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arXiv:cond-mat/0211367 · Europhysics Letters (EPL)

Phase space dynamics of overdamped quantum systems

Joachim Ankerhold

Published Feb 1, 2003• 19 citations
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Abstract

The phase space dynamics of dissipative quantum systems in strongly condensed phase is considered. Based on the exact path integral approach, it is shown that the Wigner transform of the reduced density matrix obeys a time evolution equation of Fokker-Planck type valid from high down to very low temperatures. The effect of quantum fluctuations is discussed and the accuracy of these findings is tested against exact data for a harmonic system.

DOI
10.1209/epl/i2003-00323-8

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The phase space dynamics of dissipative quantum systems in strongly condensed phase is considered. Based on the exact path integral approach, it is shown that the Wigner transform of the reduced density matrix obeys a time evolution equation of Fokker-Planck type valid from high down to very low temperatures. The effect of quantum fluctuations is discussed and the accuracy of these findings is tested against exact data for a harmonic system.
The phase space dynamics of dissipative quantum systems in strongly condensed phase is considered. Based on the exact path integral approach it is shown that the Wigner transform of the reduced density matrix obeys a time evolution equation of Fokker-Planck type valid from high down to very low temperatures. The effect of quantum fluctuations is discussed and the accuracy of these findings is tested against exact data for a harmonic system. Typeset using REVTEX 1 Introduction–Dynamics in strongly condensed phase can be found almost everywhere in nature, e.g. for tunnel diodes in mesoscopic physics, for macromolecules in biological and soft matter systems, and for chemical reactions, to name but a few. Associated with this bunch of realizations is a rich phenomenology comprising prominent effects such as stochastic resonance [1], resonant activation [2], transport in ratchets [3], and adiabatic
Time evolution of the expectation values of various dynamical operators of the harmonic oscillator with dissipation is analitically obtained within the framework of the Lindblad's theory for open quantum systems. We deduce the density matrix of the damped harmonic oscillator from the solution of the Fokker-Planck equation for the coherent state representation, obtained from the master equation for the density operator. The Fokker-Planck equation for the Wigner distribution function is also solved by using the Wang-Uhlenbeck method of transforming it into a linearized partial differential equation for the Wigner function, subject to either the Gaussian type or the δδδ-function type of initial conditions. The Wigner functions which we obtain are two-dimensional Gaussians with different widths.
Time evolution of the expectation values of various dynamical operators of the harmonic oscillator with dissipation is analitically obtained within the framework of the Lindblad theory for open quantum systems. We deduce the density matrix of the damped harmonic oscillator from the solution of the Fokker-Planck equation for the coherent state representation, obtained from the master equation for the density operator. The Fokker-Planck equation for the Wigner distribution function, subject to either the Gaussian type or the δδδ-function type of initial conditions, is also solved by using the Wang-Uhlenbeck method. The obtained Wigner functions are two-dimensional Gaussians with different widths.
The Schrodinger equation with Gaussian dynamic fluctuating potentials is considered. This model gives a convenient example of an open quantum system coupled to a given external environment. The evolution equations for averaged correlators are derived and it is shown that a system coupled to a thermoequilibrium environment tends asymptotically with time to a thermodynamic density matrix. At high temperatures the quantum evolution equation for the density matrix can be approximated by the quasiclassical Fokker-Planck equation. The generalisation for multiparticle systems is also given. The results are illustrated by the particular examples of coupling with phonons and of two-level systems. Finally, it is shown how the problem can be reformulated in terms of continuous stochastic evolution in the space of psi functions and a corresponding functional formalism based on the continuous Fokker-Planck equation in the space of psi functions.
In this thesis the path integral formalism is applied to the calculation of the dynamics of dissipative quantum systems. The time evolution of a system of bilinearly coupled bosonic modes is treated using the real-time path integral technique in coherent-state representation. This method is applied to a damped harmonic oscillator within the Caldeira-Leggett model. In order to get the stationary trajectories the corresponding Lagrangian function is diagonalized and then the path integrals are evaluated by means of the stationary-phase method. The time evolution of the reduced density matrix in the basis of coherent states is given in simple analytic form for weak system-bath coupling, i.e. the so-called rotating-wave terms can be evaluated exactly but the non-rotating-wave terms only in a perturbative manner. The validity range of the rotating-wave approximation is discussed from the viewpoint of spectral equations. In addition, it is shown that systems without initial system-bath correlations can exhibit initial jumps in the population dynamics even for rather weak dissipation. Only with initial correlations the classical trajectories for the system coordinate can be recovered. The path integral formalism in a combined phase-space and coherent-state representation is applied to the problem of curve-crossing dynamics. The system of interest is described by two coupled one-dimensional harmonic potential energy surfaces interacting with a heat bath. The mapping approach is used to rewrite the Lagrangian function of the electronic part of the system. Using the Feynman-Vernon influence-functional method the bath is eliminated whereas the non-Gaussian part of the path integral is treated using the perturbation theory in the small coordinate shift between potential energy surfaces. The vibrational and the population dynamics is considered in a lowest order of the perturbation. The dynamics of a Gaussian wave packet is analyzed along a one-dimensional reaction coordinate. Also the damping rate of coherence in the electronic part of the relevant system is evaluated within the ordinary and variational perturbation theory. The analytic expressions for the rate functions are obtained in the low and high temperature regimes.
The analysis of dissipative transport equations within the framework of open quantum systems with Fokker-Planck-type scattering is carried out from the perspective of a Wigner function approach. In particular, the well-posedness of the self-consistent whole-space problem in 3D is analyzed: existence of solutions, uniqueness and asymptotic behavior in time, where we adopt the viewpoint of mild solutions in this paper. Also, the admissibility of a density matrix formulation in Lindblad form with Fokker-Planck dissipation mechanisms is discussed. We remark that our solution concept allows to carry out the analysis directly on the level of the kinetic equation instead of on the level of the density operator. AMS 1991 Subject classification: 35Q40, 35S10, 81Q99, 81V99 Key words: Open quantum system, Wigner equation, large-time behavior, self-similarity. 1. Introduction This paper is concerned with the analysis of a class of dissipative quantum models that arise when considering the motio...