The tools of atomic physics enable researchers to explore rich quantum mechanical phenomena by way of light-matter interactions. In some applications, light is used to manipulate or modify the properties of a material medium, for instance, laser-cooling and optical trapping of neutral atoms and ions; electromagnetically-induced-transparency (EIT); and Bose- Einstein-Condensation (BEC). Likewise, there are applications where matter is used to manipulate the properties of light, as for example, non-linear optical processes; atomic quantum memories; and quantum-information-processing. This thesis explores two routes towards manipulating light using matter and vice versa in our lab. The work presented in this thesis falls under two categories, one is the experimental side where we have designed and built a laser system to cool a thermal gas of 39K atoms to sub-Doppler temperatures, using the ‘Gray Molasses’ technique. This work is motivated by the long term goal of performing quantum simulation experiments with degenerate quantum gas of K. The second category is on the theoretical (numerical) side, where we introduce a novel quantum memory protocol for coherent storage and processing of broadband light pulses, based on a fundamental physical process in atomic physics, called the ‘Autler-Townes’ effect. Ultracold quantum gases are one of the most versatile systems in the field of cold atom physics; these atomic systems can be experimentally controlled and manipulated with high degree of precision and are thus, widely used to model the behavior of other complex quantum mechanical systems. Laser cooling is the first and indeed a crucial stage towards creating an ultracold gas of atoms. In this thesis, we describe an optical setup for producing a laser-cooled and trapped gas of bosonic 39K atoms, using D1 and D2 atomic transition-lines. The optical setup is built to generate appropriate laser frequencies for implementing various stages of the experiment: red- detuned two and three-dimensional magneto-optical traps (MOT) on the D2-line; a blue-detuned gray molasses phase on the D1-line; as well as optical pumping, imaging and push beams on the D2-line. We also highlight the underlying physics behind the blue-detuned gray molasses cooling and the advantages it offers in cooling species like K and Li. We also discuss in detail, the techniques used for frequency locking our lasers, namely, saturated absorption spectroscopy (SAS) and beatnote locking. The second part of the thesis describes a new atomic quantum-memory scheme for storing broadband pulses of light, which we call the ‘Autler- Townes Splitting (ATS)’ protocol. We show the light storage and retrieval operation in three different configurations, via numerical simulation of Maxwell-Bloch equations. We also discuss the strategies for getting high storage and retrieval efficiency in the ATS memory in terms of only two phenomenological parameters, both of which are experimentally accessible. We have shown that a near-unity efficiency is achievable for a wideband signal, under moderate values of atomic density and laser powers; this significantly relaxes the technical requirements of our protocol when compared to other broadband storage schemes.
The tools of atomic physics enable researchers to explore rich quantum mechanical phenomena by way of light-matter interactions. In some applications, light is used to manipulate or modify the properties of a material medium, for instance, laser-cooling and optical trapping of neutral atoms and ions; electromagnetically-induced-transparency (EIT); and Bose- Einstein-Condensation (BEC). Likewise, there are applications where matter is used to manipulate the properties of light, as for example, non-linear optical processes; atomic quantum memories; and quantum-information-processing. This thesis explores two routes towards manipulating light using matter and vice versa in our lab. The work presented in this thesis falls under two categories, one is the experimental side where we have designed and built a laser system to cool a thermal gas of 39K atoms to sub-Doppler temperatures, using the ‘Gray Molasses’ technique. This work is motivated by the long term goal of performing quantum simulation experiments with degenerate quantum gas of K. The second category is on the theoretical (numerical) side, where we introduce a novel quantum memory protocol for coherent storage and processing of broadband light pulses, based on a fundamental physical process in atomic physics, called the ‘Autler-Townes’ effect. Ultracold quantum gases are one of the most versatile systems in the field of cold atom physics; these atomic systems can be experimentally controlled and manipulated with high degree of precision and are thus, widely used to model the behavior of other complex quantum mechanical systems. Laser cooling is the first and indeed a crucial stage towards creating an ultracold gas of atoms. In this thesis, we describe an optical setup for producing a laser-cooled and trapped gas of bosonic 39K atoms, using D1 and D2 atomic transition-lines. The optical setup is built to generate appropriate laser frequencies for implementing various stages of the experiment: red- detuned two and three-dimensional magneto-optical traps (MOT) on the D2-line; a blue-detuned gray molasses phase on the D1-line; as well as optical pumping, imaging and push beams on the D2-line. We also highlight the underlying physics behind the blue-detuned gray molasses cooling and the advantages it offers in cooling species like K and Li. We also discuss in detail, the techniques used for frequency locking our lasers, namely, saturated absorption spectroscopy (SAS) and beatnote locking. The second part of the thesis describes a new atomic quantum-memory scheme for storing broadband pulses of light, which we call the ‘Autler- Townes Splitting (ATS)’ protocol. We show the light storage and retrieval operation in three different configurations, via numerical simulation of Maxwell-Bloch equations. We also discuss the strategies for getting high storage and retrieval efficiency in the ATS memory in terms of only two phenomenological parameters, both of which are experimentally accessible. We have shown that a near-unity efficiency is achievable for a wideband signal, under moderate values of atomic density and laser powers; this significantly relaxes the technical requirements of our protocol when compared to other broadband storage schemes.
