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arXiv:cond-mat/0204505 · Progress of Theoretical Physics Supplement

First-Order Phase Transitions in Frustrated Spin Systems

Akihisa Koga, Akira Kawaguchi, Kouichi Okunishi, Norio Kawakami

Published Jan 1, 2002• 1 citation
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Abstract

We give a short review of our recent works on the first-order quantum phase transitions in frustrated spin chains with orthogonal-dimer structure. When the ratio of the competing antiferromagnetic exchange couplings is varied, a first-order transition occurs between the dimer phase and the plaquette phase, which is accompanied by the discontinuity in the spin excitation gap. We further show that strong frustration triggers the phase transitions in a magnetic field, which exhibit plateaus and jumps in the magnetization curve. The hole-doping effect is also addressed for the orthogonal-dimer chain with linked-tetrahedra structure. It is found that the competing antiferromagnetic interactions result in a first-order metal-insulator transition upon hole doping.

DOI
10.1143/ptps.145.52

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We give a short review of our recent works on the first-order quantum phase transitions in frustrated spin chains with orthogonal-dimer structure. When the ratio of the competing antiferromagnetic exchange couplings is varied, a first-order transition occurs between the dimer phase and the plaquette phase, which is accompanied by the discontinuity in the spin excitation gap. We further show that strong frustration triggers the phase transitions in a magnetic field, which exhibit plateaus and jumps in the magnetization curve. The hole-doping effect is also addressed for the orthogonal-dimer chain with linked-tetrahedra structure. It is found that the competing antiferromagnetic interactions result in a first-order metal-insulator transition upon hole doping.
We give a short review of our recent works on the first-order quantum phase transitions in frustrated spin chains with orthogonal-dimer structure. When the ratio of the competing antiferromagnetic exchange couplings is varied, a first-order transition occurs between the dimer phase and the plaquette phase, which is accompanied by the discontinuity in the spin excitation gap. We further show that strong frustration triggers the phase transitions in a magnetic field, which exhibit plateaus and jumps in the magnetization curve. The hole-doping effect is also addressed for the orthogonal-dimer chain with linked-tetrahedra structure. It is found that the competing antiferromagnetic interactions result in a firstorder metal-insulator transition upon hole doping. Recently antiferromagnetic quantum spin systems with strong frustration have been studied intensively. A typical example is SrCu2(BO3)2 1) where the spin-1/2 magnetic Cu ions are located on the orthogonal-dimer lattice (the so-called Shastry-Sutherland model). 2) Various interesting phenomena were observed for this compound
We investigate the low-energy properties of the orthogonal-dimer spin chain characterized by a frustrated dimer-plaquette structure. When the competing antiferromagnetic couplings are varied, the first-order quantum phase transition occurs between the dimer and the plaquette phases, which is accompanied by nontrivial features due to frustration: besides the discontinuity in the lowest excitation gap at the transition point, a sharp level crossing occurs for the spectrum in the plaquette phase. We further reveal that the plateau in the magnetization curve at 1/4 of the full moment dramatically changes its character in the vicinity of the critical point. It is argued that the first-order phase transition in this system captures some essential properties found in the two-dimensional orthogonal-dimer model proposed for SrCu2(BO3)2.{\mathrm{SrCu}}_{2}({\mathrm{BO}}_{3}{)}_{2}.SrCu2​(BO3​)2​.
We investigate quantum phase transitions in a frustrated orthogonal-dimer chain with an arbitrary spin S> 1/2.S>~1/2.S> 1/2. When the ratio of the competing exchange couplings is varied, first-order phase transitions occur 2S2S2S times among distinct spin-gap phases. The introduction of single-ion anisotropy further enriches the phase diagram. The phase transitions described by the present model possess most of the essential properties inherent in frustrated quantum spin systems.
Hole-doping effects are investigated on the {\it t-J} ladder model with the linked-tetrahedra structure. We discuss how a metal-insulator transition occurs upon hole doping with particular emphasis on the effects of geometrical frustration. By computing the electron density and the spin correlation function by the density matrix renormalization group, we show that strong frustration triggers a first-order transition to a metallic phase, when holes are doped into the plaquette-singlet phase. By examining spin excitations in a metallic case in detail, we discuss whether the spin-gap phase persists upon hole doping according to the strength of frustration. It is further shown that the lowest excited state in a spin-gap metallic phase can be described in two independent quasiparticles.
Hole-doping effects are investigated on the {\it t-J} ladder model with the linked-tetrahedra structure. We discuss how a metal-insulator transition occurs upon hole doping with particular emphasis on the effects of geometrical frustration. By computing the electron density and the spin correlation function by the density matrix renormalization group, we show that strong frustration triggers a first-order transition to a metallic phase, when holes are doped into the plaquette-singlet phase. By examining spin excitations in a metallic case in detail, we discuss whether the spin-gap phase persists upon hole doping according to the strength of frustration. It is further shown that the lowest excited state in a spin-gap metallic phase can be described in two independent quasiparticles.
We study the frustrated dimer-plaquette quantum spin chain for ferromagnetic dimer bonds. This quantum system undergoes a series of first-order ground-state phase transitions driven by frustration or by a magnetic field. We find that the different nature of the ground-state phases has a strong influence on the magnetization curve as well as the low-temperature thermodynamics. In particular, the magnetization curve exhibits plateaus and jumps, the number of which depends on the strength of frustration. The temperature dependence of the susceptibility may either show an activated spin-gap behavior for small frustration or a Curie-like paramagnetic behavior for strong frustration.