Coupled quantum dots are an example of the ubiquitous quantum double potential well. In a typical transport experiment, each quantum dot is also coupled to a continuum of states. Our approach takes this into account by using a Green’s function formalism to solve the full system. The time-dependent solution is then explored in different limiting cases. In general, a combination of coherent and incoherent behavior is observed. In the case that the coupling of each dot to the macroscopic world is equal, however, the time evolution is purely coherent. The double-well potential is one of the simplest and best understood problems in modern quantum mechanics. Its utility is likewise unparalleled. Potential applications of double-well devices have been noted in Refs. [1-5]. For such devices to be useful, an understanding of the processes which couple the microscopic device to the macroscopic environment is paramount. That is to say, the decoherence processes of such systems must be well understood. To this end, we consider a simple exactly solvable model of two coupled quantum dots. An excellent review of related systems and some approximate solutions are given in Ref. [6]. Each dot is coupled to an environment (a triple-barrier system) as in Fig. 1. The environment consists of a continuum of states, as would be appropriate for a macroscopic lead. Only one state in each quantum dot is considered, which amounts to the assumption that the tunneling parameters connecting our two states to any neglected state are much less than the energy differences with that state. The Hamiltonian of the system can be written as the sum of two terms, H = H0 + Hc. The first term, H0, represents the dynamics of the simple two-state system, H0 = ε1d † 1d1 + ε2d † 2 d2 + V (d† 1d2 + d†Coupled quantum dots are an example of the ubiquitous quantum double potential well. In a typical transport experiment, each quantum dot is also coupled to a continuum of states. Our approach takes this into account by using a Green’s function formalism to solve the full system. The time-dependent solution is then explored in different limiting cases. In general, a combination of coherent and incoherent behavior is observed. In the case that the coupling of each dot to the macroscopic world is equal, however, the time evolution is purely coherent. The double-well potential is one of the simplest and best understood problems in modern quantum mechanics. Its utility is likewise unparalleled. Potential applications of double-well devices have been noted in Refs. [1-5]. For such devices to be useful, an understanding of the processes which couple the microscopic device to the macroscopic environment is paramount. That is to say, the decoherence processes of such systems must be well understood. To this end, we consider a simple exactly solvable model of two coupled quantum dots. An excellent review of related systems and some approximate solutions are given in Ref. [6]. Each dot is coupled to an environment (a triple-barrier system) as in Fig. 1. The environment consists of a continuum of states, as would be appropriate for a macroscopic lead. Only one state in each quantum dot is considered, which amounts to the assumption that the tunneling parameters connecting our two states to any neglected state are much less than the energy differences with that state. The Hamiltonian of the system can be written as the sum of two terms, H = H0 + Hc. The first term, H0, represents the dynamics of the simple two-state system, H0 = ε1d † 1d1 + ε2d † 2 d2 + V (d† 1d2 + d†

Jan 1, 20028 citations

Time-dependent single-electron transport through quantum dots

T. Fujisawa, T. Hayashi, Satoshi Sasaki

We describe time-dependent single-electron transport through quantum dots in the Coulomb blockade regime. Coherent dynamics of a single charge qubit in a double quantum dot is discussed with full one-qubit manipulation. Strength of decoherence is controlled with the applied voltage, but uncontrolled decoherence arises from electron–phonon coupling and background fluctuations. Then energy-relaxation dynamics is discussed for orbital and spin degree of freedom in a quantum dot. The electron–phonon interaction and spin–orbit coupling can be investigated as the dissipation problem. Finally, charge detection measurement is presented for statistical analysis of single-electron tunnelling transitions and for a sensitive qubit read-out device.We describe time-dependent single-electron transport through quantum dots in the Coulomb blockade regime. Coherent dynamics of a single charge qubit in a double quantum dot is discussed with full one-qubit manipulation. Strength of decoherence is controlled with the applied voltage, but uncontrolled decoherence arises from electron–phonon coupling and background fluctuations. Then energy-relaxation dynamics is discussed for orbital and spin degree of freedom in a quantum dot. The electron–phonon interaction and spin–orbit coupling can be investigated as the dissipation problem. Finally, charge detection measurement is presented for statistical analysis of single-electron tunnelling transitions and for a sensitive qubit read-out device.

Reports on Progress in PhysicsFeb 20, 2006111 citations

Non-Markovian dynamics of charge carriers in quantum dots

E Vaz, Jordan Kyriakidis

We have investigated the dynamics of bound particles in multilevel current-carrying quantum dots. We look specifically in the regime of resonant tunnelling transport, where several channels are available for transport. Through a non-Markovian formalism under the Born approximation, we investigate the real-time evolution of the confined particles including transport-induced decoherence and relaxation. In the case of a coherent superposition between states with different particle number, we find that a Fock-space coherence may be preserved even in the presence of tunneling into and out of the dot. Real-time results are presented for various asymmetries of tunneling rates into different orbitals.We have investigated the dynamics of bound particles in multilevel current-carrying quantum dots. We look specifically in the regime of resonant tunnelling transport, where several channels are available for transport. Through a non-Markovian formalism under the Born approximation, we investigate the real-time evolution of the confined particles including transport-induced decoherence and relaxation. In the case of a coherent superposition between states with different particle number, we find that a Fock-space coherence may be preserved even in the presence of tunneling into and out of the dot. Real-time results are presented for various asymmetries of tunneling rates into different orbitals.

