It is investigated theoretically that magnetized Bose-Einstein condensation (BEC) with the internal (spin) degrees of freedom exhibits a rich variety of phase transitions, depending on the sign of the interaction in the spin channel. In the antiferromagnetic interaction case there exist always double BEC transitions from single component BEC to multiple component BEC. In the ferromagnetic case BEC becomes always unstable at a lower temperature, leading to a phase separation. The detailed phase diagram for the temperature vs the polarization, the spatial spin structure, the distribution of non-condensates and the excitation spectrum are examined for the harmonically trapped systems.
It is investigated theoretically that magnetized Bose-Einstein condensation (BEC) with the internal (spin) degrees of freedom exhibits a rich variety of phase transitions, depending on the sign of the interaction in the spin channel. In the antiferromagnetic interaction case there exist always double BEC transitions from single component BEC to multiple component BEC. In the ferromagnetic case BEC becomes always unstable at a lower temperature, leading to a phase separation. The detailed phase diagram for the temperature vs the polarization, the spatial spin structure, the distribution of non-condensates and the excitation spectrum are examined for the harmonically trapped systems.
We analyze the structure of spin-one Bose-Einstein condensates in the presence of a homogeneous magnetic field. We classify the homogeneous stationary states and study their existence, bifurcations, and energy spectra. We reveal that phase separation can occur in the ground state of antiferromagnetic (polar) condensates while the spin components of the ferromagnetic condensates are always miscible and no phase separation occurs. Our theoretical model, confirmed by numerical simulations, explains that this phenomenon takes place when the energy of the lowest homogeneous state is a concave function of the magnetization. In particular, we predict that phase separation can be observed in a 23Na condensate confined in a highly elongated harmonic trap. Finally, we discuss the phenomena of dynamical instability and spin domain formation.
The achievement in cooling alkali atomic gases, such as 87Rb, 23Na and 7Li, to quantum degeneracy opens up a way to study magnetism in spinor bosons, because these constituent atoms usually have a hyperfine spin degree of freedom. This article reviews several basic problems related to the ferromagnetic phase transition in spinor atomic Bose gases from a theoretical perspective. After a brief discussion on various possible origins of the ferromagnetic interaction, the phase diagram of the ferromagnetically coupled spinor bosons is investigated. It is found that the ferromagnetic transition occurs always above Bose-Einstein condensation and the Bose condensate is fully polarized. The low-lying collective excitations of the spinor condensate, including spin and density modes, are discussed. The spectrum of the density mode is of the Bogliubov form and the spin wave spectrum has a k2-formed dispersion relation at long wavelengths. The spin-wave stiffness coefficient contains contribut
We study experimentally the equilibrium phase diagram of a spin-1 Bose-Einstein condensate with antiferromagnetic interactions, in a regime where spin and spatial degrees of freedom are decoupled. For a given total magnetization mz, we observe for low magnetic fields an ``antiferromagnetic'' phase where atoms condense in the $m=\ifmmode\pm\else\textpm\fi{}1$ Zeeman states, and occupation of the m=0 state is suppressed. Conversely, for large enough magnetic fields, a phase transition to a ``broken-axisymmetry'' phase takes place: The m=0 component becomes populated and rises sharply above a critical field Bc(mz). This behavior results from the competition between antiferromagnetic spin-dependent interactions (dominant at low fields) and the quadratic Zeeman energy (dominant at large fields). We compare the measured Bc as well as the global shape of the phase diagram with mean-field theory, and find good quantitative agreement.
Spinor Bose-Einstein condensates under external magnetic fields exhibit well-characterized spin domains of its ground state due to spin-dependent interactions. At low temperatures, collision-induced spin-mixing instabilities may promote the condensate to dwell into metastable states occurring near the phase boundaries. In this paper, we study theoretically the metastable spin-phase diagram of a spin-1 antiferromagnetic Bose-Einstein condensate at zero and finite temperatures. The approach makes use of Hartree-Fock theory and exploits the symmetry of the Hamiltonian and of the order parameters yielding a closed system of transcendental equations for the free energy, fully avoiding the use of self-consistency methods. Our results are consistent with recent experiments and allow us to explain qualitatively the different types of observed quench dynamics. In addition, we found that similar phenomena should occur in antiferromagnetic spinor condensates with a sudden change in the temperature. It is shown also that the increase in temperature induces a traceable shift of the ferromagnetic-polar transition boundary, behavior previously not noted by self-consistent mean-field calculations.
In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field B. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field Bc, asymptotic values of n0 (relative atom number in mF=0 state) at large B and the phase diagram of n0. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of n0. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" Ts and the ``kinetic temperature" Tk with Ts≪Tk, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.
The ground states of Bose-Einstein condensates (BECs) of spin-2 bosons are classified into three distinct phases (ferromagnetic, ``antiferromagnetic,'' and cyclic) depending on the s-wave scattering lengths of binary collisions for total-spin 0, 2, and 4 channels. Many-body spin correlations and magnetic response of the condensate in each of these phases are studied in a mesoscopic regime, while low-lying excitation spectra are investigated in the thermodynamic regime. In the mesoscopic regime, where the system is so tightly confined that the spatial degrees of freedom are frozen, the exact, many-body ground state for each phase is found to be expressed in terms of the creation operators of pair or trio bosons having spin correlations. These pairwise and trio-wise units are shown to bring about some unique features of spin-2 BECs such as a huge jump in magnetization from minimum to maximum possible values and the robustness of the minimum-magnetization state against an applied magnetic field. In the thermodynamic regime, where the system is spatially uniform, low-lying excitation spectra in the presence of magnetic field are obtained analytically using the Bogoliubov approximation. In the ferromagnetic phase, the excitation spectrum consists of one Goldstone mode and four single-particle modes. In the antiferromagnetic phase, where spin-singlet ``pairs'' undergo Bose-Einstein condensation, the spectrum consists of two Goldstone modes and three massive ones, all of which become massless when magnetic field vanishes. In the cyclic phase, where boson ``trios'' condense into a spin-singlet state, the spectrum is characterized by two Goldstone modes, one single-particle mode having a magnetic-field-independent energy gap, and a gapless single-particle mode that becomes massless in the absence of magnetic field.