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Two-Level Interference in Nanosystems

A. Wacker

Published Jan 1, 2013• 0 citations
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Japanese Journal of Applied Physics•Sep 25, 2023•2 citations
The processes of reemission of ultrashort electromagnetic pulses by arbitrary nanosystems consisted of isolated complex atoms have been considered. The angular distributions of reemission spectra have been obtained for a series of regular nanosystems. It has been shown that the interference of the photon-emission amplitudes leads to the appearance of characteristic “diffraction” maxima. One-, two-, and three-dimensional nanostructures, as well as planar and cylindrical constructions as models of planar nanosystems and nanotubes, were used as examples that allow a simple analytical consideration.
The effect of defects in nanostructured targets on interference spectra at the reemission of attosecond electromagnetic pulses has been considered. General expressions have been obtained for calculations of spectral distributions for one-, two-, and three-dimensional multiatomic nanosystems consisting of identical complex atoms with defects such as bends, vacancies, and breaks. Changes in interference spectra by a linear chain with several removed atoms (chain with breaks) and by a linear chain with a bend have been calculated as examples allowing a simple analytical representation. Generalization to two- and three-dimensional nanosystems has been developed.
Abstract In this study, the steepest-entropy-ascent quantum thermodynamics (SEAQT) framework is used to investigate the excitation transfer (ET) dynamics of two-level nanosystems (TLSs), focusing on non-resonant processes that involve a dynamic local phonon system. In contrast to other methods based on Markovian or non-Markovian quantum master equations, SEAQT analysis always guarantees the positivity of the density operators, thus enabling the discussion of both transient and long-term dynamics of nanosystems. The findings of this study demonstrate that the relaxation time of coherent phonons, relative to the Rabi oscillation period in two TLSs, significantly affects the relaxation process of non-resonant ETs. Moreover, the degree of mutual synchronization between ET dynamics of TLSs and local (coherent) phonons can either prolong or shorten the decoherence time, presenting a way to control the coherence in nanosystems and stimulate quantum device applications.