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arXiv:cond-mat/0203238 · Physical Review Letters

Interactions and Disorder in Quantum Dots: Instabilities and Phase Transitions

Ganpathy N. Murthy, Harsh Mathur

Published Sep 3, 2002• 27 citations
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Abstract

Using a fermionic renormalization group approach, we analyze a model where the electrons diffusing on a quantum dot interact via Fermi-liquid interactions. Describing the single-particle states by random matrix theory, we find that interactions can induce phase transitions (or crossovers for finite systems) to regimes where fluctuations and collective effects dominate at low energies. Implications for experiments and numerical work on quantum dots are discussed.

DOI
10.1103/physrevlett.89.126804

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Using a fermionic renormalization group approach, we analyze a model where the electrons diffusing on a quantum dot interact via Fermi-liquid interactions. Describing the single-particle states by random matrix theory, we find that interactions can induce phase transitions (or crossovers for finite systems) to regimes where fluctuations and collective effects dominate at low energies. Implications for experiments and numerical work on quantum dots are discussed.
Quantum dots with a large Thouless number ggg embody a regime where both disorder and interactions can be treated nonperturbatively using large-NNN techniques (with N=gN=gN=g) and quantum phase transitions can be studied. Here we focus on dots where the noninteracting Hamiltonian is drawn from a crossover ensemble between two symmetry classes, where the crossover parameter introduces a tunable energy scale independent of and much smaller than the Thouless energy. We show that the quantum critical regime, dominated by collective critical fluctuations, can be accessed at this energy scale. The nonperturbative physics of this regime can only be described by the large-NNN approach, as we illustrate with two experimentally relevant examples.
We provide a framework for analyzing the problem of interacting electrons in a ballistic quantum dot with chaotic boundary conditions within an energy ET{E}_{T}ET​ (the Thouless energy) of the Fermi energy. Within this window we show that the interactions can be characterized by Landau Fermi-liquid parameters. When g, the Thouless number (also the dimensionless conductance when it has strong coupling to leads) of the dot, is large, we find that the disordered interacting problem can be solved in a saddle-point approximation which becomes exact as $\stackrel{\ensuremath{\rightarrow}}{g}\ensuremath{\infty}$ (as in a $\mathrm{l}\mathrm{a}\mathrm{r}\mathrm{g}\mathrm{e}\ensuremath{-}N$ theory). The infinite g theory has two phases as a function of the Landau parameter um{u}_{m}um​ in a channel with angular momentum m: A weak-coupling phase where constant charging and exchange interactions dominate the low-energy physics, as in previous ``universal Hamiltonian'' treatments, and a strong-coupling phase characterized by the same order parameter as in the Pomeranchuk transition in clean systems (a spontaneous interaction-induced Fermi-surface distortion), but smeared and pinned by disorder. Thus, both interactions and disorder are crucial to the existence of these phases. At finite g, the two phases and critical point evolve into three regimes in the ${u}_{m}\ensuremath{-}1/g$ plane---weak- and strong-coupling regimes separated by crossover lines from a quantum-critical regime controlled by the quantum-critical point. In this, the first of a two part series, we focus on the consequences of this picture for Coulomb Blockade experiments. We employ analytical and numerical methods to predict the statistics of single-particle levels, Coulomb Blockade peak spacings, conductance peak heights, and quasiparticle widths. We show that in the strong-coupling and quantum-critical regions, the quasiparticle acquires a width of the same order as the level spacing $\ensuremath{\Delta}$ within a few $\ensuremath{\Delta}\mathrm{'}\mathrm{s}$ of the Fermi energy due to coupling to collective excitations. In the strong-coupling regime if m is odd, the dot will (if isolated) crossover from the orthogonal to unitary ensemble for an exponentially small external flux or will (if strongly coupled to leads) break time-reversal symmetry spontaneously. For any m, the peak-spacing distribution becomes broader than expected in previous works and even has support at negative values, which in turn is correlated with small peak heights. Ballistic/chaotic quantum dots afford us unrivalled theoretical and experimental control over the problem of simultaneous disorder and interactions due to the 1/g1/g1/g expansion and our ability to vary disorder and interaction much more readily than in the bulk.