Abstract \nThis work is split into two parts, in part one of this thesis we report on the improvement of the lifetime of a quantum memory based on neutral atoms while in part two we will focus on a new setup to perform experiments on neutral atoms within a 2D optical lattice. In the quantum memory experiment we used a blue-detuned optical dipole trap to confine the atoms in a minimum intensity region of the light beam, reducing dephasing due to differential light shift. We saw improvement in comparison to a previous experiment \nusing red-detuned dipole traps. The anticipated lifetime could not be reached, however. We observed oscillations of the retrievability of our stored state which we explain by the evolution of the transversal component of the spinwave using Monte-Carlo simulations. In the second part we report on our new setup, built to investigate a broad range of \nexperiments regarding 2D physics on optical lattices. This field is of special interest as it allows to simulate Hamiltonians of a wide range e.g. from solid state physics and opens possibilities regarding large-scale Entanglement/one-way computing. In particular we discuss 2D Mott-insulators, 2D-Bloch oscillation induced transport phenomena and ring-exchange in a superlattice plaquette. \n
Neutral atomic gases provide fantastic opportunities for studying and controlling quantum phenomena, ranging from many-body physics to quantum computers. In our research, we use the well-known interactions between cold gases and electromagnetic radiation to harness various quantum degrees of freedom. Quantum memories, used for storing and manipulating photonic signals, will be a key component in quantum communications systems, especially in realizing critical quantum repeater infrastructure. Cold atoms have significant potential as high performance spin-wave quantum memories, due to the long storage times associated with low temperature and slow thermal diffusion. In our work, we demonstrate two memory protocols in ultracold (sometimes Bose-condensed) atoms, which hold the potential for high-performance light storage: the Autler-Townes splitting (ATS) and superradiant approaches. These methods provide a path towards practical implementations in both ground- and satellite-based quantum communications systems, and we are working on both increasing performance and developing practical implementations.
Simulating highly correlated quantum systems with classical computers exceed their capa- bilities as the system size increases. In analog quantum simulators, the system of interest is mimicked by another quantum system in a highly controllable and accessible environ- ment. Even though quantum simulations with ultracold atoms have been demonstrated successfully, ultra-low temperature regimes are experimentally challenging to achieve and still remain to be explored. New approaches to realizing ever lower temperatures, especially in Fermi systems, have been and continue to be a constant pursuit in Atomic, Molecular, and Optical Physics (AMO). Within this thesis, a new quantum gas experiment of fermionic 6Li and bosonic 166Er is presented and first results on sympathetic cooling of Li to quantum degeneracy by Er are demonstrated. The experimental apparatus is described in detail with a focus on the Li subsystem of the dual-species experiment. Standard and further developed laser cooling techniques used to produce a Magneto-Optical Trap (MOT) of Li are characterized, along with their associated vacuum system stages. In this context, a combined Optical Pumping / Transversal Cooling (OP/TC) technique of the atomic beam on the D1-line is presented, and an enhancement of the MOT loading rate by one order of magnitude is demonstrated. The architecture and building blocks of the laser system for providing resonant light at 671 nm for laser cooling of Li are detailed, and laser locking techniques for frequency stabilization and light amplification by injection locking of high-power laser diodes are presented. Special focus is placed on the introduction and characterization of a new laser- diode-independent injection locking technique, keeping spectrally pure amplified light by a periodic slave current optimization routine executed by a microcontroller. The system has been submitted for patent approval. In further steps of optical cooling of Li, a non-standard free-space Gray Molasses (GM) technique based on intensity ramps, providing temperatures as low as 13 µK, is presented. The non-standard technique is characterized and compared to the standard pulse GM approach, which typically achieves 50 µK only. Cooling steps for preparing an ultracold Li cloud in the glass cell start from an Optical Dipole Trap (ODT) loaded by a compressed Magneto-Optical Trap (cMOT) and consecutive evaporation into a 1D transport lattice of counter propagating 1064 nm laser beams. By detuning one of the lattice beams, optical transport over 1 m to the glass cell with an efficiency of 74% is demonstrated. In a combined ErLi sequence, the two species are transported to the glass cell together and loaded to 1064 nm ODTs. Sympathetic cooling of Li by forced evaporation of Er to T/TF = 0.77 ± 0.10 next to the production of an Er BEC are presented. To conclude, this work introduces a new promising dual-species quantum gas experiment and its ability for providing sympathetic cooling of Li by Er to quantum degeneracy is demon- strated. These findings are an encouraging foundation for achieving higher degeneracies by refined experimental control in pursuit of penetrating unexplored temperature regimes in quantum simulators.
