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arXiv:cond-mat/0106390 · Physical review. B, Condensed matter

Superconducting correlations in metallic nanoparticles: Exact solution of the BCS model by the algebraic Bethe ansatz

Huan-Qiang Zhou, Jon Links, Ross H. McKenzie, M. D. Gould

Published Jan 11, 2002• 98 citations
arXivHTMLPDF

Abstract

Superconducting pairing of electrons in nanoscale metallic particles with discrete energy levels and a fixed number of electrons is described by the reduced Bardeen, Cooper, and Schrieffer model Hamiltonian. We show that this model is integrable by the algebraic Bethe ansatz. The eigenstates, spectrum, conserved operators, integrals of motion, and norms of wave functions are obtained. Furthermore, the quantum inverse problem is solved, meaning that form factors and correlation functions can be explicitly evaluated. Closed form expressions are given for the form factors and correlation functions that describe superconducting pairing.

DOI
10.1103/physrevb.65.060502

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Superconducting pairing of electrons in nanoscale metallic particles with discrete energy levels and a fixed number of electrons is described by the reduced Bardeen, Cooper, and Schrieffer model Hamiltonian. We show that this model is integrable by the algebraic Bethe ansatz. The eigenstates, spectrum, conserved operators, integrals of motion, and norms of wave functions are obtained. Furthermore, the quantum inverse problem is solved, meaning that form factors and correlation functions can be explicitly evaluated. Closed form expressions are given for the form factors and correlation functions that describe superconducting pairing.
In this review we demonstrate how the algebraic Bethe ansatz is used for the calculation of the energy spectra and form factors (operator matrix elements in the basis of Hamiltonian eigenstates) in exactly solvable quantum systems. As examples we apply the theory to several models of current interest in the study of Bose–Einstein condensates, which have been successfully created using ultracold dilute atomic gases. The first model we introduce describes Josephson tunnelling between two coupled Bose–Einstein condensates. It can be used not only for the study of tunnelling between condensates of atomic gases, but for solid state Josephson junctions and coupled Cooper pair boxes. The theory is also applicable to models of atomic–molecular Bose–Einstein condensates, with two examples given and analysed. Additionally, these same two models are relevant to studies in quantum optics. Finally, we discuss the model of Bardeen, Cooper and Schrieffer in this framework, which is appropriate for systems of ultracold fermionic atomic gases, as well as being applicable for the description of superconducting correlations in metallic grains with nanoscale dimensions. In applying all the above models to physical situations, the need for an exact analysis of small-scale systems is established due to large quantum fluctuations which render mean-field approaches inaccurate.
We present a derivation of a previously announced result for matrix elements between exact eigenstates of the pairing Hamiltonian. Our results, which generalize the well-known Bardeen–Cooper–Schrieffer (BCS) (Bardeen et al 1957 Phys. Rev. 108 1175; 1957 Phys. Rev. 106 162) expressions for what are known as ‘coherence factors’, are derived based on the Slavnov (1989 Theor. Math. Phys. 79 502) formula for overlaps between Bethe-ansatz states, thus making use of the known connection between the exact diagonalization of the BCS Hamiltonian, due to Richardson (1963 Phys. Lett. 3 277; 1964 Nucl. Phys. A 52 221), and the algebraic Bethe ansatz. The resulting formula has a compact form after a suitable parameterization of the energy plane. Although we apply our method here to the pairing Hamiltonian, it may be adjusted to study what is termed the ‘Sutherland limit’ (Sutherland 1995 Phys. Rev. Lett. 74 816) for exactly solvable models, namely where a macroscopic number of rapidities form a large string.
Integrable systems take a special niche in quantum many-body systems. Due to the underlying algebraic structure, it is possible to capture all the quantum correlations exactly within a Bethe Ansatz wavefunction at a favourably scaling computational cost. Richardson [1] and Gaudin [2] have shown that the reduced Bardeen-Cooper-Schrieffer (BCS) Hamiltonian of superconductivity [3] is integrable and that the Bethe Ansatz state corresponds to a product wave function of generalized Cooper pairs [4]. In this formulation, the Bethe ansatz state is equivalent to a non-orthogonal geminal, which is widely used in quantum chemistry to describe electron pair correlations in atoms and molecules [5]. Inspired by Richardson-Gaudin integrable systems, it is possible to construct classes of non-orthogonal geminals, allowing for an accurate description of realistic and non-integrable strongly correlated atoms and molecules, while retaining the favorable computational scaling [6, 7]. In this contribution, I will discuss Richardson-Gaudin integrability and why it is useful for strongly correlated systems.
We demonstrate a novel approach that allows the determination of very general classes of exactly solvable Hamiltonians via Bethe ansatz methods. This approach combines aspects of both the co-ordinate Bethe ansatz and algebraic Bethe ansatz. The eigenfunctions are formulated as factorisable operators acting on a suitable reference state. Yet, we require no prior knowledge of transfer matrices or conserved operators. By taking a variational form for the Hamiltonian and eigenstates we obtain general exact solvability conditions. The procedure is conducted in the framework of Hamiltonians describing the crossover between the low-temperature phenomena of superconductivity, in the Bardeen-Cooper-Schrieffer (BCS) theory, and Bose-Einstein condensation (BEC).