An advanced computer code is undergoing development for numerically simulating laser cooling and trapping of large numbers of atoms. The code is expected to be useful in practical engineering applications and to contribute to understanding of the roles that light, atomic collisions, background pressure, and numbers of particles play in experiments using laser-cooled and -trapped atoms. The code is based on semiclassical theories of the forces exerted on atoms by magnetic and optical fields. Whereas computer codes developed previously for the same purpose account for only a few physical mechanisms, this code incorporates many more physical mechanisms (including atomic collisions, sub-Doppler cooling mechanisms, Stark and Zeeman energy shifts, gravitation, and evanescent-wave phenomena) that affect laser-matter interactions and the cooling of atoms to submillikelvin temperatures. Moreover, whereas the prior codes can simulate the interactions of at most a few atoms with a resonant light field, the number of atoms that can be included in a simulation by the present code is limited only by computer memory. Hence, the present code represents more nearly completely the complex physics involved when using laser-cooled and -trapped atoms in engineering applications. Another advantage that the code incorporates is the possibility to analyze the interaction between cold atoms of different atomic number. Some properties that cold atoms of different atomic species have, like cross sections and the particular excited states they can occupy when interacting with each other and light fields, play important roles not yet completely understood in the new experiments that are under way in laboratories worldwide to form ultracold molecules. Other research efforts use cold atoms as holders of quantum information, and more recent developments in cavity quantum electrodynamics also use ultracold atoms to explore and expand new information-technology ideas. These experiments give a hint on the wide range of applications and technology developments that can be tackled using cold atoms and light fields. From more precise atomic clocks and gravity sensors to the development of quantum computers, there will be a need to completely understand the whole ensemble of physical mechanisms that play a role in the development of such technologies. The code also permits the study of the dynamic and steady-state operations of technologies that use cold atoms. The physical characteristics of lasers and fields can be time-controlled to give a realistic simulation of the processes involved such that the design process can determine the best control features to use. It is expected that with the features incorporated into the code it will become a tool for the useful application of ultracold atoms in engineering applications. Currently, the software is being used for the analysis and understanding of simple experiments using cold atoms, and for the design of a modular compact source of cold atoms to be used in future research and development projects. The results so far indicate that the code is a useful design instrument that shows good agreement with experimental measurements (see figure), and a Windows-based user-friendly interface is also under development.
An advanced computer code is undergoing development for numerically simulating laser cooling and trapping of large numbers of atoms. The code is expected to be useful in practical engineering applications and to contribute to understanding of the roles that light, atomic collisions, background pressure, and numbers of particles play in experiments using laser-cooled and -trapped atoms. The code is based on semiclassical theories of the forces exerted on atoms by magnetic and optical fields. Whereas computer codes developed previously for the same purpose account for only a few physical mechanisms, this code incorporates many more physical mechanisms (including atomic collisions, sub-Doppler cooling mechanisms, Stark and Zeeman energy shifts, gravitation, and evanescent-wave phenomena) that affect laser-matter interactions and the cooling of atoms to submillikelvin temperatures. Moreover, whereas the prior codes can simulate the interactions of at most a few atoms with a resonant light field, the number of atoms that can be included in a simulation by the present code is limited only by computer memory. Hence, the present code represents more nearly completely the complex physics involved when using laser-cooled and -trapped atoms in engineering applications. Another advantage that the code incorporates is the possibility to analyze the interaction between cold atoms of different atomic number. Some properties that cold atoms of different atomic species have, like cross sections and the particular excited states they can occupy when interacting with each other and light fields, play important roles not yet completely understood in the new experiments that are under way in laboratories worldwide to form ultracold molecules. Other research efforts use cold atoms as holders of quantum information, and more recent developments in cavity quantum electrodynamics also use ultracold atoms to explore and expand new information-technology ideas. These experiments give a hint on the wide range of applications and technology developments that can be tackled using cold atoms and light fields. From more precise atomic clocks and gravity sensors to the development of quantum computers, there will be a need to completely understand the whole ensemble of physical mechanisms that play a role in the development of such technologies. The code also permits the study of the dynamic and steady-state operations of technologies that use cold atoms. The physical characteristics of lasers and fields can be time-controlled to give a realistic simulation of the processes involved such that the design process can determine the best control features to use. It is expected that with the features incorporated into the code it will become a tool for the useful application of ultracold atoms in engineering applications. Currently, the software is being used for the analysis and understanding of simple experiments using cold atoms, and for the design of a modular compact source of cold atoms to be used in future research and development projects. The results so far indicate that the code is a useful design instrument that shows good agreement with experimental measurements (see figure), and a Windows-based user-friendly interface is also under development.
