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Renormalization Group Study on Coupled Random Antiferromagnetic Spin-1/2 Chains

Published Jan 1, 2005• 0 citations
OpenAlex

Abstract

This dissertation is a systematic theoretical effort to investigate the low-energy properties of random antiferromagnetic quantum spin-1/2 systems beyond one dimension. We use the celebrated real space renormalization group (RSRG) technique developed by Dasgupta, Ma, and Hu to understand the static and dynamic properties of random antiferromagnetic spin-1/2 ladders and weakly coupled random antiferromagnetic spin-1/2 chains. Pure antiferromagnetic spin-1/2 ladders are known to be in the spin liquid phase with a ¯nite energy gap in the excitation spectrum and a short range spin-spin correlation. We are interested in investigating the nature of these systems when disorder, controlled by bond randomness and the presence of impurities, is introduced. Using real-space renormalization group method we are able to find that when disorder comes from bond randomness only, the system flows into a Griffith phase which is characterized by non-universal diverging spin susceptibility and short-range spin-spin correlation. When impurities with spin 0 or 1 are introduced into the system, the system flows into a different fixed point which is controlled by large effective spins whose susceptibility is characterized by a universal Curie-like 1=T behavior. This conclusion holds for any impurities with integer spin. We also study the low-energy collective excitations and dynamical response functions of weakly coupled random antiferromagnetic spin-1/2 chains at low temperature whose low energy properties are governed by the strong-randomness fixed point. By combining RSRG technique to tackle the intrachain couplings and Random Phase Approximation (RPA) formalism for the interchain couplings, we show that the system supports collective spin wave excitations with linear dispersions and calculate the spin wave velocity in terms of microscopic parameters of the chain. Our result agrees with the measured dispersion for Zn-doped CuGeO3 where it shows a linear dispersion along the chain. We predict the spectra weight within RPA which can be qualitatively compared to the scattering intensity in the Inelastic Neutron Scattering experiment.

