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arXiv:cond-mat/0202355 · Physical review. B, Condensed matter

Thermodynamics of strongly disordered spin ladders

Eddy Yusuf, Kun Yang

Published Jun 10, 2002• 13 citations
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Abstract

We study antiferromagnetic two-leg spin-1/2 ladders with strong bond randomness, using the real-space renormalization-group method. We find the low-temperature spin susceptibility of the system follows nonuniversal power laws, and that the ground-state spin-spin correlation is short ranged. Our results suggest that there is no phase transition when the bond randomness increases from zero; for strong enough randomness the system is in a Griffith region with divergent spin susceptibility and short-range spin-spin correlation.

DOI
10.1103/physrevb.65.224428

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We study antiferromagnetic two-leg spin-1/2 ladders with strong bond randomness, using the real-space renormalization-group method. We find the low-temperature spin susceptibility of the system follows nonuniversal power laws, and that the ground-state spin-spin correlation is short ranged. Our results suggest that there is no phase transition when the bond randomness increases from zero; for strong enough randomness the system is in a Griffith region with divergent spin susceptibility and short-range spin-spin correlation.
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The effect of quenched disorder on the low-energy properties of various antiferromagnetic spin-ladder models is studied by a numerical strong disorder renormalization-group method and by density-matrix renormalization. For strong enough disorder the originally gapped phases with finite topological or dimer order become gapless. In these quantum Griffiths phases the scaling of the energy, as well as the singularities in the dynamical quantities, are characterized by a finite dynamical exponent, z, which varies with the strength of disorder. At the phase boundaries, separating topologically distinct Griffiths phases the singular behavior of the disordered ladders is generally controlled by an infinite randomness fixed point.
This dissertation is a systematic theoretical effort to investigate the low-energy properties of random antiferromagnetic quantum spin-1/2 systems beyond one dimension. We use the celebrated real space renormalization group (RSRG) technique developed by Dasgupta, Ma, and Hu to understand the static and dynamic properties of random antiferromagnetic spin-1/2 ladders and weakly coupled random antiferromagnetic spin-1/2 chains. Pure antiferromagnetic spin-1/2 ladders are known to be in the spin liquid phase with a ¯nite energy gap in the excitation spectrum and a short range spin-spin correlation. We are interested in investigating the nature of these systems when disorder, controlled by bond randomness and the presence of impurities, is introduced. Using real-space renormalization group method we are able to find that when disorder comes from bond randomness only, the system flows into a Griffith phase which is characterized by non-universal diverging spin susceptibility and short-range spin-spin correlation. When impurities with spin 0 or 1 are introduced into the system, the system flows into a different fixed point which is controlled by large effective spins whose susceptibility is characterized by a universal Curie-like 1=T behavior. This conclusion holds for any impurities with integer spin. We also study the low-energy collective excitations and dynamical response functions of weakly coupled random antiferromagnetic spin-1/2 chains at low temperature whose low energy properties are governed by the strong-randomness fixed point. By combining RSRG technique to tackle the intrachain couplings and Random Phase Approximation (RPA) formalism for the interchain couplings, we show that the system supports collective spin wave excitations with linear dispersions and calculate the spin wave velocity in terms of microscopic parameters of the chain. Our result agrees with the measured dispersion for Zn-doped CuGeO3 where it shows a linear dispersion along the chain. We predict the spectra weight within RPA which can be qualitatively compared to the scattering intensity in the Inelastic Neutron Scattering experiment.
We investigate the effects of quenched disorder, in the form of site and bond dilution, on the physics of the S=1/2S=1/2S=1/2 antiferromagnetic Heisenberg model on even-leg ladders. Site dilution is found to prune rung singlets and thus create localized moments which interact via a random, unfrustrated network of effective couplings, realizing a random-exchange Heisenberg model in one spatial dimension. This system exhibits a power-law diverging correlation length as the temperature decreases. Contrary to previous claims, we observe that the scaling exponent is nonuniversal, i.e., doping dependent. This finding can be explained by the discrete nature of the values taken by the effective exchange couplings in the doped ladder. Bond dilution on even-leg ladders leads to a more complex evolution with doping of correlations, which are weakly enhanced in 2-leg ladders, and are even suppressed for low dilution in the case of 4-leg and 6-leg ladders. We clarify the different aspects of correlation enhancement and suppression due to bond dilution by isolating the contributions of rung-bond dilution and leg-bond dilution.
We present a new perturbative real space renormalization group (RG) to study random quantum spin chains and other one-dimensional disordered quantum systems. The method overcomes problems of the original approach which fails for quantum random chains with spins larger than S=1/2. Since it works even for weak disorder, we are able to obtain the zero temperature phase diagram of the random antiferromagnetic Heisenberg spin-1 chain as a function of disorder. We find a random singlet phase for strong disorder. As the disorder decreases, the system shows a crossover from a Griffiths to a disordered Haldane phase.
We consider S=1/2 antiferromagnetic Heisenberg chains with alternating bonds and quenched disorder, which represents a theoretical model of the compound CuCl_{2x}Br_{2(1-x)}(γ-{pic})_2. Using a numerical implementation of the strong disorder renormalization group method we study the low-energy properties of the system as a function of the concentration, x, and the type of correlations in the disorder. For perfect correlation of disorder the system is in the random dimer (Griffiths) phase having a concentration dependent dynamical exponent. For weak or vanishing disorder correlations the system is in the random singlet phase, in which the dynamical exponent is formally infinity. We discuss consequences of our results for the experimentally measured low-temperature susceptibility of CuCl_{2x}Br_{2(1-x)}(γ-{pic})_2.