arXiv:0802.3928Journal of Physics Conference SeriesMar 1, 200810 citations

Time-dependent quantum transport through an interacting quantum dot beyond sequential tunneling: second-order quantum rate equations

B Dong, Guo-Hui Ding, X. L. Lei

A general theoretical formulation for the effect of a strong on-site Coulomb interaction on the time-dependent electron transport through a quantum dot under the influence of arbitrary time-varying bias voltages and/or external fields is presented, based on slave bosons and the Keldysh nonequilibrium Green's function (GF) techniques. To avoid the difficulties of computing double-time GFs, we generalize the propagation scheme recently developed by Croy and Saalmann to combine the auxiliary-mode expansion with the celebrated Lacroix's decoupling approximation in dealing with the second-order correlated GFs and then establish a closed set of coupled equations of motion, called second-order quantum rate equations (SOQREs), for an exact description of transient dynamics of electron correlated tunneling. We verify that the stationary solution of our SOQREs is able to correctly describe the Kondo effect on a qualitative level. Moreover, a comparison with other methods, such as the second-order von Neumann approach and Hubbard-I approximation, is performed. As illustrations, we investigate the transient current behaviors in response to a step voltage pulse and a harmonic driving voltage, and linear admittance as well, in the cotunneling regime.A general theoretical formulation for the effect of a strong on-site Coulomb interaction on the time-dependent electron transport through a quantum dot under the influence of arbitrary time-varying bias voltages and/or external fields is presented, based on slave bosons and the Keldysh nonequilibrium Green's function (GF) techniques. To avoid the difficulties of computing double-time GFs, we generalize the propagation scheme recently developed by Croy and Saalmann to combine the auxiliary-mode expansion with the celebrated Lacroix's decoupling approximation in dealing with the second-order correlated GFs and then establish a closed set of coupled equations of motion, called second-order quantum rate equations (SOQREs), for an exact description of transient dynamics of electron correlated tunneling. We verify that the stationary solution of our SOQREs is able to correctly describe the Kondo effect on a qualitative level. Moreover, a comparison with other methods, such as the second-order von Neumann approach and Hubbard-I approximation, is performed. As illustrations, we investigate the transient current behaviors in response to a step voltage pulse and a harmonic driving voltage, and linear admittance as well, in the cotunneling regime.

arXiv:1411.5747Journal of Physics Condensed MatterMay 6, 201510 citations

Out-of-Equilibrium Kondo Effect in Double Quantum Dots

Ramón Aguado, David C. Langreth

The out-of-equilibrium transport properties of a double quantum dot system in the Kondo regime are studied theoretically by means of a two-impurity Anderson Hamiltonian with interimpurity hopping. The Hamiltonian is solved by means of a nonequilibrium generalization of the slave-boson mean-field theory. It is demonstrated that measurements of the differential conductance dI/dV, for appropriate values of voltages and tunneling couplings, can give a direct observation of the coherent superposition between the many-body Kondo states of each dot. For large voltages and arbitrarily large interdot tunneling, there is a critical voltage above which the physical behavior of the system again resembles that of two decoupled quantum dots.The out-of-equilibrium transport properties of a double quantum dot system in the Kondo regime are studied theoretically by means of a two-impurity Anderson Hamiltonian with interimpurity hopping. The Hamiltonian is solved by means of a nonequilibrium generalization of the slave-boson mean-field theory. It is demonstrated that measurements of the differential conductance dI/dV, for appropriate values of voltages and tunneling couplings, can give a direct observation of the coherent superposition between the many-body Kondo states of each dot. For large voltages and arbitrarily large interdot tunneling, there is a critical voltage above which the physical behavior of the system again resembles that of two decoupled quantum dots.

arXiv:cond-mat/9912376Physical Review LettersAug 28, 2000218 citations

Synchronized coherent charge oscillations in coupled double quantum dots

Eric Kleinherbers, Philipp Stegmann, Jürgen König

We study coherent charge oscillations in double quantum dots tunnel coupled to metallic leads. If two such systems are coupled by Coulomb interaction, there are, in total, six (instead of only two) oscillation modes of the entangled system with interaction-dependent oscillation frequencies. By tuning the bias voltage, one can engineer decoherence such that only one of the six modes, in which the charge oscillations in both double quantum dots become synchronized in antiphase, is singled out. We suggest using waiting-time distributions and the ${g}^{(2)}$ -correlation function to detect the common frequency and the phase locking.We study coherent charge oscillations in double quantum dots tunnel coupled to metallic leads. If two such systems are coupled by Coulomb interaction, there are, in total, six (instead of only two) oscillation modes of the entangled system with interaction-dependent oscillation frequencies. By tuning the bias voltage, one can engineer decoherence such that only one of the six modes, in which the charge oscillations in both double quantum dots become synchronized in antiphase, is singled out. We suggest using waiting-time distributions and the ${g}^{(2)}$-correlation function to detect the common frequency and the phase locking.

arXiv:2107.10218Physical review. B./Physical review. BOct 11, 202110 citations

{g}^{(2)}

-correlation function to detect the common frequency and the phase locking.