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arXiv:cond-mat/0209431 · Physical Review Letters

Three-Body Problem in a Dilute Bose-Einstein Condensate

Thorsten Köhler

Published Nov 1, 2002• 128 citations
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Abstract

We derive the explicit three-body contact potential for a dilute condensed Bose gas from microscopic theory. The three-body coupling constant exhibits the general form predicted by Wu [Phys. Rev. 115, 1390 (1959)]] and is determined in terms of the amplitudes of two- and three-body collisions in vacuum. In the present form, the coupling constant becomes accessible to quantitative studies which should provide the crucial link between few-body collisions and the stability of condensates with attractive two-body forces.

DOI
10.1103/physrevlett.89.210404

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We derive the explicit three-body contact potential for a dilute condensed Bose gas from microscopic theory. The three-body coupling constant exhibits the general form predicted by Wu [Phys. Rev. 115, 1390 (1959)]] and is determined in terms of the amplitudes of two- and three-body collisions in vacuum. In the present form, the coupling constant becomes accessible to quantitative studies which should provide the crucial link between few-body collisions and the stability of condensates with attractive two-body forces.
It is shown that the effective interaction strength of three bosons at small collision energies can be extracted from their wave function at zero energy. Asymptotic expansions of this wave function at large interparticle distances are derived, from which is defined a quantity DDD named three-body scattering hypervolume, which is an analog of the two-body scattering length. Given any finite-range interactions, one can thus predict the effective three-body force from a numerical solution of the Schr\"odinger equation. In this way, the constant DDD for hard-sphere bosons is computed, leading to the first complete result for the ground-state energy per particle of a dilute Bose-Einstein condensate (BEC) of hard spheres to order ${\ensuremath{\rho}}^{2}$, where $\ensuremath{\rho}$ is the number density. Effects of DDD are also demonstrated in the three-body energy in a finite box of size LLL, which is expanded to the order ${L}^{\ensuremath{-}7}$, and in the three-body scattering amplitude in vacuum. The three-body scattering amplitude calculated in this paper disagrees with an earlier calculation in the literature, because of the omission of the two-body effective range in that earlier work. Another key prediction is the condensate fractions of dilute BECs, which also disagree with an earlier work in the literature based on the effective field theory (EFT), as a result of short-range physics. An EFT prediction of the BEC ground-state energy, however, is corroborated.
This thesis is devoted to the rigorous study of dilute Bose gases with two-body and three-body interactions at zero temperature in two and three dimensions. Bose gases are many-body quantum systems composed of bosons, which notably do not obey the Pauli exclusion principle. As a consequence, at extremely low temperatures, a macroscopic fraction of the particles can occupy the same one-body quantum state. This phenomenon, known as Bose–Einstein condensation, was predicted in the 1920s by Bose and Einstein for noninteracting Bose gases, and first realised experimentally by the groups of Cornell and Wieman, and Ketterle, earning them the Nobel Prize for Physics in 2001. However, proving the occurrence of Bose–Einstein condensation in general interacting bosonic systems remains a major open problem and constitutes a central theme in this thesis. Another important property of bosonic matter is that it is generally more unstable than fermionic matter. In particular, for systems interacting via the Coulomb force, the Pauli exclusion principle is essential for explaining the stability of the second kind, which states that the energy and volume scale linearly with the number of particles. Nonetheless, bosonic systems with attractive but less singular interactions can also be stable, and the rigorous proof of this fact forms a second focus of this thesis. In three dimensions, we consider predominantly repulsive interactions. Firstly, we prove a leading order upper bound on the thermodynamic ground state energy of Bose gases with hard-core three-body interactions, which matches an existing lower bound. In addition, we obtain a simpler proof for integrable potentials. Secondly, we derive the leading order of the thermodynamic ground state energy of Bose gases with combined two-body and three-body interactions. More specifically, we show that, at the leading order, the ground state energy is entirely characterised by the scattering length of the two-body potential and the scattering hypervolume of the three-body potential. Thirdly, we study the time evolution of Bose–Einstein condensates with three-body interactions in the so-called Gross–Pitaevskii regime. We show that Bose–Einstein condensation is preserved under many-body evolution and that the condensate wavefunction evolves according to the quintic Gross–Pitaevskii equation. In particular, we show that the effective coupling constant is universal in the sense that it depends only on the scattering hypervolume of the interaction potential. As a by-product of our proof, we derive a stability of the second kind result for Bose gases with attractive two-body interactions and repulsive three-body interactions. In two dimensions, we consider trapped Bose gases with mean-field-type interactions, including the purely attractive case. We prove the stability of the second kind of the system and the convergence of the ground state energy per particle to that of a non-linear Schrödinger energy functional. As a consequence of the stability of the second kind, we also obtain Bose–Einstein condensation for the many-body ground states.
We consider a trapped dilute gas of NNN bosons in R3\mathbb{R}^3R3 interacting via a three-body interaction potential of the form N V(N1/2(x−y,x−z))N\, V(N^{1/2}(x-y,x-z))NV(N1/2(x−y,x−z)). In the limit N→∞N\to \inftyN→∞, we prove that every approximate ground state of the system is a convex superposition of minimizers of a 3D energy-critical nonlinear Schrödinger functional where the nonlinear coupling constant is proportional to the scattering energy of the interaction potential. In particular, the NNN-body ground state exhibits complete Bose--Einstein condensation if the nonlinear Schrödinger minimizer is unique up to a complex phase.
The stability of a Bose-Einstein condensed state of trapped ultra-cold atoms is investigated under the assumption of an attractive two-body and a repulsive three-body interaction. The Ginzburg-Pitaevskii-Gross (GPG) nonlinear Schrödinger equation is extended to include an effective potential dependent on the square of the density and solved numerically for the s-wave. The lowest collective mode excitations are determined and their dependences on the number of atoms and on the strength of the three-body force are studied. The addition of three-body dynamics can allow the number of condensed atoms to increase considerably, even when the strength of the three-body force is very small compared with the strength of the two-body force. We study in detail the first-order liquid-gas phase transition for the condensed state, which can happen in a critical range of the effective three-body force parameter.
The stability of a Bose–Einstein condensed state of trapped ultra-cold atoms is investigated under the assumption of an attractive two-body and a repulsive three-body interaction. The Ginzburg–Pitaevskii–Gross (GPG) nonlinear Schrödinger equation is extended to include an effective potential dependent on the square of the density and solved numerically for the s-wave. The lowest collective mode excitations are determined and their dependences on the number of atoms and on the strength of the three-body force are studied. The addition of three-body dynamics can allow the number of condensed atoms to increase considerably, even when the strength of the three-body force is very small compared with the strength of the two-body force. We study in detail the first-order liquid–gas phase transition for the condensed state, which can happen in a critical range of the effective three-body force parameter. 1.
The two- and three-body contacts are central to a set of univeral relations between microscopic few-body physics within an ultracold Bose gas and its thermodynamical properties. They may also be defined in trapped few-particle systems, which is the subject of this work. In this work, we focus on the unitary three-body problem in a trap, where interactions are as strong as allowed by quantum mechanics. We derive analytic results for the two- and three-body contacts in this regime and compare them with existing limiting expressions and previous numerical studies.