Ultracold matter offers a unique capability to reach the best high-precision spectroscopy measurements and leads to exciting perspectives in many different areas of science and technology. Molecules, thanks to their complex spectra, couple with a broader range of photons compared to atoms, so they are extremely attractive for fundamental science or to design new quantum technologies. However, to date, only a few molecular species have been brought to temperatures of the order of the microkelvin. This was done by laser cooling, a process that has been demonstrated only for species featuring an unpaired electron that does not participate to the chemical bond. \n \nA different approach, which is indifferent to the molecule electronic structure and thus potentially universal, is sympathetic cooling, where neutral molecules are cooled in a bath of ultracold atoms. However, inelastic collisions between molecules and the coolant is a major obstacle that has hindered the advances of this method thus far. Trapping the molecules in their absolute ground state would circumvent this problem or at least greatly simplify it. In this thesis we simulate the feasibility of an experiment in which metastable CO molecules are first slowed down to a few m/s with a microstructured Stark decelerator, then they are stopped by a strong DC electrical barrier and finally they are transferred irreversibly to their absolute ground state and captured in an optical trap. \nUnfortunately, the results of the simulations indicate that the total number of molecules that can be accumulated in the optical trap is rather low, far behind the observation threshold. Therefore, we concluded that other approaches to produce ultracold molecules must to be searched.
In the last decades, experimental access to the quantum regime has been gained in a large variety of systems, including dilute ultracold gases, trapped ions, micromechanical oscillators, superconducting circuits, and many more.These systems allow for such exciting applications as quantum computing and communication, quantum metrology and quantum simulation.A physical system's quantum mechanical features can only be revealed by cooling it until the thermal excitations are negligible.To date, the coldest temperatures are reached with ultracold gases by a combination of laser cooling and evaporation, inherently producing individual ensembles.However, many applications can greatly benefit from a continuous source of ultracold atoms, for example sympathetic cooling of molecules or nanoscopic objects.Ideally, this cooling source operates without light, as most molecules have a rich internal structure and can absorb photons of many wavelengths.Another promising application of continuous sources of ultracold matter is atom interferometry.Such interferometers perform measurements of inertial forces, time and gravity.Currently, each cold sample is destroyed by its evaluation and the measurement is interrupted by the preparation of a new samples.Continuous sources can help to eliminate this restriction.So far, no dark and continuous sources exist in the microkelvin regime.This thesis presents the first preparation of such an ultracold atom cloud which is continuously replenished and protected from light.The continuously refilled reservoir is prepared by loading a magnetically guided atom beam into an elongated magnetic trapping potential.This static potential has an entrance barrier which allows atoms from a guided beam to enter the trap.Once in the trap, the atoms undergo collisions and redistribute their kinetic energy.Those gaining energy can escape again, but those losing energy are trapped.A steady state with 3.8 × 10 7 atoms atoms at a temperature of 102 µK is reached and maintained.The setup of the continuous loading scheme is described in this thesis.A key component is a mesoscopic atom chip which produces all magnetic fields for the continuous loading scheme.The initial atom source is a high-flux double magneto-optical trap system.An atomic beam is created out of the precooled atoms and guided to the static trap through a stray light protection allowing for a dark retrapping region.The cooling scheme does not rely on any specific atomic properties of the atoms and can thus be applied to a wide range of particles.The results offer exciting perspectives for an application as a continuous source of ultracold atoms, either as a coolant for sympathetic cooling or as a resource for metrology.
Abstract The invention and development of laser methods for cooling and trapping atoms have led to the advent of the physics of ultracold matter. Low-temperature quantum physics has so far dealt with condensed media, wherein quantum phenomena (superfluidity and superconductivity) usually manifest themselves at temperatures of a few kelvin. Laser cooling and trapping of atoms have made it possible to successively attain millikelvin, microkelvin, and nanokelvin temperatures, at which the de Broglie wavelength of the atoms becomes commensurable with the interatomic separation, even in dilute gases. The interaction of atoms in ultracold dilute gases becomes essentially quantum mechanical. The physics of such quantum gases is more akin to the well-developed physics of condensed matter at low temperatures. It is in essence a boundary field between atomic, laser, and condensed-matter physics. Following the first, pioneering experiments on the Bose–Einstein condensation of alkali-metal atoms, this field has continued to develop at a very fast pace, which can be explained by the vast variety of particles (atoms, isotopes, and molecules) that can be laser cooled and trapped under degeneracy conditions. This is much more than physicists had at their disposal previously (3,4He). Moreover, laser radiation and magnetic fields additionally make it possible to control not only the intrinsic quantum state of the interacting ultracold particle species, but also the interaction of the particles. All this makes the research in the field of quantum gases a great breakthrough, both in atomic–molecular physics and in many-body-interaction physics, which heretofore was the prerogative of low-temperature condensed-matter physics.
