the symmetric TLS is unstable against a local lattice deformation via coupling to phonons. The lattice distortion disappears above a critical temperature Tc{\mathit{T}}_{\mathit{c}}Tc​. The ground-state equilibrium situation of the TLS corresponds to H\ensuremath{\ne}0 and a Fermi-liquid picture applies. The values for the specific heat become very large as H\ensuremath{\rightarrow}0. For small fields the specific heat shows a double-peak structure, which is particularly pronounced for n=2.
The two-channel Kondo (2CK) effect with its exotic ground state properties has remained difficult to realize in physical systems. At low energies, a quantum impurity with orbital degree of freedom, like a proton bound in an interstitial lattice space, comprises a 3-level system with a unique ground state and (at least) doubly degenerate rotational excitations with excitation energy Delta0Delta_0Delta0​. When immersed in a metal, electronic angular momentum scattering induces transitions between any two of these levels (couplings JJJ), while the electron spin is conserved. We show by extensive numerical renormalization group (NRG) calculations that without fine-tuning of parameters this system exhibits a 2CK fixed point, due to Kondo correlations in the excited-state doublet whose degeneracy is stabilized by the host lattice parity, while the channel symmetry (electron spin) is guaranteed by time reversal symmetry. We find a pronounced plateau in the entropy at S(TK<T<Delta0)=kBln2S(T_K < T < Delta_0) = k_B ln 2S(TK​<T<Delta0​)=kB​ln2 between the high-TTT value, S(TggDelta0)=kBln3S(T gg Delta_0) = k_B ln 3S(TggDelta0​)=kB​ln3, and the 2CK ground state value, S(0)=kBlnsqrt2S(0) = k_B lnsqrt{2}S(0)=kB​lnsqrt2. This indicates a downward renormalization of the doublet below the non-interacting ground state, thus realizing the 2CK fixed point, in agreement with earlier conjectures. We mapped out the phase diagram of the model in the J−Delta0J-Delta_0J−Delta0​ plane. The Kondo temperature TKT_KTK​ shows non-monotonic JJJ-dependence, characteristic for 2CK systems.newline indent Beside the two-channel Kondo effect of the model, we also study the single-channel version, which is realized by applying a strong magnetic field to the conduction band electrons so that their degeneracy is lifted and consequently having only one kind of electrons scattering off the impurity. This single-channel case is easier to analyze since the Hilbert space is not as large as that of the 2CK. We equally find a downward renormalization of the excited state energy by the Kondo correlations in the SU(2) doublet. In a wide range of parameter values this stabilizes the single-channel Kondo fixed point and a phase diagram is also mapped out for the model. In the single-channel version a plateau is found in the entropy at S(TK<T<Delta0)=kBln2S(T_K < T < Delta_0) = k_B ln 2S(TK​<T<Delta0​)=kB​ln2 between high-TTT value, S(TggDelta0)=kBln3S(T gg Delta_0) = k_B ln 3S(TggDelta0​)=kB​ln3, and the single-channel Kondo ground state value, S(0)=kBln1S(0) = k_B ln 1S(0)=kB​ln1.
A detailed and comprehensive study of the one-impurity multichannel Kondo model is presented. In the limit of a large number of conduction electron channels k>>1, the low-energy fixed point is accessible to a renormalization group improved perturbative expansion in 1/k. This straightforward approach enables us to examine the scaling, thermodynamics and dynamical response functions in great detail and make clear the following features: (i) the criticality of the fixed point, (ii) the universal non-integer degeneracy, and (iii) that the compensating spin cloud has a spatial extent of the order of one lattice spacing.
