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arXiv:cond-mat/0209017

Thermal Superradiance and the Clausius-Mossotti Lorentz-Lorenz Equations

Sivasubramanian, S., A. Widom, Yogendra Narain Srivastava

Published Sep 1, 2002• 1 citation
arXivHTMLPDF

Abstract

Electric polarization phenomena in insulating systems have long been described in mean field theory by the (static) Clausius-Mossotti or (dynamic) Lorentz-Lorenz polarizabilities. It is here shown, in the strong coupling regime, that a thermodynamic phase instability exists in these models. The resulting thermodynamic phase diagram coincides with that obtained from Dicke-Preparata model of thermal superradiance.

DOI
10.48550/arxiv.cond-mat/0209017

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Electric polarization phenomena in insulating systems have long been described in mean field theory by the (static) Clausius-Mossotti or (dynamic) Lorentz-Lorenz polarizabilities. It is here shown, in the strong coupling regime, that a thermodynamic phase instability exists in these models. The resulting thermodynamic phase diagram coincides with that obtained from Dicke-Preparata model of thermal superradiance.
Electromagnetic superradiant field coherence exists in a condensed matter system if the electromagnetic field oscillators undergo a mean displacement. Transitions into thermal states with ordered superradiant phases have been shown to theoretically exist in Dicke-Preparata models. The theoretical validity of these models for condensed matter has been called into question due to non-relativistic diamagnetic terms in the electronic Hamiltonian. The microscopic bases of Dicke-Preparata thermal superradiance for realistic macroscopic systems are explored in this work. The impossibility of diaelectric correlations in condensed matter systems (via the Landau-Lifshitz theorem) provides a strong theoretical basis for understanding the physical reality of condensed matter thermodynamic superradiant phases.
In this doctoral thesis, the thermodynamic phases und phase transitions of a generalised Dicke model are studied and characterised. Both, finite and vanishing temperatures are considered. The Dicke model of quantum optics describes collective phenomena which occur when light interacts with a many-atom system. In the thermodynamic limit, a so-called Hepp–Lieb superradiant phase transition sets in. A superradiant phase develops for low temperatures or strong coupling between light and atoms, which is characterised by a macroscopic excitation of the light field and a spontaneous, collective polarisation of the atoms. This thesis discusses a generalised version of the Dicke model, which is described by a quantum mechanical system consisting of three-level atoms in Lambda-configuration and two modes of a resonator. By means of the Holstein–Primakoff transformation, the Hamiltonian of this system is written in terms of four interacting, non-linear oscillators, which can be linearised in the thermodynamic limit, yielding the ground-state energy as well as the low-energy excitations. The phase diagram consisting of two superradiant phases separated by continuous and first-order phase transitions is derived. In order to clarify the question whether or not the superradiant phase transition of this generalised Dicke model can be observed experimentally for real atoms, the significance of the diamagnetic term is discussed. In contrast to the original Dicke model, superradiant phase transitions are possible in principle. This is due to the first-order phase transitions. In addition, a no-go theorem for continuous superradiant phase transitions is presented. The argument is based on the Thomas–Reiche–Kuhn sum rule. Last, we study the superradiant phase transition of the generalised Dicke model at finite temperatures. Therefore, the partition sum is computed and analysed in the thermodynamic limit using Laplace’s method. At finite temperatures, the properties of the phase diagram and phases remain. However, here all phase transitions are of first order.
The thermodynamics and electrodynamics of the superradiant phase are analyzed on the basis of the Emeljanov-Klimontovich model by means of a mean field approach and random phase approximation. The model considers infinite modes of radiation field. The superradiant phase is characterized by a static and homogeneous Bose condensation of the transverse collective mode with zero wave vector. The thermodynamic quantities and the dispersion relations for the collective mode are obtained in closed forms. While the thermodynamic properties of the present model are the same as those of the Dicke model, the electrodynamics differs in form from the latter. A softening of the lower branch of the collective mode behaves as (T-Tc)1/2 for T>Tc, whereas for T≪Tc it obeys a law Tc-T or (Tc-T)1/2 according to the different regions of temperature and the polarizations. A light velocity is renormalized with an anisotropic constant.
Recently, Mendonça et al. [arXiv:2503.04961] investigated the Dicke-XXZ model and the Dicke-Ising model. For the latter model, their calculated quantum phase diagram contradicts claims about the existence of an intermediate phase with superradiant and antiferromagnetic order and the change in order of some phase transition lines, observed in other studies. In this comment we demonstrate that both features are indeed present in the Dicke-Ising model for the investigated parameter range in [arXiv:2503.04961].
Abstract The dynamics of the Dicke model, which describes the interaction of N two-level atoms with a resonant field mode, is studied in the presence of dissipation and in strong non-equilibrium for a moderate number of atoms. Starting from a highly excited state, it is investigated to what extent signatures of superradient phenomena known from the thermodynamic limit , namely, superradiant light emission and atom-field correlations characteristic for the superradiant phase, appear on transient time scales. Attention is also paid to subtleties of modeling dissipation in the weak coupling limit and to the dynamics in phase space. The latter allows phase space correlators to be defined as indicators for collective behavior on transient time scales. These findings may be of relevance for the realization of Dicke physics with superconducting circuits.
The possibility of the superradiant phase transition in polarizable materials described by the minimal-coupling Hamiltonian with the longitudinal dipole-dipole interaction is examined. We try to reduce the Hamiltonian into the Dicke one in the homogeneous and infinite case, and discuss the stability of normal ground state by the formalism of the Green function in the spatially inhomogeneous case. The presence of the longitudinal dipole-dipole interaction does not enable the superradiant phase transition, if the transverse and longitudinal fields are decoupled. Although the full dipole-dipole interaction can be eliminated in the electric-dipole gauge in the absence of overlap between individual atomic dipoles, we cannot reduce the Hamiltonian to the Dicke one, because the elimination is justified only if all the transverse and longitudinal fields remain. Even if the transverse and longitudinal fields are mixed in spatially inhomogeneous systems, the normal ground state is still stable if the system does not show the superradiant phase transition in the homogeneous case.