This thesis describes the progress achieved towards two goals. One is the construction of a compact magneto-optical trap (MOT) apparatus, used both as a standalone undergraduate laboratory experiment and as part of a public engagement demonstration of cold atom physics. The setup, which utilises a dichroic atomic vapour laser lock (DAVLL) system plus homemade sideband generation electronics, is capable of trapping and cooling up to 8x10⁷ ⁸⁵Rb atoms in a standard six-beam laser cooling scheme. The second goal is the loading of an ultracold ensemble of ⁸⁷Rb atoms into novel optical trap geometries using a phase-only liquid crystal spatial light modulator (LC SLM) for applications to atomtronics and quantum simulation. Details of a double vacuum chamber apparatus, designed to produce the first Bose-Einstein condensates (BECs) at St Andrews, are provided. The setup incorporates a hybrid trap evaporative cooling scheme towards quantum degeneracy and reliably produces BECs of 1.9 10⁵ ⁸⁷Rb atoms. Two computational techniques, developed during the course of this project, are presented with the aim of creating flexible, smooth holographic optical traps. The first method illuminates a single SLM with overlapped, co-propagating light beams of different wavelengths to create a composite optical pattern for atom manipulation. The second uses conjugate gradient minimisation to create exceptionally high fidelity light patterns in both amplitude and phase for light in the output plane. These techniques, combined with the implementation of a light sheet into the experimental setup, are used to trap atoms in both a ring profile and in a set of narrow waveguides connected with a tunnelling barrier.
Quantum memories are an essential building block for quantum information science, and in particular for the implementation of quantum communications across long distances. A quantum memory is defined as a system capable of storing and retrieving quantum states on-demand, such as quantum bits (qubits). Atomic ensembles are good candidates for this purpose because they enables strong light-matter coupling in case of a large number of atoms. Moreover, the collective effect, enhanced in the regime of large optical depth, can lead to storage efficiency close to unity. Thus, in this thesis, a large magneto-optical trap for cesium atoms is used as a atomic medium in order to implement a quantum memory protocol based on electromagnetically induced transparency (EIT). First, the EIT phenomenon is studied through a criterion for the discrimination between the EIT and the Autler-Townes splitting models. We then report on the implementation of an EIT-based memory for photonic qubits encoded in orbital angular momentum (OAM) of light. A reversible memory for Laguerre-Gaussian modes is implemented, and we demonstrate that the optical memory preserves the handedness of the helical structure at the single-photon level. Then, a full quantum state tomography of the retrieved OAM encoded qubits is performed, giving fidelities above the classical bound. This showed that our optical memory operates in the quantum regime. Finally, we present the implementation of the so-called DLCZ protocol in our ensemble of cold atoms, enabling the generation of heralded single photons. A homodyne detection setup allows us to realize the quantum tomography of the created photonic state.
During my PhD, I participated in the full setup from scratch of an experiment that aims at cooling down and manipulating two fermionic alkaline atomic species, 6Li and 40K. Our goal is to study ultracold Fermi mixtures with mass imbalance, and to realize a flexible quantum analog simulator. In fact, for certain quantum many-body problems, such as high critical temperature superconductivity and frustrated anti-ferromagnetism, there is neither complete analytical nor numerical solution. Therefore, cold atoms systems, due to their purity and their high degree of tunability, even on their interaction itself, offer an interesting complementary point of view in the study of those phenomena. As far as the experimental setup is concerned, we built an ultra-high vacuum system, a complete and stable laser source for each species, as well as two performing atomic sources, a 6Li Zeeman slower and a 40K bidimensionnal magneto-optical trap; most of the optical and electrical quantities, as well as the imaging diagnostics, being computer controlled. Once those preliminary steps have been performed and optimized, we could obtain an efficient double magneto-optical trap, containing typically 5x10^9 atoms of 6Li and 8x10^9 atoms of 40K. In this configuration, we produced the first 6Li40K* heteronuclear molecules by photoassociation, for which we identified 70 rovibrational lines. In a second part, I describe in detail the magnetic transport of the atomic mixture, between the magneto-optical trap chamber and a science cell, located in an ultra-high vacuum region with large optical access. The complete setup, from its design to its experimental implementation and optimization, as well as the development of the program and the useful numerical diagnostics, are the heart of my work. The transport efficiency could be tested and optimized, allowing for an efficient transfer of the mixture in the science cell. Thus, after this thesis, all the experimental tools are operational in order to allow for evaporative cooling of the mixture in an optically plugged magnetic trap. Therefore, the field is open for quantum simulation and understanding of many-body problems in ultracold Fermi mixtures.