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This dissertation is a systematic theoretical effort to investigate the low-energy properties of random antiferromagnetic quantum spin-1/2 systems beyond one dimension. We use the celebrated real space renormalization group (RSRG) technique developed by Dasgupta, Ma, and Hu to understand the static and dynamic properties of random antiferromagnetic spin-1/2 ladders and weakly coupled random antiferromagnetic spin-1/2 chains. Pure antiferromagnetic spin-1/2 ladders are known to be in the spin liquid phase with a ¯nite energy gap in the excitation spectrum and a short range spin-spin correlation. We are interested in investigating the nature of these systems when disorder, controlled by bond randomness and the presence of impurities, is introduced. Using real-space renormalization group method we are able to find that when disorder comes from bond randomness only, the system flows into a Griffith phase which is characterized by non-universal diverging spin susceptibility and short-range spin-spin correlation. When impurities with spin 0 or 1 are introduced into the system, the system flows into a different fixed point which is controlled by large effective spins whose susceptibility is characterized by a universal Curie-like 1=T behavior. This conclusion holds for any impurities with integer spin. We also study the low-energy collective excitations and dynamical response functions of weakly coupled random antiferromagnetic spin-1/2 chains at low temperature whose low energy properties are governed by the strong-randomness fixed point. By combining RSRG technique to tackle the intrachain couplings and Random Phase Approximation (RPA) formalism for the interchain couplings, we show that the system supports collective spin wave excitations with linear dispersions and calculate the spin wave velocity in terms of microscopic parameters of the chain. Our result agrees with the measured dispersion for Zn-doped CuGeO3 where it shows a linear dispersion along the chain. We predict the spectra weight within RPA which can be qualitatively compared to the scattering intensity in the Inelastic Neutron Scattering experiment.
Quantum Heisenberg spin chains with random couplings and spin sizes are studied using a real-space renormalization group technique. These systems belong to a new universality class of disordered quantum spin systems realized in, e.g., ${\mathrm{Sr}}_{3}\mathrm{Cu}{\mathrm{Pt}}_{1\ensuremath{-}x}{\mathrm{Ir}}_{x}{\mathrm{O}}_{6}$. The low-energy fixed point is characterized by the formation of weakly coupled large effective spins. At low temperature TTT the entropy obeys a power law ${T}^{\ensuremath{\delta}}$ ($\ensuremath{\delta}\ensuremath{\approx}0.44$), and the susceptibility follows a Curie-like behavior.
We have carried out Monte Carlo studies of a random-exchange antiferromagnetic spin-(1/2) chain. For systems with XY-like (anisotropic) and with Heisenberg (isotropic) coupling, our results confirm the existence of a disorder-induced low-temperature (T) divergence in the long-wavelength Sz{S}^{z}Sz-Sz{S}^{z}Sz susceptibility \ensuremath{\chi} which was previously predicted by real-space renormalization-group (RSRG) treatments. Over the finite temperature range studied, these results are consistent with a 1/(T ln2{\mathrm{ln}}^{2}ln2T) behavior of \ensuremath{\chi}, and hence in qualitative agreement with the RSRG results. As in the XY-Heisenberg regime, we also find a disorder-induced enhancement of the low-T susceptibility for a system with Ising-like exchange coupling which, over the finite temperature range studied, is again consistent with RSRG results. However, there are inconsistencies between the RSRG predictions in the Ising-like regime at very low temperatures, and the exact results for the random-exchange Ising chain and the low-temperature behavior of \ensuremath{\chi} in the Ising-like regime may in fact be more complicated than predicted by RSRG. Finally, we also present results for the antiferromagnetic susceptibility and structure factor. For both Heisenberg and Ising-like systems, we find that disorder suppresses the long-range antiferromagnetic correlations at low T.
We investigate weakly coupled spin-1/2 ladders in a magnetic field. The work is motivated by recent experiments on the compound (C5H12N)2CuBr4\mathrm{(C_5H_{12}N)_2CuBr_4}(C5​H12​N)2​CuBr4​ (BPCB). We use a combination of numerical and analytical methods, in particular the density matrix renormalization group (DMRG) technique, to explore the phase diagram and the excitation spectra of such a system. We give detailed results on the temperature dependence of the magnetization and the specific heat, and the magnetic field dependence of the nuclear magnetic resonance (NMR) relaxation rate of single ladders. For coupled ladders, treating the weak interladder coupling within a mean field approach, we compute the transition temperature of triplet condensation and its corresponding antiferromagnetic order parameter. Existing experimental measurements are discussed and compared to our theoretical results. Furthermore we compute, using time dependent DMRG, the dynamical correlations of a single spin ladder. Our results allow to directly describe the inelastic neutron scattering cross section up to high energies. We focus on the evolution of the spectra with the magnetic field and compare their behavior for different couplings. The characteristic features of the spectra are interpreted using different analytical approaches such as the mapping onto a spin chain, a Luttinger liquid (LL) or onto a t-J model. For values of parameters for which such measurements exist, we compare our results to inelastic neutron scattering experiments on the compound BPCB and find excellent agreement. We make additional predictions for the high energy part of the spectrum that are potentially testable in future experiments.
The low energy properties of the spin-1/2 random Heisenberg chain with ferromagnetic and antiferromagnetic interactions are studied by means of the density matrix renormalization group (DMRG) and real space renormalization group (RSRG) method for finite chains. The results of the two methods are consistent with each other. The deviation of the gap distribution from that of the random singlet phase and the formation of the large-spin state is observed even for relatively small systems. For a small fraction of the ferromagnetic bond, the effect of the crossover to the random singlet phase on the low temperature susceptibility and specific heat is discussed. The crossover concentration of the ferromagnetic bond is estimated from the numerical data.
The Ma-Dasgupta real-space renormalization methods allow to study disordered systems which are governed by strong disorder fixed points. After a general introduction to the qualitative ideas and to the quantitative renormalization rules, we describe the explicit exact results that can be obtained in various one-dimensional models, either classical or quantum, either for dynamics or statics. The main part of this dissertation is devoted to statistical physics models, with special attention to (i) the off-equilibrium dynamics of a particle diffusing in a Brownian potential or in a trap landscape, (ii) the coarsening dynamics and the equilibrium of classical disordered spin chains, (iii) the delocalization transition of a random polymer at an interface. The last part of the dissertation deals with two disordered quantum spin chains which exhibit a zero-temperature phase transition as the disorder varies, namely (a) the random antiferromagnetic S=1 spin chain, (b) the random transverse field Ising chain.