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arXiv:1406.2420 · Physical Review A

Stability of polarizable materials against superradiant phase transition

Motoaki Bamba, Tetsuo Ogawa

Published Dec 16, 2014• 50 citations
arXivHTMLPDF

Abstract

The possibility of the superradiant phase transition in polarizable materials described by the minimal-coupling Hamiltonian with the longitudinal dipole-dipole interaction is examined. We try to reduce the Hamiltonian into the Dicke one in the homogeneous and infinite case, and discuss the stability of normal ground state by the formalism of the Green function in the spatially inhomogeneous case. The presence of the longitudinal dipole-dipole interaction does not enable the superradiant phase transition, if the transverse and longitudinal fields are decoupled. Although the full dipole-dipole interaction can be eliminated in the electric-dipole gauge in the absence of overlap between individual atomic dipoles, we cannot reduce the Hamiltonian to the Dicke one, because the elimination is justified only if all the transverse and longitudinal fields remain. Even if the transverse and longitudinal fields are mixed in spatially inhomogeneous systems, the normal ground state is still stable if the system does not show the superradiant phase transition in the homogeneous case.

DOI
10.1103/physreva.90.063825

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•Jan 1, 2017•0 citations
The possibility of the superradiant phase transition in polarizable materials described by the minimal-coupling Hamiltonian with the longitudinal dipole-dipole interaction is examined. We try to reduce the Hamiltonian into the Dicke one in the homogeneous and infinite case, and discuss the stability of normal ground state by the formalism of the Green function in the spatially inhomogeneous case. The presence of the longitudinal dipole-dipole interaction does not enable the superradiant phase transition, if the transverse and longitudinal fields are decoupled. Although the full dipole-dipole interaction can be eliminated in the electric-dipole gauge in the absence of overlap between individual atomic dipoles, we cannot reduce the Hamiltonian to the Dicke one, because the elimination is justified only if all the transverse and longitudinal fields remain. Even if the transverse and longitudinal fields are mixed in spatially inhomogeneous systems, the normal ground state is still stable if the system does not show the superradiant phase transition in the homogeneous case.
In this paper, we reveal a second-order phase transition for the Dicke model with the dipole–dipole interaction between the atoms. By means of Holstein–Primakoff transformation, the energy spectra for both the normal and superradiant phases are explicitly obtained and therefore the scaling behaviour near the critical transition point can be given clearly. It is also shown that the dipole–dipole interactions between the atoms deeply affect the critical transition point, the ground-state and excitation energies and the scaled atomic inversion in the ground state.
We investigate the possibility of a Dicke-type superradiant phase transition of an atomic gas with an extended model which takes into account the short-range depolarizing interaction between atoms that approach each other as close as the atomic size scale, which interaction appears in a regularized electric-dipole picture of the QED of atoms. By using a mean-field model, we find that a critical density does indeed exist, though the atom-atom contact interaction shifts it to a higher value than that from the bare Dicke model.
The full Dicke model is composed of a single bosonic mode and an ensemble of NNN identical two-level atoms. In the model, the coupling between the bosonic mode and the atoms generates resonant and nonresonant processes. We also consider a dipole-dipole interaction between the atoms, which is able to generate entangled states in the atomic system. By assuming thermal equilibrium with a reservoir at temperature ${\ensuremath{\beta}}^{\ensuremath{-}1}$, the transition from fluorescent to superradiant phase and the quantum phase transition are investigated. It is shown that the critical behavior of the full Dicke model is not modified by the introduction of the dipole-dipole interaction.
The dissipative phase transitions in the open transverse and longitudinal Dicke-Ising model (DIM), which incorporates nearest-neighbor Ising-type spin interactions into the Dicke framework, are investigated within a mean-field approach and further validated by detailed stability analysis. While the dissipative phase diagram of the transverse DIM is only slightly shifted upward compared with its ground-state counterpart, dissipation in the longitudinal DIM stabilizes bistable nonequilibrium steady states and induces first-order phase transitions that are absent in the ground-state phase diagram. This bistable phase is characterized by the coexistence of superradiant and antiferromagnetic orders, and it converts a ground-state triple point into a tetracritical point, at which the boundaries of the first- and second-order transitions intersect. Our results reveal that the interplay among spin interactions, light-matter coupling, and dissipation supports a diverse set of nonequilibrium phase transitions and provides broad tunability of the phase diagram. These findings offer a theoretical foundation for exploring nonequilibrium physics in realistic open solid-state quantum systems.
The Dicke model generalized to the case where the dependence of the coupling constant on individual atoms is taken into account is investigated. It is shown that the generalized Dicke model exhibits a quantum phase transition from the normal phase to the superradiant phase in the thermodynamic limit, as well as the standard Dicke model. The mean photon number, the atomic inversion, the lowest excitation energy, and the entanglement entropy between the field and the atoms are evaluated analytically or numerically, and the critical behavior is examined. As a result, it turns out that the critical behavior in the generalized model is essentially the same as that in the standard model. This implies universality in the Dicke model.
In this doctoral thesis, the thermodynamic phases und phase transitions of a generalised Dicke model are studied and characterised. Both, finite and vanishing temperatures are considered. The Dicke model of quantum optics describes collective phenomena which occur when light interacts with a many-atom system. In the thermodynamic limit, a so-called Hepp–Lieb superradiant phase transition sets in. A superradiant phase develops for low temperatures or strong coupling between light and atoms, which is characterised by a macroscopic excitation of the light field and a spontaneous, collective polarisation of the atoms. This thesis discusses a generalised version of the Dicke model, which is described by a quantum mechanical system consisting of three-level atoms in Lambda-configuration and two modes of a resonator. By means of the Holstein–Primakoff transformation, the Hamiltonian of this system is written in terms of four interacting, non-linear oscillators, which can be linearised in the thermodynamic limit, yielding the ground-state energy as well as the low-energy excitations. The phase diagram consisting of two superradiant phases separated by continuous and first-order phase transitions is derived. In order to clarify the question whether or not the superradiant phase transition of this generalised Dicke model can be observed experimentally for real atoms, the significance of the diamagnetic term is discussed. In contrast to the original Dicke model, superradiant phase transitions are possible in principle. This is due to the first-order phase transitions. In addition, a no-go theorem for continuous superradiant phase transitions is presented. The argument is based on the Thomas–Reiche–Kuhn sum rule. Last, we study the superradiant phase transition of the generalised Dicke model at finite temperatures. Therefore, the partition sum is computed and analysed in the thermodynamic limit using Laplace’s method. At finite temperatures, the properties of the phase diagram and phases remain. However, here all phase transitions are of first order.