We investigate the low-temperature dynamics of single electron boxes and transistors close to their degeneracy point using renormalization-group methods. We show that intermode scattering is a relevant perturbation and always drives the system to the two-channel Kondo fixed point, where the two channels correspond to the real spins of the conduction electrons. However, the crossover temperature T∗,{T}^{*},T∗, below which Matveev's two-channel Kondo scenario [K.A. Matveev, Phys. Rev. B 51, 1743 (1995)] develops decreases exponentially with the number of conduction modes in the tunneling junctions and is extremely small in most cases. Above T∗{T}^{*}T∗ the ``infinite channel model'' of G. Falci, G. Sch\"on, and G.T. Zimany, Phys. Rev. Lett. 74, 3257 (1995) turns out to be a rather good approximation. We discuss the experimental limitations and suggest an experimental setup to observe the multichannel Kondo behavior.
The interaction between a tunneling atom in a double potential well and the conduction electrons of different angular momenta results in an anisotropic two-channel orbital Kondo problem, but the Kondo temperature TK{\mathit{T}}_{\mathit{K}}TK​ found earlier has always been somewhat small. That difficulty can be resolved by including some of the excited states of the atom in the well. The TK{\mathit{T}}_{\mathit{K}}TK​ calculated is around 1--10 K in agreement with experiments. The same result can be obtained even if the direct electron assisted tunneling is ignored.
Correlations are a central ingredient of modern condensed matter physics. With the advent of mesoscopic physics, it became possible to study correlated systems in non-equilibrium situations, which can be reached by e.g. driving a constant current through a quantum dot. A basic question is how correlations on the one hand and a non-equilibrium current on the other hand influence each other. Here this interplay is studied for the model system of a quantum dot in the Kondo regime using the real time renormalization group (RTRG) method. This method is a functional renormalization group (RG) method allowing a non-perturbative description of correlated systems in non-equilibrium. For the Kondo quantum dot the method is generalized to the case of double vertices. The RTRG method not only provides equations for the calculation of the renormalized coupling between the quantum dot spin and the reservoir electrons, but also equations for the calculation of the non-equilibrium decoherence rate and the non-equilibrium current.The RG equations are derived to second order. This approximation is expected to be valid as long as the quantum dot does not enter the strong coupling regime, i.e. the effective coupling strength between the quantum dot spin and the electrons does not become too large. It is found that this is the case if the bias voltage applied to the dot or the temperature is much larger than the Kondo temperature.It is shown that the RG equations lead to coupling functions depending on the energy of the incident and the scattered electron. This dependence is simplified to the dependence on the average energy of the incident and the scattered electron in the weak coupling regime.A closer inspection of the RG equations for the couplings shows that they not only contain terms leading to a logarithmic increase of the coupling strength but also subleading terms which are unimportant in the weak coupling regime. The RG equations are solved analytically for the case where the subleading terms are neglected. It is found that the coupling functions develop resonances at energies associated with the chemical potentials of the reservoirs. The height of these resonances is determined by the decoherence rate. However, for bias voltages much larger than the Kondo temperature these resonances do not affect the conductance for a two terminal setup, so the conductance does not provide a measure for the decoherence rate in this case. It is found that the conductance for the two terminal setup is a universal function of voltage/Kondo temperature and temperature/Kondo temperature in the weak coupling regime. This function is calculated analytically in the limits of vanishing voltage or temperature. Furthermore, it is found that for zero temperature the decoherence rate is proportional to the non-equilibrium current flowing through the system. This supports the physical picture that a non-equilibrium current is associated with a decoherence rate, which cuts the logarithmic scaling of the coupling strength.Finally, the RG equations are solved numerically for zero temperature including the subleading corrections found before. As expected, the subleading corrections have no impact on the decoherence rate and the conductance in the weak coupling regime. On the other hand, it is found that they lead to strong deviations from the results of the analytic leading logarithmic approximation if the bias voltage approaches the Kondo temperature. Generally, it is found that the subleading corrections lead to a saturation of the decoherence rate and the conductance to some finite value. However, for the numerical solution a numerical regularization parameter has to be introduced. It turns out that the saturation value found depends on its value, so no statements on the precise value of the decoherence rate and the current can be made in this regime.