Slowing, cooling, and trapping molecules One of the major achievements in physics during the last two decades of the twentieth century was the ability to cool and trap atoms [1]. Laser cooling can produce previously inconceivable atomic temperatures of less than 1 μK. Atoms with sufficiently low kinetic energy can be trapped in magnetic and optical traps and thus studied for a prolonged time, thereby improving the resolution of spectroscopy by many orders of magnitude as well as reducing Doppler broadening. Furthermore, besides the external degrees of freedom, the internal degrees of freedom of the atoms can also be manipulated, leading to full control of the atoms. One of the holy grails of physics, the achievement of Bose–Einstein condensation in a dilute gas, was achieved mainly because of laser cooling and trapping of atoms. One of the natural extensions of laser cooling and trapping of atoms is the application of the techniques to molecules. Molecules offer a much richer internal structure than atoms, and thus provide extended possibilities to experimentalists. However, atomic laser cooling is based on the repetitive scattering of light and requires a closed, or at least nearly closed, two-level system. Because of the complicated internal structure of molecules, a closed two-level system cannot usually be found because they have many different electronic, vibrational, and rotational states and in general can decay to many different states after absorption of light (see Chap. 16). This requires a complete rethinking of the schemes that are used to cool atoms. Still, because of the extended possibilities cold molecules can offer with respect to cold atoms, there have been a large number of techniques developed to slow, cool, and trap them. These techniques can be divided into two classes, namely direct and indirect cooling. In the first case, molecules at cryogenic or room temperature are directly slowed and cooled. Although many different slowing techniques are used, this chapter focuses on Stark slowing of molecules since it was the first technique developed. Apart from the Stark shift of the molecules, the Zeeman and light shift of molecules can also be used to slow them. The idea behind Stark slowing is to subject the moving molecules to a continuously increasing electric field so that their kinetic energy is converted into potential energy.
The tools of atomic physics enable researchers to explore rich quantum mechanical phenomena by way of light-matter interactions. In some applications, light is used to manipulate or modify the properties of a material medium, for instance, laser-cooling and optical trapping of neutral atoms and ions; electromagnetically-induced-transparency (EIT); and Bose- Einstein-Condensation (BEC). Likewise, there are applications where matter is used to manipulate the properties of light, as for example, non-linear optical processes; atomic quantum memories; and quantum-information-processing. This thesis explores two routes towards manipulating light using matter and vice versa in our lab. The work presented in this thesis falls under two categories, one is the experimental side where we have designed and built a laser system to cool a thermal gas of 39K atoms to sub-Doppler temperatures, using the ‘Gray Molasses’ technique. This work is motivated by the long term goal of performing quantum simulation experiments with degenerate quantum gas of K. The second category is on the theoretical (numerical) side, where we introduce a novel quantum memory protocol for coherent storage and processing of broadband light pulses, based on a fundamental physical process in atomic physics, called the ‘Autler-Townes’ effect. Ultracold quantum gases are one of the most versatile systems in the field of cold atom physics; these atomic systems can be experimentally controlled and manipulated with high degree of precision and are thus, widely used to model the behavior of other complex quantum mechanical systems. Laser cooling is the first and indeed a crucial stage towards creating an ultracold gas of atoms. In this thesis, we describe an optical setup for producing a laser-cooled and trapped gas of bosonic 39K atoms, using D1 and D2 atomic transition-lines. The optical setup is built to generate appropriate laser frequencies for implementing various stages of the experiment: red- detuned two and three-dimensional magneto-optical traps (MOT) on the D2-line; a blue-detuned gray molasses phase on the D1-line; as well as optical pumping, imaging and push beams on the D2-line. We also highlight the underlying physics behind the blue-detuned gray molasses cooling and the advantages it offers in cooling species like K and Li. We also discuss in detail, the techniques used for frequency locking our lasers, namely, saturated absorption spectroscopy (SAS) and beatnote locking. The second part of the thesis describes a new atomic quantum-memory scheme for storing broadband pulses of light, which we call the ‘Autler- Townes Splitting (ATS)’ protocol. We show the light storage and retrieval operation in three different configurations, via numerical simulation of Maxwell-Bloch equations. We also discuss the strategies for getting high storage and retrieval efficiency in the ATS memory in terms of only two phenomenological parameters, both of which are experimentally accessible. We have shown that a near-unity efficiency is achievable for a wideband signal, under moderate values of atomic density and laser powers; this significantly relaxes the technical requirements of our protocol when compared to other broadband storage schemes.