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Japanese Journal of Applied Physics

Relaxation dynamics of nonresonant excitation transfer processes assisted by coherent phonon environment

Tenpei Morishita, Kiyoshi Kobayashi, Akira Ishikawa

Published Sep 25, 2023• 2 citations
Publisher

Abstract

Abstract In this study, the steepest-entropy-ascent quantum thermodynamics (SEAQT) framework is used to investigate the excitation transfer (ET) dynamics of two-level nanosystems (TLSs), focusing on non-resonant processes that involve a dynamic local phonon system. In contrast to other methods based on Markovian or non-Markovian quantum master equations, SEAQT analysis always guarantees the positivity of the density operators, thus enabling the discussion of both transient and long-term dynamics of nanosystems. The findings of this study demonstrate that the relaxation time of coherent phonons, relative to the Rabi oscillation period in two TLSs, significantly affects the relaxation process of non-resonant ETs. Moreover, the degree of mutual synchronization between ET dynamics of TLSs and local (coherent) phonons can either prolong or shorten the decoherence time, presenting a way to control the coherence in nanosystems and stimulate quantum device applications.

DOI
10.35848/1347-4065/acfcfa

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Abstract In this study, the steepest-entropy-ascent quantum thermodynamics (SEAQT) framework is used to investigate the excitation transfer (ET) dynamics of two-level nanosystems (TLSs), focusing on non-resonant processes that involve a dynamic local phonon system. In contrast to other methods based on Markovian or non-Markovian quantum master equations, SEAQT analysis always guarantees the positivity of the density operators, thus enabling the discussion of both transient and long-term dynamics of nanosystems. The findings of this study demonstrate that the relaxation time of coherent phonons, relative to the Rabi oscillation period in two TLSs, significantly affects the relaxation process of non-resonant ETs. Moreover, the degree of mutual synchronization between ET dynamics of TLSs and local (coherent) phonons can either prolong or shorten the decoherence time, presenting a way to control the coherence in nanosystems and stimulate quantum device applications.
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The steepest-entropy-ascent quantum thermodynamic (SEAQT) framework is used to model the decoherence that occurs during the state evolution of two different microscopic composite systems. The test cases are a $\text{two}\ensuremath{-}\text{spin}\ensuremath{-}\frac{1}{2}\ensuremath{-}\text{particle}$ composite system and a particle-photon field composite system like that experimentally studied in cavity quantum electrodynamics. The first system is used to study the characteristics of the nonlinear equation of motion of the SEAQT framework when modeling the state evolution of a microscopic composite system with particular interest in the phenomenon of decoherence. The second system is used to compare the numerical predictions of the SEAQT framework with experimental cavity quantum electrodynamic data available in the literature. For the two different numerical cases presented, the time evolution of the density operator of the composite system as well as that of the reduced operators belonging to the two constituents is traced from an initial nonequilibrium state of the composite along its relaxation towards stable equilibrium. Results show for both cases how the initial entanglement and coherence is dissipated during the state relaxation towards a state of stable equilibrium.
The equation of motion of steepest-entropy-ascent quantum thermodynamics (SEA-QT) was first postulated in the early 1980s with the intent of modeling the non-linear dynamic behavior encountered in nature, which the unitary (linear) dynamics of the Schrödinger-von Neumann equation cannot. The SEA-QT equation is used here to model the decoherence phenomenon between two distinguishable and indivisible elementary constituents of type spin–½ (e.g., quantum bits or qubits). The resulting set of non-linear, first-order differential equations is solved with a fourth-order-Runge-Kutta routine provided by Matlab®. The time evolution of the state of the composite system as well as that of the reduced and locally-perceived states of the two constituents are traced from an initial non-equilibrium state of the composite along its relaxation towards stable equilibrium at constant system energy. An entangled and generally coherent, initial non-equilibrium state of the composite quantum system is prepared using a heuristic approach, which consists of randomly and homogeneously generating an initial point on the Bloch sphere for each of the constituents and then using a weighted average of their projections to arrive at an initial state for the composite. Results show how the initial entanglement and coherence between the two spin–½ constituents are reduced during relaxation towards a state of stable equilibrium. When the two particles are non-interacting, the initial coherence is lost once stable equilibrium is reached. When they are interacting, the coherence in the final stable equilibrium state is only that due to the interaction.
Open quantum systems are studied from the thermodynamical point of view unifying the principle of maximum informational entropy and the hypothesis of relaxation times hierarchy. The result of the unification is a non-Markovian and local-in-time master equation that provides a direct connection for dynamical and thermodynamical properties of open quantum systems. The power of the approach is illustrated by the application to the damped harmonic oscillator and the damped driven two-level system, resulting in analytical expressions for the non-Markovian and nonequilibrium entropy and inverse temperature.
Abstract Decoherence has been observed to be one of the main limitations to build a practical quantum computer. This is because the qubits that conform it rapidly lose the entanglement and correlations existent among them due to interactions with the environment. In this work, the relaxation time of a Transmon qubit interacting with an environment is predicted by using the steepest-entropy-ascent quantum thermodynamics framework and the Lindblad master equation. For the study it is considered that the environment behaves as a thermal bath composed of a collection of harmonic oscillators. Results show that the qubit processes from a non-equilibrium state to a state of stable equilibrium, exchanging energy with the thermal bath during the process. In addition, the prediction of the relaxation time of the qubit is in agreement with experimental results obtained from the literature. The decoherence time is also accurately predicted by the models.
We study the decoherence dynamics of a superconducting qubit coupled to a quantum two-level system (TLS) in addition to its weak coupling to a background environment [1]. We identify two weak-coupling regimes, which differ by the relation between qubit and TLS decoherence times, and a strong coupling regime. We find expressions for the qubit decoherence rates in the weak-coupling regimes. For a weakly coupled and strongly dissipative TLS we find that the qubit dynamics is markovian, whereas for a weakly dissipative TLS the qubit dynamics shows non-markovian behavior. In the strong-coupling regime we study the driven qubit dynamics and we analyze the differences from standard Rabi-oscillations due to the coupling to the quantum TLS [2]. In doing so we identify signatures in the qubit dynamics that can be used to characterize the TLS. We also investigate the possibility of using environmental TLSs with long coherence times for quantum information processing [3]. By using the Josephson junction as a bus and the TLSs in the environment as qubits, we demonstrate that initialization, a universal set of quantum gates, and read-out of the TLSs can be implemented, even though the TLSs themselves cannot be directly accessed.