We apply a combination of numerical renormalization group (NRG) and renormalized perturbation theory (RPT) to a model of two quantum dots (impurities) described by two Anderson impurity models hybridized to their respective baths. The dots are coupled via a direct Coulomb interaction U12{U}_{12}U12​ and a spin exchange interaction JJJ. The model has two types of quantum critical points, one at J=JcJ={J}_{c}J=Jc​ to a local singlet state and one at U12=U12c{U}_{12}={U}_{12}^{c}U12​=U12c​ to a locally charge ordered state. The renormalized parameters which determine the low energy behavior are calculated from the NRG. The results confirm the values predicted from the RPT on the approach to the critical points, which can be expressed in terms of a single energy scale T∗{T}^{*}T∗ in all cases. This includes cases without particle-hole symmetry, and cases with asymmetry between the dots, where there is also a transition at J=JcJ={J}_{c}J=Jc​. The results give a comprehensive quantitative picture of the behavior of the model in the low energy Fermi liquid regimes, and some of the conclusions regarding the emergence of a single energy scale may apply to a more general class of quantum critical points, such as those observed in some heavy fermion systems.
We study correlated two-level quantum dots, coupled in effective one-channel fashion to metallic leads, with electron interactions including on-level and interlevel Coulomb repulsions, as well as the interorbital Hund's rule exchange favoring the spin-1 state in the relevant sector of the free dot. For arbitrary dot occupancy, the underlying phases, quantum phase transitions (QPTs), thermodynamics, single-particle dynamics, and electronic transport properties are considered, and direct comparison is made to conductance experiments on lateral quantum dots. Two distinct phases arise generically, one characterized by a normal Fermi liquid fixed point (FP) and the other by an underscreened (USC) spin-1 FP. Associated QPTs, which occur in general in a mixed valent regime of nonintegral dot charge, are found to consist of continuous lines of Kosterlitz-Thouless transitions, separated by first-order level-crossing transitions at high symmetry points. A ``Friedel-Luttinger sum rule'' is derived and, together with a deduced generalization of Luttinger's theorem to the USC phase (a singular Fermi liquid), is used to obtain a general result for the T=0T=0T=0 zero-bias conductance, expressed solely in terms of the dot occupancy and applicable to both phases. Relatedly, dynamical signatures of the QPT show two broad classes of behavior, corresponding to the collapse of either a Kondo resonance, or antiresonance, as the transition is approached from the Fermi liquid phase, the latter behavior being apparent in experimental differential conductance maps. The problem is studied using the numerical renormalization group method, combined with analytical arguments.
Understanding the effects of disorder in quantum many-body systems is one of the central challenges of contemporary statistical physics. Its interplay with interactions and quantum fluctuations profoundly modifies the nature of quantum states and their dynamics, giving rise to phenomena such as localization, ergodicity breaking, and the emergence of complex collective behavior. This thesis presents new results on two classes of disordered quantum systems. The first part is devoted to the study of the many-body localization transition, a paradigmatic example of disorder-induced ergodicity breaking. The critical properties of the transition are investigated using a numerical renormalization-group approach, establishing a connection between its scaling behavior and that of the Anderson localization transition on tree-like graphs. The second part focuses on the zero-temperature quantum spin-glass phase of the two-dimensional bond-disordered Heisenberg model. Combining large-scale numerical simulations with a semiclassical expansion, evidence is provided for the existence of the spin-glass phase. The effective model governing the semiclassical fluctuations is further analyzed to characterize the low-energy excitation spectrum and its localization properties. Finally, the weak-disorder regime is investigated and its implications for the ferromagnetic phase are discussed. Overall, the results presented in this thesis contribute to the understanding of the effects of disorder in interacting quantum many-body systems, encompassing both localization phenomena and the collective behavior of disordered quantum magnets.
Numerous correlated electron systems exhibit a strongly scale-dependent behavior. Upon lowering the energy scale, collective phenomena, bound states, and new effective degrees of freedom emerge. Typical examples include (i) competing magnetic, charge, and pairing instabilities in two-dimensional electron systems; (ii) the interplay of electronic excitations and order parameter fluctuations near thermal and quantum phase transitions in metals; and (iii) correlation effects such as Luttinger liquid behavior and the Kondo effect showing up in linear and nonequilibrium transport through quantum wires and quantum dots. The functional renormalization group is a flexible and unbiased tool for dealing with such scale-dependent behavior. Its starting point is an exact functional flow equation, which yields the gradual evolution from a microscopic model action to the final effective action as a function of a continuously decreasing energy scale. Expanding in powers of the fields one obtains an exact hierarchy of flow equations for vertex functions. Truncations of this hierarchy have led to powerful new approximation schemes. This review is a comprehensive introduction to the functional renormalization group method for interacting Fermi systems. A self-contained derivation of the exact flow equations is presented and frequently used truncation schemes are described. Reviewing selected applications it is shown how approximations based on the functional renormalization group can be fruitfully used to improve our understanding of correlated fermion systems.