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Possibility to obtain highly monochromatic and polarized photons

A.I. Alikhanyan, R.O. Avakyan, G.L. Bayatyan

Published Jan 1, 1973• 0 citations
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Intense source of monochromatic photons

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Photon emission with nonclassical photon statistics is discussed with a single InAlAs quantum dot. The deterministic single-photon generation in which the emitted photon wavelength matches well to the highly sensitive wavelength region of highly efficient, low-noise Si-single-photon detectors and also to an atmospheric transmission window is demonstrated. Competing transition processes between neutral and charged exciton species originating from an exclusive formation in the same single quantum dot are clarified. It was found that suppressing the charged exciton formation is possible by a quasi-resonant excitation for a deterministic monochromatic single-photon generation. Polarization-dependent photoluminescence spectroscopy clearly indicates the preservation of photon polarizations between photons emitted by biexciton/exciton recombinations. Furthermore, the deterministic polarization-correlated photon pair generation with biexciton-exciton cascaded transition occurring in a single quantum dot is directly confirmed by the polarized second-order photon correlation measurements. This indicates a longer polarization flip time than the exciton lifetime, which is an essential requirement for the deterministic Einstein-Podolsky-Rosen photon pair generation under the present biexciton-exciton cascaded transition scheme.

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Quantum theory of photon emission during strong-laser-field-induced ionization

Dejan B. Milošević

We formulate a quantum theory of photon emission during strong-laser-field-induced ionization and show that such photons can be emitted in a single-step process. The probability of this process is many orders of magnitude higher than that of the well-known high-order harmonic generation, which is a three-step process. We analyzed photon emission for various wavelengths and intensities of the laser field and found that the probability of photon emission is maximal for energies near 5 eV and that it can be shifted to higher energies for higher intensity. For a bichromatic linearly polarized laser field the photon emission rate can be controlled with the relative phase between the field components and can be one order of magnitude higher than in the monochromatic case. For circular laser polarization the rate of photon emission is lower than for the linear one and it depends on the emitted photon direction (it is much lower if the emitted photon polarization is perpendicular to the laser-field polarization plane). For the counterrotating bicircular field the rate is much higher than for the corotating bicircular field, monochromatic circularly and linearly polarized fields, and bichromatic linearly polarized field. The rate is the highest for orthogonally polarized two-color field for the relative phase $\ensuremath{\pi}/2$.

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Circular Dichroism in the Photoionization of Unpolarized Atoms by Two Crossing Photon Beams

Alexei V. Meremianin, Nikolai L. Manakov

The polarization dependence of the photoionization probability was analyzed in the case when a randomly oriented atom is irradiated by two crossing polarized monochromatic photon beams with the same frequency. It was found that the angular distributions of photoelectrons exhibit the effect of circular dichroism (CD), which consists of the dependence of the photoionization probability on the sign of the circular polarization degree of each beam. We demonstrate that the CD effect exists only for coherent crossing photon beams. It was shown that CD effects are strongly dependent on the phase difference between the electric field vectors of the photon beams and have a quite large magnitude. The possibilities of the experimental observation of CD effects are discussed.

Atoms•Dec 3, 2021•0 citations
Photon emission with nonclassical photon statistics is discussed with a single InAlAs quantum dot. The deterministic single-photon generation in which the emitted photon wavelength matches well to the highly sensitive wavelength region of highly efficient, low-noise Si-single-photon detectors and also to an atmospheric transmission window is demonstrated. Competing transition processes between neutral and charged exciton species originating from an exclusive formation in the same single quantum dot are clarified. It was found that suppressing the charged exciton formation is possible by a quasi-resonant excitation for a deterministic monochromatic single-photon generation. Polarization-dependent photoluminescence spectroscopy clearly indicates the preservation of photon polarizations between photons emitted by biexciton/exciton recombinations. Furthermore, the deterministic polarization-correlated photon pair generation with biexciton-exciton cascaded transition occurring in a single quantum dot is directly confirmed by the polarized second-order photon correlation measurements. This indicates a longer polarization flip time than the exciton lifetime, which is an essential requirement for the deterministic Einstein-Podolsky-Rosen photon pair generation under the present biexciton-exciton cascaded transition scheme.
We formulate a quantum theory of photon emission during strong-laser-field-induced ionization and show that such photons can be emitted in a single-step process. The probability of this process is many orders of magnitude higher than that of the well-known high-order harmonic generation, which is a three-step process. We analyzed photon emission for various wavelengths and intensities of the laser field and found that the probability of photon emission is maximal for energies near 5 eV and that it can be shifted to higher energies for higher intensity. For a bichromatic linearly polarized laser field the photon emission rate can be controlled with the relative phase between the field components and can be one order of magnitude higher than in the monochromatic case. For circular laser polarization the rate of photon emission is lower than for the linear one and it depends on the emitted photon direction (it is much lower if the emitted photon polarization is perpendicular to the laser-field polarization plane). For the counterrotating bicircular field the rate is much higher than for the corotating bicircular field, monochromatic circularly and linearly polarized fields, and bichromatic linearly polarized field. The rate is the highest for orthogonally polarized two-color field for the relative phase $\ensuremath{\pi}/2$.
The polarization dependence of the photoionization probability was analyzed in the case when a randomly oriented atom is irradiated by two crossing polarized monochromatic photon beams with the same frequency. It was found that the angular distributions of photoelectrons exhibit the effect of circular dichroism (CD), which consists of the dependence of the photoionization probability on the sign of the circular polarization degree of each beam. We demonstrate that the CD effect exists only for coherent crossing photon beams. It was shown that CD effects are strongly dependent on the phase difference between the electric field vectors of the photon beams and have a quite large magnitude. The possibilities of the experimental observation of CD effects are discussed.